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We explore the nonlinear response of tailor-cut light-matter hybrid states in a novel regime, where both the Rabi frequency induced by a coherent driving field and the vacuum Rabi frequency set by a cavity field are comparable to the…

Quantum Physics · Physics 2021-05-05 J. Mornhinweg , M. Halbhuber , C. Ciuti , D. Bougeard , R. Huber , C. Lange

Recent experiments in polariton chemistry have demonstrated that reaction rates can be modified by vibrational strong coupling to an optical cavity mode. Importantly, this modification only occurs when the frequency of the cavity mode is…

Chemical Physics · Physics 2023-05-15 Marit R. Fiechter , Johan E. Runeson , Joseph E. Lawrence , Jeremy O. Richardson

We apply a mixed quantum-classical (MQC) approach to the quantum Rabi model, involving a classical optical field coupled self-consistently to a quantum two-level system. Under the rotating wave approximation, we analytically show this…

Quantum Physics · Physics 2025-06-13 Ming-Hsiu Hsieh , Roel Tempelaar

Cavity polaritons derived from the strong light-matter interaction at the quantum level provide a basis for efficient manipulation of quantum states via cavity field. Polaritons with narrow linewidth and long lifetime are appealing in…

Quantum Physics · Physics 2024-05-24 Yuwei Lu , Jingfeng Liu , Haoxiang Jiang , Zeyang Liao

Recent years have seen significant developments in the study of strong light-matter coupling including the control of chemical reactions by altering the vibrational normal modes of molecules. In the vibrational strong coupling regime the…

Quantum Physics · Physics 2021-08-27 John Bonini , Johannes Flick

The optical hybridization of the electronic states in strongly coupled molecule-cavity systems have revealed unique properties such as lasing, room temperature polariton condensation, and the modification of excited electronic landscapes…

Breaking the time-reversal symmetry of light is of great importance for fundamental physics and has attracted increasing interest in the study of non-reciprocal photonic devices. Here, we experimentally demonstrate a chiral cavity QED…

Quantum Physics · Physics 2023-04-20 Pengfei Yang , Ming Li , Xing Han , Hai He , Gang Li , Chang-Ling Zou , Pengfei Zhang , Yuhua Qian , Tiancai Zhang

The extended quantum Rabi models make a significant contribution to understand the quantum nature of the atom-light interaction. We transform two kinds of extended quantum Rabi model, anisotropic Rabi model and asymmetric Rabi model, into…

Quantum Physics · Physics 2022-07-20 Yibo Liu , Lijun Mao , Yunbo Zhang

We experimentally resolve the dispersion of multiple vibro-polariton modes issued from the strong coupling of different vibrational bands of the methylene group (CH2) in a 2.56$\mu$m thick polyethylene film with the confined modes of a…

We study a quantum dot strongly coupled to a single high-finesse optical microcavity mode. We use a rotating wave approximation method, commonly used in ion-laser interactions, tegether with the Lamb-Dicke approximation to obtain an…

Other Condensed Matter · Physics 2008-05-26 Jonas Larson , Hector Moya-Cessa

We define the anisotropic Rabi model as the generalization of the spin-boson Rabi model: The Hamiltonian system breaks the parity symmetry; the rotating and counter-rotating interactions are governed by two different coupling constants; a…

Quantum Physics · Physics 2014-06-18 Qiong-Tao Xie , Shuai Cui , Jun-Peng Cao , Luigi Amico , Heng Fan

We study quantum optics with the atoms coupled to the quantized electromagnetic (EM) field in a non-inertial reference frame by making use of quantum field theory in curved spacetime. We rigorously establish the microscopic model for a…

Quantum Physics · Physics 2015-08-03 Sheng-Wen Li , Z. H. Wang , Lan Zhou , C. P. Sun

We employ an exact quantum mechanical simulation technique to investigate a model of cavity-modified chemical reactions in the condensed phase. The model contains the coupling of the reaction coordinate to a generic solvent, cavity coupling…

Quantum Physics · Physics 2023-07-03 Lachlan P. Lindoy , Arkajit Mandal , David R. Reichman

A simple way to calculate Rabi frequencies is outlined for interactions of atomic or nuclear multipole moments with laser fields that focuses on their relative geometry. The resulting expression takes the form of a dot product between the…

Quantum Physics · Physics 2025-11-06 Wesley C. Campbell

The quantum Rabi model describes the interaction between a two-level quantum system and a single bosonic mode. We propose a method to perform a quantum simulation of the quantum Rabi model introducing a novel implementation of the two-level…

The multi-level system $^{55}$Mn$^{2+}$ is used to generate two pseudo-harmonic level systems, as representations of the same electronic sextuplet at different nuclear spin projections. The systems are coupled using a forbidden nuclear…

Strongly Correlated Electrons · Physics 2017-07-26 S. Bertaina , G. Yue , C-E Dutoit , I. Chiorescu

We introduce crystal polaritons, hybrid excitations formed when the collective excitations of a periodic quantum-emitter array strongly couple to the resonant Bloch modes of a metasurface. This realizes a cavity-QED platform in which…

Experiments based on cavity quantum electrodynamics (QED) are widely used to study the interaction of a light field with a discrete frequency spectrum and emitters. More recently, the field of waveguide QED has attracted interest due to the…

Rabi oscillations typify the inherent nonlinearity of optical excitations in quantum dots. Using an integral kernel formulation to solve the 3D Maxwell-Bloch equations in ensembles of up to $10^4$ quantum dots, we observe features in Rabi…

Atomic and Molecular Clusters · Physics 2017-09-13 Connor Glosser , B. Shanker , Carlo Piermarocchi

Circuit quantum electrodynamics (QED) studies the interaction of artificial atoms, open transmission lines and electromagnetic resonators fabricated from superconducting electronics. While the theory of an artificial atom coupled to one…