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Chemical manifestations of strong light-matter coupling have been recently subject of intense experimental and theoretical studies. Here we review the present status of this field. Section 1 is an introduction to molecular polaritonics and…

Chemical Physics · Physics 2021-12-15 Tao E. Li , Bingyu Cui , Joseph E. Subotnik , Abraham Nitzan

Investigating the interaction of electron beams with materials and light has been a field of research since more than a century. The field was advanced theoretically by the raise of quantum mechanics and technically by the introduction of…

Optics · Physics 2017-10-11 Nahid Talebi

Two-photon optical transitions combined with long-range dipole-dipole interactions can be used for the coherent manipulation of collective metastable states composed of different atoms. We show that it is possible to induce optical…

Quantum Physics · Physics 2007-05-23 M. D. Lukin , P. R. Hemmer

We present a theory of cooperative light scattering valid in any dimension: connecting theories for an open line, open plane, and open space in the non-relativistic regime. This theory includes near-field and dipole-orientation effects,…

Quantum Physics · Physics 2017-03-29 Tyler Hill , Barry C. Sanders , Hui Deng

Superradiance, in which the collective behavior of emitters can generate enhanced radiative decay, was first predicted by a model, now known as the Dicke model, that contains a collection of two-level systems (the emitters) all interacting…

Optics · Physics 2025-02-05 Xuecheng Tao , John P. Philbin , Prineha Narang

We report generation of a new quantum interference effect in spontaneous emission from a resonantly driven system of two identical two-level atoms due to the spatial variation of the laser phase at the positions of the atoms. This…

Quantum Physics · Physics 2008-10-06 Sumanta Das , G. S. Agarwal , Marlan O. Scully

We investigate the collective scattering of coherent light from a thermal alkali-metal vapor with temperatures ranging from 350 to 450 K, corresponding to average atomic spacings between $0.7 \lambda$ and $0.1 \lambda$. We develop a…

Quantum Physics · Physics 2021-07-28 Sofia Ribeiro , Thomas F. Cutler , Charles S. Adams , Simon A. Gardiner

Experiments show that light-matter strong coupling affects chemical properties, though the underlying mechanism remains unclear. We present an ab initio quantum electrodynamics coupled cluster method for the collective strong coupling…

Chemical Physics · Physics 2024-11-18 Matteo Castagnola , Marcus T. Lexander , Henrik Koch

The competition between electron localization and de-localization in Mott insulators underpins the physics of strongly-correlated electron systems. Photo-excitation, which re-distributes charge between sites, can control this many-body…

Strongly Correlated Electrons · Physics 2015-08-05 S. Wall , D. Brida , S. R. Clark , H. P. Ehrke , D. Jaksch , A. Ardavan , S. Bonora , H. Uemura , Y. Takahashi , T. Hasegawa , H. Okamoto , G. Cerullo , A. Cavalleri

We theoretically investigate an ensemble of three-level room-temperature atoms in a two-mode optical cavity, focusing on the case of counterpropagating light fields. We find that in the limit of large detunings the problem admits relatively…

Quantum Physics · Physics 2016-09-12 G. T. Hickman

Very often it is an implied paradigm of molecular magnetism that magnetic molecules in a crystal interact so weakly that measurements of dc magnetic observables reflect ensemble properties of single molecules. But the number of cases where…

Strongly Correlated Electrons · Physics 2016-03-02 J. Schnack

Nowadays the most intriguing features of wave particle complementarity of single photon is exemplified by the famous Wheeler's delayed choice experiment in linear optics, nuclear magnetic resonance and integrated photonic device systems.…

We discover a surprising relation between the collective motion of nucleons within atomic nuclei, traditionally understood to be driven by long-range correlations, and short-range nucleon-nucleon interactions. Specifically, we find that…

We study the collective interaction of excitons in closely spaced artificial molecules and arrays of nearly identical quantum dots with the electromagnetic modes. We discuss how collective fluorescence builds up in the presence of a small…

Mesoscale and Nanoscale Physics · Physics 2007-06-18 Anna Sitek , Pawel Machnikowski

The cooperative modification of spontaneous radiative decay is a paradigmatic many-emitter effect in quantum optics. So far its experimental realization has involved interactions mediated by rapidly escaping photons that do not play an…

Quantum Physics · Physics 2025-01-22 Youngshin Kim , Alfonso Lanuza , Dominik Schneble

In weakly bound diatomic molecules, energy levels are closely spaced and thus more susceptible to mixing by magnetic fields than in the constituent atoms. We use this effect to control the strengths of forbidden optical transitions in…

Atomic Physics · Physics 2015-12-22 B. H. McGuyer , M. McDonald , G. Z. Iwata , W. Skomorowski , R. Moszynski , T. Zelevinsky

The question whether the linear absorption spectra of metal clusters can be interpreted as density oscillations (collective ``plasmons'') or can only be understood as transitions between distinct molecular states is still a matter of debate…

Atomic and Molecular Clusters · Physics 2009-11-07 S. Kümmel , K. Andrae , P. -G. Reinhard

The rapidly developing and converging fields of polaritonic chemistry and quantum optics necessitate a unified approach to predict strongly-correlated light-matter interactions with atomic-scale resolution. Combining concepts from both…

Quantum Physics · Physics 2018-09-19 Johannes Flick , Prineha Narang

We calculate the dynamics of one and two two-level atoms interacting with the electromagnetic vacuum field in the vicinity of an optical nanofiber without making either the Born or the Markov approximations. We use a constant dielectric…

Quantum Physics · Physics 2023-07-19 Alberto Del Ángel , P. Solano , P. Barberis-Blostein

In open-shell atoms and ions, processes such as photoionization, combination (Raman) scattering, electron scattering and recombination, are often mediated by many-electron compound resonances. We show that their interference (neglected in…

Atomic Physics · Physics 2015-05-14 V. V. Flambaum , M. G. Kozlov , G. F. Gribakin
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