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Protein fibril accumulation at interfaces is an important step in many physiological processes and neurodegenerative diseases as well as in designing materials. Here we show, using $\beta$-lactoglobulin fibrils as a model, that semiflexible…

Biomolecules · Quantitative Biology 2015-05-20 Sophia Jordens , Emily E. Riley , Ivan Usov , Lucio Isa , Peter D. Olmsted , Raffaele Mezzenga

In this work, we investigate crystallization from droplets formed on micro-patterned surfaces. By solvent exchange in a micro-chamber, a ternary solution consisting of a model compound beta-alanine, water, and isopropanol, was displaced by…

Soft Condensed Matter · Physics 2021-04-16 Howon Choi , Zixiang Wei , Jae Bem You , Huaiyu Yang , Xuehua Zhang

Freezing in the vicinity of water-vapor interfaces is of considerable interest to a wide range of disciplines, most notably the atmospheric sciences. In this work, we use molecular dynamics and two advanced sampling techniques, forward flux…

Statistical Mechanics · Physics 2014-11-04 Amir Haji-Akbari , Ryan S. DeFever , Sapna Sarupria , Pablo G. Debenedetti

Surfaces of surfactant-templated polyacrylamide hydrogels were imaged by atomic force microscopy (AFM), and the surface morphology was studied by numerical scaling analysis. The templated gels were formed by polymerizing acrylamide plus a…

Soft Condensed Matter · Physics 2007-05-23 Mukundan Chakrapani , S. J. Mitchell , D. H. Van Winkle , P. A. Rikvold

A glass surface may still flow below the bulk glass transition temperature, where the underlying bulk is frozen. Assuming the existence at T=T* of a bulk thermodynamical glass transition, we show that the glass-vapor interface is generally…

Materials Science · Physics 2009-10-31 E. A. Jagla , E. Tosatti

Samples of $\alpha$-SiC have been sintered with liquid phase (LPS) to 1950 $^\circ$C, in atmosphere of argon and processing times between 1 and 7 hours. Using scanning electron microscopy (SEM) the microstructure of the samples has been…

The formation of periodic wrinkles in soft layered materials due to mechanical instabilities is prevalent in nature and has been proposed for use in multiple applications. However, such phenomena have been explored predominantly in…

We present a computational study of the void-induced microstructure in amorphous silicon ($\it a$-Si) by generating ultra-large models of $\it a$-Si with a void-volume fraction of 0.3$\%$, as observed in small-angle x-ray scattering (SAXS)…

Disordered Systems and Neural Networks · Physics 2019-10-02 Durga Paudel , Raymond Atta-Fynn , David A. Drabold , Parthapratim Biswas

The ability to synthesize and control two-dimensional (2D) crystals creates numerous opportunities for studying emergent states of matter and their novel functionalities. Freestanding films provide a particularly versatile platform for…

Materials Science · Physics 2024-02-13 Yifan Su , Alfred Zong , Anshul Kogar , Di Lu , Seung Sae Hong , Byron Freelon , Timm Rohwer , Harold Y. Hwang , Nuh Gedik

The plastic deformation mechanisms of tungsten carbide at room and elevated temperatures influence the wear and fracture properties of WC-Co hardmetal composite materials. The relationship between residual defect structures, including…

Materials Science · Physics 2021-11-05 Vivian Tong , Helen Jones , Ken Mingard

Controlled crystallization, melting and vitrification are important fundamental processes in nature and technology. However, the microscopic details of these fundamental phenomena still lack understanding, in particular how the cooling rate…

Soft Condensed Matter · Physics 2024-07-08 M. P. M. Schelling , T. W. J. Verouden , T. C. M. Stevens , J. -M. Meijer

Wrinkling is commonly observed as mechanical instability when a stiff thin film bound on a compliant thick substrate undergoes in-plane compression exceeding a threshold. Despite significant efforts to create a broad range of surface…

Soft Condensed Matter · Physics 2025-03-11 Yuchong Gao , Yinding Chi , Mohit Patel , Lishuai Jin , Jiaqi Liu , Pierre-Thomas Brun , Shu Yang

The effect of increasing temperature on the structural stability and interactions of two kinds of Al/Zr (Al(1%wtSi)/Zr and Al(Pure)/Zr) multilayer mirrors are investigated. All Al/Zr multilayers annealed from 200^{\circ}C to 500^{\circ}C,…

Materials Science · Physics 2015-06-11 Qi Zhong , Shuang Ma , Zhong Zhang , Runze Qi , Jia Li , Zhanshan Wang , Philippe Jonnard

The influence of the external pressure and surface energy on the wetting transition at nanotextured interfaces is studied using molecular dynamics and continuum simulations. The surface roughness of the composite interface is introduced via…

Soft Condensed Matter · Physics 2018-07-12 Bishal Bhattarai , Nikolai V. Priezjev

We have performed molecular dynamics simulations of solid-solid contacts lubricated by a model fluid displaying many of the properties of water, particularly its expansive freezing. Near the region where expansive freezing occurs, the…

Condensed Matter · Physics 2009-11-07 E. A. Jagla

The structure of polymers at solid interfaces evolves over time, but the corresponding changes in their rheological properties remain poorly understood. Here, using a home-built quartz tuning fork atomic force microscope-based…

Fluid Dynamics · Physics 2025-08-22 Jaewon Shim , Manhee Lee , Wonho Jhe

The deformation kinetics for glassy solid helium confined in microscopic domain at very low temperature regime was investigated using a transition-rate model considering the shear thinning behavior which means, once material being subjected…

General Physics · Physics 2009-04-09 Zotin K. -H. Chu

A study of wetting was carried out on porous silicon films with pore diameters spanning three orders of magnitude. Water contact angle measurements on adjoining porous and nonporous regions yielded Wenzel roughness ratios that were either…

Materials Science · Physics 2022-11-15 S. J. Spencer , C. G. Deacon , G. T. Andrews

The structures of the liquid surface and the liquid-solid interface of sodium have been characterized with extensive first-principles molecular dynamics simulations. Friedel oscillations in the electronic charge density at the free surface…

Materials Science · Physics 2007-05-23 Brent G. Walker , Nicola Marzari , Carla Molteni

Temperature-responsive properties of surface-attached poly(N-isopropylacrylamide) (PNIPAM) network films with well-controlled chemistry are investigated. The synthesis consists of cross-linking and grafting preformed ene-reactive polymer…

Materials Science · Physics 2016-04-13 Mengxing Li , Bruno Bresson , F Cousin , Christian Fretigny , Yvette Tran