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Ordinary band structure calculations of quantum materials often incorrectly predicted metallic, instead of insulating electronic structure, motivating Mott-Hubbard strong electron correlation as a gapping mechanism. More recently, allowing…

Materials Science · Physics 2024-08-02 Jia-Xin Xiong , Xiuwen Zhang , Alex Zunger

We examine the phase diagram of the extended Hubbard model on a square lattice, for both attractive and repulsive nearest-neighbor interactions, using CDMFT+HFD, a combination of Cluster Dynamical Mean Field theory (CDMFT) and a…

Strongly Correlated Electrons · Physics 2024-06-05 Sarbajaya Kundu , David Sénéchal

Density functional theory (DFT) embedding provides a formally exact framework for interfacing correlated wave-function theory (WFT) methods with lower-level descriptions of electronic structure. Here, we report techniques to improve the…

Chemical Physics · Physics 2015-06-12 Jason D. Goodpaster , Taylor A. Barnes , Frederick R. Manby , Thomas F. Miller

We address the nature of the Mott transition in the Hubbard model at half-filling using cluster Dynamical Mean Field Theory (DMFT). We compare cluster DMFT results with those of single site DMFT. We show that inclusion of the short range…

Strongly Correlated Electrons · Physics 2009-11-13 H. Park , K. Haule , G. Kotliar

Metal-insulator transition materials such as NbO2 have generated much excitement in recent years for their potential applications in computing and sensing. NbO2 has generated considerable debate over the nature of the phase transition, and…

We present a new approach based on the static density functional theory (DFT) to describe paramagentic MnO, which is a representative paramagnetic Mott insulator. We appended the spin noncollinearity and the canonical ensemble to the…

Strongly Correlated Electrons · Physics 2020-07-14 Sangmoon Yoon , Seoung-Hun Kang , Sangmin Lee , Kuntae Kim , Jeong-Pil Song , Miyoung Kim , Young-Kyun Kwon

The concept of electronic correlations plays an important role in modern condensed matter physics. It refers to interaction effects which cannot be explained within a static mean-field picture as provided by Hartree-Fock theory. Electronic…

Strongly Correlated Electrons · Physics 2015-03-17 Dieter Vollhardt

The nearly free electron metal next to a localized Mott insulating state has been recently proposed as a way to probe Kondo lattice physics and to gain insight into how the two extremes of localized and delocalized electron states interact…

Dynamical mean-field theory (DMFT) has been employed in conjunction with density functional theory (DFT+DMFT) to investigate the metal-insulator transition (MIT) of strongly correlated $3d$ electrons due to quantum confinement. We shed new…

Strongly Correlated Electrons · Physics 2021-06-02 A. D. N. James , M. Aichhorn , J. Laverock

Reports of metallic behavior in two-dimensional (2D) systems such as high mobility metal-oxide field effect transistors, insulating oxide interfaces, graphene, and MoS2 have challenged the well-known prediction of Abrahams, et al. that all…

Mesoscale and Nanoscale Physics · Physics 2015-05-27 M. S. Osofsky , S. C. Hernández , A. Nath , V. D. Wheeler , S. Walton , C. M. Krowne , D. K. Gaskill

The iterative perturbation theory of the dynamical mean field theory is generalized to arbitrary electron occupation in case of multi-orbital Hubbard bands. We present numerical results of doubly degenerate Eg bands in a simple cubic…

Strongly Correlated Electrons · Physics 2007-12-06 Takeo Fujiwara , Susumu Yamamoto , Yasushi Ishii

The interplay between band and atomic aspects in materials with co-existing wide-band and flat-band states, or wide-band and effectively dispersionless electronic states is increasingly expected to lead to novel behavior. Using dynamical…

Strongly Correlated Electrons · Physics 2025-08-12 M. S. Laad , S. R. Hassan

We report on optical properties of various polymorphs of hafnia predicted within the framework of density functional theory. The full potential linearised augmented plane wave method was employed together with the Tran-Blaha modified…

Materials Science · Physics 2016-09-21 Pavel Ondračka , David Holec , David Nečas , Lenka Zajíčková

Dynamical mean-field theory (DMFT) is a non-perturbative technique for the investigation of correlated electron systems. Its combination with the local density approximation (LDA) has recently led to a material-specific computational scheme…

Strongly Correlated Electrons · Physics 2009-11-10 D. Vollhardt , K. Held , G. Keller , R. Bulla , Th. Pruschke , I. A. Nekrasov , V. I. Anisimov

Simulations are carried out based on the dynamical mean-field theory (DMFT) in order to investigate the properties of correlated thin films for various values of the chemical potential, temperature, interaction strength, and applied…

Strongly Correlated Electrons · Physics 2016-05-04 Petar Bakalov , Davoud Nasr Esfahani , Lucian Covaci , Francois Peeters , Jacques Tempere , Jean-Pierre Locquet

Density of states, dynamic (optical) conductivity and phase diagram of paramagnetic two-dimensional Anderson-Hubbard model with strong correlations and disorder are analyzed within the generalized dynamical mean-field theory (DMFT+Sigma…

Strongly Correlated Electrons · Physics 2010-05-17 E. Z. Kuchinskii , N. A. Kuleeva , I. A. Nekrasov , M. V. Sadovskii

We explore the phase diagram of the Mott metal-insulator transition (MIT), focusing on the effects of particle-hole asymmetry (PHA) in the single-band Hubbard model. Our dynamical mean-field theory (DMFT) study reveals that the introduction…

Strongly Correlated Electrons · Physics 2025-09-26 Mateus Marques , Bruno M. de Souza Melo , Alexandre R. Rocha , Caio Lewenkopf , Luis G. G. V. Dias da Silva

The density driven Mott transition is studied by means of Dynamical Mean-Field Theory in the Hubbard-Holstein model, where the Hubbard term leading to the Mott transition is supplemented by an electron-phonon (e-ph) term. We show that an…

Strongly Correlated Electrons · Physics 2007-08-07 M. Capone , G. Sangiovanni , C. Castellani , C. Di Castro , M. Grilli

Mott insulators can be portrayed as "unsuccessful metals": systems in which a strong Coulomb repulsion prevents charge conduction notwithstanding the metal-like density of conduction electrons. The possibility to unlock such large density…

Strongly Correlated Electrons · Physics 2016-10-24 G. Mazza , A. Amaricci , M. Capone , M. Fabrizio

In this Letter we report the first LDA+DMFT (method combining Local Density Approximation with Dynamical Mean-Field Theory) results of magnetic and spectral properties calculation for paramagnetic phases of FeO at ambient and high pressures…

Strongly Correlated Electrons · Physics 2010-11-03 A. ~O. ~Shorikov , Z. ~V. ~Pchelkina , V. ~I. ~Anisimov , S. ~L. ~Skornyakov , M. ~A. ~Korotin