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Related papers: Exciton mapping at subwavelength scales in two-dim…

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Excitons in thin layers of semiconducting transition metal dichalcogenides are highly subject to the strongly modified Coulomb electron-hole interaction in these materials. Therefore, they do not follow the model system of a two-dimensional…

Exciton-polariton modes arising from interaction between bound excitons in monolayer thin semiconductor sheets and photons in a Fabry-Perot microcavity are considered theoretically. We calculate the dispersion curves, mode lifetimes, Rabi…

Mesoscale and Nanoscale Physics · Physics 2015-12-30 Mikhail I. Vasilevskiy , Darío G. Santiago-Pérez , Carlos Trallero-Giner , Nuno M. R. Peres , Alexey Kavokin

Monolayer transition-metal dichalcogenides are direct gap semiconductors with great promise for optoelectronic devices. Although spatial correlation of electrons and holes plays a key role, there is little experimental information on such…

Materials Science · Physics 2015-06-23 A. T. Hanbicki , M. Currie , G. Kioseoglou , A. L. Friedman , B. T. Jonker

Optical properties of single-wall carbon nanotubes (SWCNTs) for light polarized parallel to the nanotube axis have been extensively studied, whereas their response to light polarized perpendicular to the nanotube axis has not been well…

Mesoscale and Nanoscale Physics · Physics 2019-01-23 Fumiya Katsutani , Weilu Gao , Xinwei Li , Yota Ichinose , Yohei Yomogida , Kazuhiro Yanagi , Junichiro Kono

The development of van der Waals heterostructures has introduced unconventional phenomena that emerge at atomically precise interfaces. For example, interlayer excitons in two-dimensional transition metal dichalcogenides show intriguing…

Mesoscale and Nanoscale Physics · Physics 2024-05-02 N. Fang , Y. R. Chang , S. Fujii , D. Yamashita , M. Maruyama , Y. Gao , C. F. Fong , D. Kozawa , K. Otsuka , K. Nagashio , S. Okada , Y. K. Kato

We combine linear and non-linear optical spectroscopy at 4K with ab initio calculations to study the electronic bandstructure of MoSe2 monolayers. In 1-photon photoluminescence excitation (PLE) and reflectivity we measure a separation…

Materials Science · Physics 2015-11-05 G. Wang , I. C. Gerber , L. Bouet , D. Lagarde , A. Balocchi , M. Vidal , E. Palleau , T. Amand , X. Marie , B. Urbaszek

Neutral and charged excitons (trions) in atomically-thin materials offer important capabilities for photonics, from ultrafast photodetectors to highly-efficient light-emitting diodes and lasers. Recent studies of van der Waals (vdW)…

Mesoscale and Nanoscale Physics · Physics 2020-08-04 Jaydeep Joshi , Tong Zhou , Sergiy Krylyuk , Albert V. Davydov , Igor Zutic , Patrick M. Vora

Exciton condensation, the Bose-Einstein-like condensation of quasibosonic particle-hole pairs, has been the subject of much theoretical and experimental interest and holds promise for ultra-energy-efficient technologies. Recent advances in…

Excitons - the particle-hole bound states - composed of localized electron-hole states in semiconducting systems are crucial to explaining the optical spectrum. Spectroscopic measurements can contain signatures of these two particle bound…

Mesoscale and Nanoscale Physics · Physics 2018-06-19 Avinash Rustagi , Alexander F. Kemper

We report a new dark exciton in monolayer MoS$_2$ using second harmonic generation spectroscopy. Hereby, the spectrally dependent second harmonic generation intensity splits into two branches, and an anticrossing is observed at $\sim$ 25…

Mesoscale and Nanoscale Physics · Physics 2024-08-22 Chenjiang Qian , Viviana Villafañe , Pedro Soubelet , Peirui Ji , Andreas V. Stier , Jonathan J. Finley

We have studied emission properties of high-density excitons in single-walled carbon nanotubes through nonlinear photoluminescence excitation spectroscopy. As the excitation intensity was increased, all emission peaks arising from different…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 Y. Murakami , J. Kono

Coherent coupling between excitons is at the heart of many-body interactions with transition metal dichalcogenide (TMD) heterostructures as an emergent platform for the investigation of these interactions. We employ multi-dimensional…

Mesoscale and Nanoscale Physics · Physics 2022-01-05 Torben L. Purz , Eric W. Martin , Pasqual Rivera , William G. Holtzmann , Xiaodong Xu , Steven T. Cundiff

Various properties of interlayer excitons in double-layer transition metal dichalcogenides quantum dots are analyzed using a low-energy effective Hamiltonian with Coulomb interaction. We solve the single-particle Hamiltonian with and…

Mesoscale and Nanoscale Physics · Physics 2024-08-15 Xiang Liu , Zheng Tao , Wenchen Luo , Tapash Chakraborty

Using accurate first-principles calculations based on many-body perturbation theory we predict that two-dimensional MoS$_2$ hosts edge excitons with universal character, intrinsic to the existence of edges and lying well below the onset of…

Mesoscale and Nanoscale Physics · Physics 2020-05-06 Pino D'Amico , Marco Gibertini , Deborah Prezzi , Daniele Varsano , Andrea Ferretti , Nicola Marzari , Elisa Molinari

Two-dimensional (2D) monolayer phosphorene, a 2D system with quasi-one-dimensional (quasi-1D) excitons, provides a unique 2D platform for investigating the dynamics of excitons in reduced dimensions and fundamental many-body interactions.…

Materials Science · Physics 2016-02-03 Renjing Xu , Jiong Yang , Ye Win Myint , Jiajie Pei , Han Yan , Fan Wang , Yuerui Lu

The presence of electron energy loss (EELS) peak is proposed theoretically in molybdenum disulfide (MoS2) nanosheets. Using density functional theory simulations and calculations, one EELS peak is identified in the visible energy range, for…

Two-dimensional group-VI transition metal dichalcogenide semiconductors, such as MoS2, WSe2 and others, exhibit strong light-matter coupling and possess direct band gaps in the infrared and visible spectral regimes, making them potentially…

Mesoscale and Nanoscale Physics · Physics 2020-03-03 Thomas Mueller , Ermin Malic

Excitons play an essential role in the optical response of two-dimensional materials. These are bound states showing up in the band gaps of many-body systems and are conceived as quasiparticles formed by an electron and a hole. By…

Momentum resolved electron energy-loss spectroscopy was used to measure the dispersions of excitons in a free-standing monolayer of WSe2. Besides the parabolically dispersed valley excitons, a sub-gap dispersive exciton was observed at…

Materials Science · Physics 2020-03-04 Jinhua Hong , Ryosuke Senga , Thomas Pichler , Kazu Suenaga

Chemical vapor deposition (CVD) allows lateral edge epitaxy of transition metal dichalcogenide heterostructures with potential applications in optoelectronics. Critical for carrier and exciton transport is the quality of the two materials…