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The optical frequency comb has made a significant impact in precision spectroscopy and on our ability to probe atomic, molecular and, recently, nuclear transitions to further our understanding of their fundamental properties and how their…

Optics · Physics 2026-02-17 John J. McCauley , DylanP. Tooley , R. Jason Jones

A single photon prepared in a time-energy state described by a frequency comb combines the extreme precision of energy defined by a single tooth of the comb with a high sensitivity to small shifts in time defined by the narrowness of a…

Quantum Physics · Physics 2014-05-19 Changliang Ren , Holger F. Hofmann

Spectroscopy has attracted much attention in molecular detection, biomolecular identification, and chemical analysis for providing accurate measurement. However, it is almost unable to distinguish different sources with overlapped…

Instrumentation and Detectors · Physics 2020-05-12 Ting Qing , Shupeng Li , Yijie Fang , Xiaohu Tang , Lihan Wang , Meihui Cao , Xinyu Li , Shilong Pan

We demonstrated the observation of Rb two-photon absorption directly excided by an optical frequency comb at fiber communication bands. A chain of comb spectral control is elaborately implemented to increase the power of the second harmonic…

Optics · Physics 2015-06-16 Jiutao Wu , Dong Hou , Xiaoliang Dai , Zhengyu Qin , Zhigang Zhang , Jianye Zhao

Two-photon interference is a fundamental resource for quantum technologies and optical quantum computing, underpinning precision measurements, scalable entanglement distribution, and the operation of photonic circuits and quantum network…

It was recently demonstrated that broadband quantum cascade lasers can operate as frequency combs. As such, they operate under direct electrical pumping at both mid-infrared and THz frequencies, making them very attractive for dual-comb…

Adiabatic passage techniques allow the generation of single photons which are very long compared to the typical detector time resolution. Therefore the detection time of a photon can be measured within the duration of the single-photon…

Quantum Physics · Physics 2011-09-06 T. Legero , T. Wilk , A. Kuhn , G. Rempe

Two-photon interference is a fundamental quantum optics effect with numerous applications in quantum information science. Here, we study two-photon interference in multiple transverse-spatial modes along a single beam-path. Besides…

Quantum Physics · Physics 2021-03-31 Markus Hiekkamäki , Robert Fickler

Dual-comb spectroscopy utilizes two sets of comb lines with slightly different comb-tooth-spacings, and optical spectral information is acquired by measuring the radio-frequency beat notes between the sets of comb lines. It holds the…

Optics · Physics 2016-09-13 Xin Zhao , Guoqing Hu , Bofeng Zhao , Cui Li , Yingling Pan , Ya Liu , Takeshi Yasui , Zheng Zheng

Electro-optic frequency combs with tooth spacings as low as 100 Hz were employed to probe electromagnetically induced transparency (EIT) and hyperfine pumping in rubidium and potassium vapor cells. From the potassium EIT transition we were…

Atomic Physics · Physics 2018-12-27 David A. Long , Adam J. Fleisher , Joseph T. Hodges

Acquisition of laser frequency with high resolution under continuous and abrupt tuning conditions is important for sensing, spectroscopy and communications. Here, a single microresonator provides rapid and broad-band measurement of…

The detection of light of thermal origin is the principal means by which humanity has learned about our world and the cosmos. In optical astronomy, in particular, direct detection of thermal photons and the resolution of their spectra have…

We devise a new detection technique for mid-infrared multi-heterodyne spectroscopy. As an experimental implementation, mid-infrared light interrogates a gas sample in the 3-$\mu$m region of the fundamental CH, OH, NH stretch in molecules…

Optics · Physics 2020-03-17 Zaijun Chen , Theodor W. Hänsch , Nathalie Picqué

We demonstrate fast characterization (~1.4 microseconds) of both the dispersion and dispersion slope of long optical fiber links (~25 km) using dual quadrature spectral interferometry with an optical frequency comb. Compared to previous…

Infrared spectroscopy in the spectral fingerprint region from 6-12 um accesses the largest molecular absorption cross-sections, permitting sensitive, quantitative and species-specific measurements. Here, we show how dual-comb…

Optics · Physics 2023-06-26 O. Kara , L. Maidment , T. Gardiner , P. G. Schunemann , D. T. Reid

We report on the first demonstration of nonlinear dual-frequency-comb spectroscopy. In multi-heterodyne femtosecond Raman-induced Kerr-effect spectroscopy, the Raman gain resulting from the coherent excitation of molecular vibrations by a…

Dual-comb spectroscopy enables broadband analysis of key molecules with unparalleled frequency resolution and exceptional signal-to-noise ratios across various spectral regions. However, fully harnessing its potential for broadband…

We propose and characterize experimentally a new source of optical frequency combs for performing multi-heterodyne spectrometry. This comb modality is based on a frequency shifting loop seeded with a CW monochromatic laser. The comb lines…

Optics · Physics 2018-07-04 V. Duran , C. Schnebelin , H. Guillet De Chatellus

We report a two-photon interference experiment in which the detected photons have very different properties. The interference is observed even when no effort is made to mask the distinguishing features before the photons are detected. The…

Quantum Physics · Physics 2007-05-23 Yoon-Ho Kim , Warren P. Grice

The interference of non-classical states of light enables quantum-enhanced applications reaching from metrology to computation. Most commonly, the polarisation or spatial location of single photons are used as addressable degrees-of-freedom…

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