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By uncovering novel aspects of second harmonic generation in aluminum we show that there are unusual and remarkable consequences of resonant absorption, namely an unexpectedly critical role that bound electrons play for light-matter…

We measure nonlinear optical scattering from individual Au nanorods excited by ultrafast laser pulses on resonance with their longitudinal plasmon mode. Isolating single rods removes inhomogeneous broadening and allows the measurement of a…

Materials Science · Physics 2009-11-11 Matthew Pelton , Mingzhao Liu , Sungnam Park , Norbert F. Scherer , Philippe Guyot-Sionnest

Spherical gold nanoclusters are grown by 1.8 MeV Au++ ion implantation into an amorphous silica matrix and subsequent air annealing at 873 K. Ultraviolet and visible light absorption confirms the presence of a dipolar surface plasmon peak…

Other Condensed Matter · Physics 2007-05-23 Daniel B. Murray , S. Dhara , T. R. Ravindran , K. G. M. Nair , S. Kalavathi , Lucien Saviot , Eugene Duval

The optical transmission spectra of a series of micro-ring resonators (MRRs) are studied following the implantation of gold (Au) ions and subsequent thermal annealing, at temperatures between 500 {\deg}C and 700 {\deg}C. Whilst we find that…

Atomically precise thiolate-stabilized gold nanoclusters are currently of interest for many cross-disciplinary applications in chemistry, physics and molecular biology. Very recently, synthesis and electronic properties of "nanoalloy"…

Atomic and Molecular Clusters · Physics 2011-09-05 Sami Malola , Hannu Häkkinen

Electronic excitations in metallic nanoparticles in the optical regime that have been of great importance in surface enhanced spectroscopy and emerging applications of molecular plasmonics, due to control and confinement of electromagnetic…

Mesoscale and Nanoscale Physics · Physics 2015-10-28 Marouane Salhi , Ali Passian , George Siopsis

Metal nanostructures have received significant attention in recent years owing to their peculiar physical and chemical properties, which span a wide range of practical applications in a variety of scientific and engineering fields. Herein,…

Nonlinear optical absorption of light by materials are weak due to its perturbative nature, although a strong nonlinear response is of crucial importance to applications in optical limiting and switching. Here we demonstrate experimentally…

We report experiments on surface nanopatterning of Si targets which are irradiated with 2 keV Ar + ions impinging at near-glancing incidence, under concurrent co-deposition of Au impurities simultaneously extracted from a gold target by the…

Mesoscale and Nanoscale Physics · Physics 2016-03-30 B. Moon , S. Yoo , J. -S. Kim , S. J. Kang , J. Muñoz-García , R. Cuerno

We consider light propagation in a silicon dioxide substrate with implanted ${\mathrm{Er}}^{3+}$ ions and silver nanoparticles that are randomly and homogeneously distributed in the substrate. When their densities are large enough, the…

Optics · Physics 2024-12-17 Igor Kuzmenko , Y. Avishai , Y. B. Band

Electron beam imaging is a common technique used for characterizing the morphology of plasmonic nanostructures. During the imaging process, the electron beam interacts with traces of organic material in the chamber and produces a well-know…

Mesoscale and Nanoscale Physics · Physics 2013-11-13 Mingxia Song , Gérard Colas-des-Francs , Alexandre Bouhelier

The shape of metal nanoparticles embedded in dielectric matrices influences the optical properties of the composite material. Swift heavy ion irradiation can induce a controllable shape transformation in gold and other metals embedded in…

Materials Science · Physics 2022-04-22 Aleksi A. Leino , Ville E. Jantunen , Flyura Djurabekova

We present an intuitive analytical model for extraordinary optical transmission (EOT) through corrugated metallic films. In the framework of this model, EOT emerges from standing wave resonances of the different diffraction orders, and is…

Optics · Physics 2010-11-17 Ilai Schwarz , Nitzan Livneh , Ronen Rapaport

The review is devoted to a discussion of new (and often unexpected) aspects of the old problem of elastic light scattering by small metal particles, whose size is comparable to or smaller than the thickness of the skin layer. The main focus…

Optics · Physics 2020-09-21 Michael I. Tribelsky , Andrey E. Miroshnichenko

Controlling ultraviolet light at the nanoscale using optical Mie resonances holds great promise for a diverse set of applications, such as lithography, sterilization, and biospectroscopy. However, Mie resonances hosted by dielectric…

The last two decades have witnessed various experiments reporting very unusual magnetic properties of ensembles of gold nanoparticles surrounded by organic ligands, including ferromagnetic, paramagnetic, or (large) diamagnetic responses.…

Mesoscale and Nanoscale Physics · Physics 2018-11-14 Mauricio Gómez Viloria , Guillaume Weick , Dietmar Weinmann , Rodolfo A. Jalabert

We investigate plasmon resonances in gold nanoparticles to enhance the quantum yield of upconverting materials. For this purpose, we use a rate equation model that describes the upconversion of trivalent erbium based upconverters. Changes…

We report room temperature lasing in two-dimensional diffractive lattices of silver and gold plasmon particle arrays embedded in a dye-doped polymer that acts both as waveguide and gain medium. As compared to conventional dielectric…

Optics · Physics 2014-09-26 A. Hinke Schokker , A. Femius Koenderink

Absorption cross-section spectra for gold nanoparticles were calculated using fully quantum Stochastic Density Functional Theory and a classical Finite-Difference Time Domain (FDTD) Maxwell solver. Spectral shifts were monitored as a…

Atomic and Molecular Clusters · Physics 2018-09-26 Samuel Hernandez , Yantao Xia , Vojtěch Vlček , Robert Boutelle , Roi Baer , Eran Rabani , Daniel Neuhauser

We have observed the compensation of loss in metal by gain in interfacing dielectric in the mixture of aggregated silver nanoparticles and rhodamine 6G dye. The demonstrated six-fold enhancement of the Rayleigh scattering is the evidence of…

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