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Entangled photons exhibit non-classical light-matter interactions that create new opportunities in materials and molecular science. For example, in entangled two-photon absorption, the intensity-dependence scales linearly as if only one…

Optics · Physics 2020-05-15 Szilard Szoke , Hanzhe Liu , Bryce P. Hickam , Manni He , Scott K. Cushing

We investigate dynamics of atomic and molecular systems exposed to intense, shaped chaotic fields and a weak femtosecond laser pulse theoretically. As a prototype example, the photoionization of a hydrogen atom is considered in detail. The…

Quantum Physics · Physics 2015-05-18 Kamal P Singh , Jan M Rost

A moderately intense $450$ fs laser pulse is used to create rotational wave packets in gas phase $\rm{I_2}$ molecules. The ensuing time-dependent alignment, measured by Coulomb explosion imaging with a delayed probe pulse, exhibits the…

The way molecules absorb, transfer, and emit light can be modified by coupling them to optical cavities. The extent of the modification is often defined by the cavity-molecule coupling strength, which depends on the number of coupled…

Optics · Physics 2021-06-11 Adarsh B Vasista , Kishan S Menghrajani , William L Barnes

The ability to directly follow and time resolve the rearrangement of the nuclei within molecules is a frontier of science that requires atomic spatial and few-femtosecond temporal resolutions. While laser induced electron diffraction can…

Interfaces between molecules and 2D materials exhibit energy-driven functionalities, wherein charge transfer directs molecular motion. Unlike equilibrium systems, where molecular assemblies settle into static configurations, continuous…

We extend the semiclassical two-step model for strong-field ionization that describes quantum interference and accounts for the Coulomb potential beyond the semiclassical perturbation theory to the hydrogen molecule. In the simplest case of…

Atomic Physics · Physics 2019-03-27 N. I. Shvetsov-Shilovski , M. Lein , K. Tőkési

Torque is ubiquitous in many molecular systems, including collisions, chemical reactions, vibrations, electronic excitations and especially rotor molecules. We present a straightforward theoretical method based on forces acting on atoms and…

Chemical Physics · Physics 2016-11-23 Rui-Qin Zhang , Yan-Ling Zhao , Fei Qi , Klaus Hermann , Michel A. Van Hove

When polarized electrons traverse a region where the laser light is focused their polarization varies even if their energy and direction of motion are not changed. This effect is due to interference of the incoming electron wave and an…

High Energy Physics - Phenomenology · Physics 2009-10-30 G. L. Kotkin , H. Perlt , V. G. Serbo

The nuclear interactions of atomic and low energy antiprotons are studied. Measurements of level shifts and widths in the lightest elements are analyzed and compared with new results obtained in heavy nuclei. Simple geometric properties of…

Nuclear Theory · Physics 2017-08-23 S. Wycech

Photodissociation of a molecule produces a spatial distribution of photofragments determined by the molecular structure and the characteristics of the dissociating light. Performing this basic chemical reaction at ultracold temperatures…

Atomic Physics · Physics 2018-01-24 M. McDonald , I. Majewska , C. -H. Lee , S. S. Kondov , B. H. McGuyer , R. Moszynski , T. Zelevinsky

We connect the observed under-abundances of Li and Be in dwarfs, with recent results on nuclear cross sections at low energies: for collisions of protons with atomic or molecular targets, the measured cross sections seem too high with…

Astrophysics · Physics 2015-06-24 V. Castellani , G. Fiorentini , O. Straniero , B. Ricci

We address the feasibility of imaging geometric and orbital structure of a polyatomic molecule on an attosecond time-scale using the laser induced electron diffraction (LIED) technique. We present numerical results for the highest molecular…

The development of attosecond technology has enabled the real-time observation of coherent electron motion in atoms, molecules and condensed phases. Experimentally, it is now possible to generate laser pulses of durations of only a few tens…

Chemical Physics · Physics 2017-05-18 David Ayuso

Interaction of ultera-short laser pulses with a dense cold plasma is investigated. Due to high density, of plasma, quantum effects such that Bohm potential and quantum pressure should be considered. The results reveal that electron density…

Plasma Physics · Physics 2019-04-02 Sepideh Dashtestani , Hamidreza Mohammadi

We attempt to provide physical interpretations of light-induced desorption phenomena that have recently been observed for alkali atoms on glass surfaces of alkali vapor cells used in atomic physics experiments. We find that the observed…

Other Condensed Matter · Physics 2007-05-23 Atsushi Hatakeyama , Markus Wilde , Katsuyuki Fukutani

We use orthogonally polarized two-colour (OTC) laser pulses to separate quantum paths in multiphoton ionization of Ar atoms. Our OTC pulses consist of 400~nm and 800~nm light at a relative intensity ratio of 10:1. We find a hitherto…

We propose a two-dimensional interferometry based on electron wave packet interference with a cycle-shaped orthogonally polarized two-color laser field. With such method, sub-cycle and inter-cycle interferences can be disentangled into…

Atomic Physics · Physics 2015-06-04 Xinhua Xie

Strong magnetic fields have a large impact on the dynamics of molecules. In addition to the changes of the electronic structure, the nuclei are exposed to the Lorentz force with the magnetic field being screened by the electrons. In this…

Chemical Physics · Physics 2021-07-28 Laurens D. M. Peters , Tanner Culpitt , Laurenz Monzel , Erik I. Tellgren , Trygve Helgaker

We study the disintegration of nuclei by strong electromagnetic fields induced by ultrarelativistic heavy ions. The proposed multi-step model includes 1) the absorption of a virtual photon by a nucleus, 2) intranuclear cascades of produced…

Nuclear Theory · Physics 2008-11-26 I. A. Pshenichnov , I. N. Mishustin , J. P. Bondorf , A. S. Botvina , A. S. Iljinov