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Atomic vacancies have a strong impact in the mechanical, electronic and magnetic properties of graphene-like materials. By artificially generating isolated vacancies on a graphite surface and measuring their local density of states on the…

Mesoscale and Nanoscale Physics · Physics 2015-05-18 M. M. Ugeda , I. Brihuega , F. Guinea , J. M. Gomez-Rodriguez

Magneto-electric multiferroics exemplified by TbMnO3 possess both magnetic and ferroelectric long-range order. The magnetic order is mostly understood, whereas the nature of the ferroelectricity has remained more elusive. Competing models…

Strongly Correlated Electrons · Physics 2011-10-14 H. C. Walker , F. Fabrizi , L. Paolasini , F. de Bergevin , J. Herrero-Martin , A. T. Boothroyd , D. Prabhakaran , D. F. McMorrow

We study static vacancies in the collinear magnetic phase of a frustrated Heisenberg $J_1$-$J_2$ model. It is found that vacancies can rapidly suppress the collinear antiferromagnetic state (CAFM)and generate a new magnetic phase, an…

Strongly Correlated Electrons · Physics 2015-03-19 Bao Xu , Chen Fang , W. M. Liu , Jiangping Hu

Our first-principles results show that geometric frustration can be induced in thin films of multiferroic BiFeO3. We find that competing magnetic interactions occur in the so-called super-tetragonal phase of this material, which can be…

Materials Science · Physics 2015-06-05 Carlos Escorihuela-Sayalero , Oswaldo Diéguez , Jorge Íñiguez

The zero-temperature limit of a continuous phase transition is marked by a quantum critical point, which can generate exotic physics that extends to elevated temperatures. Magnetic quantum criticality is now well known, and has been…

Materials Science · Physics 2019-02-21 Awadhesh Narayan , Andres Cano , Alexander V. Balatsky , Nicola A. Spaldin

With a combined ab initio density functional and model Hamiltonian approach we establish that in the recently discovered multiferroic phase of the manganite Sr$_{1/2}$Ba$_{1/2}$MnO$_{3}$ the polar distortion of Mn and O ions is stabilized…

Materials Science · Physics 2015-03-09 Gianluca Giovannetti , Sanjeev Kumar , Carmine Ortix , Massimo Capone , Jeroen van den Brink

The coupling between structural, electronic and magnetic degrees of freedom across the metal-insulator transition in V2O3 makes it hard to determine the main driving mechanism behind the transition. Specifically, the role of magnetism has…

Correlated band theory is employed to investigate the magnetic and electronic properties of different arrangements of oxygen di- and tri-vacancy clusters in SrTiO$_3$. Hole and electron doping of oxygen deficient SrTiO$_3$ yields various…

Materials Science · Physics 2016-03-30 Alejandro Lopez-Bezanilla , P. Ganesh , Peter B. Littlewood

The influence of surface oxygen vacancies on the oxygen evolution reaction on bismuth vanadate is studied using hybrid density functional theory. Our findings reveal the thermodynamic instability of the neutral unionized defect (${\rm…

Materials Science · Physics 2023-06-19 Nicklas Österbacka , Hassan Ouhbi , Francesco Ambrosio , Julia Wiktor

While the recent establishment of the role of thermophoresis/diffusion-driven oxygen migration during resistance switching in metal oxide memristors provided critical insights required for memristor modeling, extended investigations of the…

Understanding the diffusion of oxygen vacancies in oxides under different external stimuli is crucial for the design of ion-based electronic devices, improve catalytic performance, etc. In this manuscript, using an external electric field…

Materials Science · Physics 2018-07-04 Lucía Iglesias , Andrés Gómez , Martí Gich , Francisco Rivadulla

Heterostructures from complex oxides allow one to combine various electronic and magnetic orders as to induce new quantum states. A prominent example is the coupling between superconducting and magnetic orders in multilayers from high-Tc…

We show that misfit strain originated from the film-substrate lattice mismatch strongly increases the value of the quadratic magnetoelectric coupling. The giant magnetoelectric coupling, size effects and misfit strain cause strong changes…

Materials Science · Physics 2008-08-02 A. N. Morozovska , M. D. Glinchuk , E. A. Eliseev , R. Blinc

Time-dependent rotational electric polarizations have been proposed to generate temporally varying magnetic moments, for example, through a combination of ferroelectric polarization and optical phonons. This phenomenon has been called…

Multiferroic TbMnO3 is investigated using x-ray diffraction in high magnetic fields. Measurements on first and second harmonic structural reflections due to modulations induced by the Mn and Tb magnetic order are presented as function of…

Strongly Correlated Electrons · Physics 2008-07-29 J. Strempfer , B. Bohnenbuck , I. Zegkinoglou , N. Aliouane , S. Landsgesell , M. v. Zimmermann , D. N. Argyriou

Contrary to traditional approaches, high entropy oxides (HEOs) strategically employ cationic disorder to engineer tunable functionalities. This disorder, stemming from multiple elements at the same crystallographic site, disrupts local…

It is shown that magnetic states and field-driven reorientation transitions in synthetic antiferromagnets crucially depend on contributions of higher-order anisotropies. A phenomenological macrospin model is derived to describe the magnetic…

Materials Science · Physics 2009-11-11 A. N. Bogdanov , U. K. Roessler

In this paper we study, both with theoretical and experimental approach, the effect of iron doping in zirconia. Combining density functional theory (DFT) simulations with the experimental characterization of thin films, we show that iron is…

The superconducting properties of high-\tc\ materials are functions of carriers concentration, which is controlled by the concentration of defects including heterovalent cations, interstitial oxygen ions, and oxygen vacancies. Here we…

Catalysis is indispensable to chemical processes and relevant to many aspects of modern life. Owing to the intriguing electronic structures and good ionic properties, multivalent transition metal oxides have attracted attention as key…