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In recent years, sliding ferroelectricity has emerged as a topic of significant interest due to its possible application in non-volatile, reconfigurable storage devices. This phenomenon is unique to two-dimensional van der Waals materials,…

Two-dimensional (2D) ferromagnets with high Curie temperature have long been the pursuit for electronic and spintronic applications. CrI3 is a rising star of intrinsic 2D ferromagnets, however, it suffers from weak exchange coupling. Here…

Materials Science · Physics 2020-09-22 Yu Guo , Nanshu Liu , Yanyan Zhao , Xue Jiang , Si Zhou , Jijun Zhao

Intercalation reactions modify the charge density in van der Waals (vdW) materials through coupled electronic-ionic charge accumulation, and are susceptible to modulation by interlayer hybridization in vdW heterostructures. Here, we…

Van der Waals monolayers featuring magnetic states provide a fundamental building block for artificial quantum matter. Here, we establish the emergence of a multicomponent ground state featuring magneto-orbital excitations of the…

Strongly Correlated Electrons · Physics 2025-03-13 Luigi Camerano , Adolfo O. Fumega , Gianni Profeta , Jose L. Lado

The ability to control magnetic properties of materials is crucial for fundamental research and underpins many information technologies. In this context, two-dimensional materials are a particularly exciting platform due to their high…

Moir\'e superlattices in van der Waals structures can be used to control the electronic properties of the material and lead to emergent correlated and topological phenomena. Its first demonstration in van der Waals magnets exhibited…

Controlling magnetic order via external fields or heterostructures enables precise manipulation and tracking of spin and exciton information, facilitating the development of high-performance optical spin valves. However, the weak…

Materials Science · Physics 2024-09-30 Jia Shi , Dan Wang , Nai Jiang , Ziqian Xin , Houzhi Zheng , Chao Shen , Xinping Zhang , Xinfeng Liu

Recent development in two-dimensional (2D) magnetic materials have motivated the search for new van der Waals magnetic materials, especially Ising-type magnets with strong magnetic anisotropy. Fe-based MPX3 (M = transition metal, X =…

Two-dimensional (2D) magnetic material CrI3 has aroused extensive attention, because it could provide a new platform for investigating the relations between crystal structures and electronic and magnetic properties. Here, we study crystal…

Materials Science · Physics 2025-06-23 Suqi Liu , Feng Sun , Aijun Hong

Layered ferromagnets with high coercivity have special applications in nanoscale memory elements in electronic circuits, such as data storage. Therefore, searching for new hard ferromagnets and effectively tuning or enhancing the coercivity…

Materials Science · Physics 2023-01-11 Xi Zhang , Le Wang , Huimin Su , Xiuquan Xia , Cai Liu , Junhao Lin , Mingyuan Huang , Yingchun Cheng , Jia-Wei Mei , Jun-Feng Dai

Strategies such as chemical substitution, strain engineering and van der Waals stacking offer powerful means to control magnetism in 2D materials, enabling the emergence of novel quantum phenomena. Here, we investigate the magnetic…

Materials Science · Physics 2024-12-30 Alberto M. Ruiz , José J. Baldoví

The electronic and magnetic structure of CrPS$_{4}$, a 2D magnetic semiconductor is examined by employing the SCAN meta-GGA density functional. We find the resulting magnetic moment and band gap are in excellent agreement with experiment.…

Strongly Correlated Electrons · Physics 2024-01-12 A. R. Alcantara , C. Lane , J. T. Haraldsen , R . M. Tutchton

Activating metamagnetic transitions between ordered states in van der Waals magnets and devices bring great opportunities in spintronics. We show that external pressure, which enhances the interlayer hopping without introducing chemical…

Strongly Correlated Electrons · Physics 2022-07-25 Tiema Qian , Eve Emmanouilidou , Chaowei Hu , Jazmine C. Green , Igor I. Mazin , Ni Ni

Single crystalline samples of the van der Waals antiferromagnet CrPS4 were studied by measurements of specific heat and comprehensive anisotropic temperature- and magnetic field-dependent magnetization. In addition, measurements of the heat…

Materials Science · Physics 2021-06-09 Sergey L. Bud'ko , Elena Gati , Tyler J. Slade , Paul C. Canfield

Recent observation of intrinsic ferromagnetism in two-dimensional (2D) CrI$_3$ is associated with the large magnetic anisotropy due to strong spin-orbit coupling (SOC) of I. Magnetic anisotropy energy (MAE) defines the stability of…

Mesoscale and Nanoscale Physics · Physics 2018-10-10 Lucas Webster , Jia-An Yan

Integrating monolayers derived from 2D van der Waals (vdW) magnetic materials into next-generation technological applications remains a significant challenge due to their structural and magnetic instability issues. Template-assisted…

Materials Science · Physics 2025-10-08 Ihsan Caha , Aqrab ul Ahmad , Francis Leonard Deepak

To magnetize surfaces of topological insulators without damaging their topological feature is a crucial step for the realization of the quantum anomalous Hall effect (QAHE), and still remains as a challenging task. Through density…

Mesoscale and Nanoscale Physics · Physics 2019-06-04 Yusheng Hou , Ruqian Wu

Motivated by the potential of atomically-thin magnets towards tunable high-frequency magnonics, we detail the spin-wave dispersion of bilayer CrI$_3$. We demonstrate that the magnonic behavior of the bilayer strongly depends on its stacking…

Materials Science · Physics 2023-03-01 M. Soenen , C. Bacaksiz , R. M. Menezes , M. V. Milosevic

Quantum states of matter combining non-trivial topology and magnetism attract a lot of attention nowadays; the special focus is on magnetic topological insulators (MTIs) featuring quantum anomalous Hall and axion insulator phases.…

Fe$_{3-x}$GeTe$_2$ is a layered van der Waals magnetic material with a relatively high ordering temperature and large anisotropy. While most studies have concluded the interlayer ordering to be ferromagnetic, there have also been reports of…