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Related papers: Photoionization of Molecular Endohedrals

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We show that the combination of two achiral components - atomic or molecular target plus a circularly polarized photon - can yield chirally structured photoelectron angular distributions. For photoionization of CO, the angular distribution…

Angular distribution of photoelectrons released by the ionization of randomly-oriented molecules with two laser fields of carrier frequencies $\omega$ and $2\omega$, which are linearly polarized in two mutually-orthogonal directions, is…

Quantum Physics · Physics 2019-06-11 Philipp V. Demekhin

We studied the hydrogen atom as a system of two quantum particles in different confinement conditions; a spherical-impenetrable-wall cavity and a fullerene molecule cage. The motion is referred to the center of spherical cavities, and the…

Atomic and Molecular Clusters · Physics 2016-12-21 Juan M. Randazzo , Carlos A. Rios

We calculate the photoionization with excitation-to photoionization ratios for atomic helium and heliumlike ions at intermediate values of the photon energies. The final state interactions between the electrons are included in the lowest…

Quantum Physics · Physics 2009-11-13 E. G. Drukarev , E. Z. Liverts , M. Ya. Amusia , R. Krivec , V. B. Mandelzweig

The photoionization of the CO molecule from the C$-1s$ orbital does not obey the Franck-Condon approximation, as a consequence of the nuclear recoil that accompanies the direct emission and intra-molecular scattering of the photoelectron.…

Atomic Physics · Physics 2021-11-24 Bejan Ghomashi , Nicolas Douguet , Luca Argenti

Strong-field photoelectron momentum imaging of the prototypical biomolecule indole was disentangled in a combined experimental and computational approach. Experimentally, strong control over the molecules enabled the acquisition of…

Atomic Physics · Physics 2021-02-03 Joss Wiese , Jolijn Onvlee , Sebastian Trippel , Jochen Küpper

We present a theoretical method for calculating multiphoton ionization amplitudes and cross sections of few-electron atoms. The present approach is based on an extraction of partial wave amplitudes from a scattering wave function, which is…

Atomic Physics · Physics 2021-04-21 Andrej Mihelic , Martin Horvat

We report detailed results on ionization in metallic quantum--dot (QD) nanorings described by the extended Hubbard model at half filling obtained by exact numerical diagonalization. In spite of very strong electron correlations, the…

Strongly Correlated Electrons · Physics 2009-06-09 Ioan Baldea , Lorenz S. Cederbaum , Jochen Schirmer

Experimental results on partial photo-ionisation cross sections of helium are analysed in the light of recent advances in the semiclassical theory of two-electron atoms. Byun et al (arXiv:physics/0701086) predict that the total…

Atomic Physics · Physics 2009-11-13 Gregor Tanner , Nark Nyul Choi , Min-Ho Lee , Achim Czasch , Reinhard Doerner

The two-photon decay in hydrogen-like ions is investigated within the framework of second order perturbation theory and Dirac's relativistic equation. Special attention is paid to the angular correlation of the emitted photons as well as to…

Atomic Physics · Physics 2014-10-23 P. Amaro , F. Fratini , S. Fritzsche , P. Indelicato , J. P. Santos , A. Surzhykov

The angle-resolved inner-shell photoionization of R-trifluoromethyloxirane, C3H3F3O, is studied experimentally and theoretically. Thereby, we investigate the photoelectron circular dichroism (PECD) for nearly-symmetric O 1s and F 1s…

Photodetachment of the outer-most electrons in few- and many-electron atomic systems is studied in the non-relativistic dipole approximation. Such a photodetachment is analyzed for the neutral atoms and positively charged atomic ions. We…

Atomic Physics · Physics 2021-11-04 Alexei M. Frolov

In this study, we have investigated the photoionization cross section of an on-center hydrogenic impurity in a multi-layered spherical quantum dot. The electronic energy levels and their wave functions have been determined fully numerically…

Mesoscale and Nanoscale Physics · Physics 2013-05-07 Mehmet Sahin , Firdes Tek , Ahmet Erdinç

We provide the initial insight into the angle-differential photodetachment spectra of fullerene anions beyond the dipole approximation by utilizing a broadly used modelling of C$_{n}$. In the model, the C$_{n}$ cage is approximated by a…

Atomic Physics · Physics 2018-10-02 V K Dolmatov , A Edwards , C G Lane

It is demonstrated by the example of the Xe atom stuffed inside the C60 fullerene, that the so-called confinement resonances in 4d subshell strongly affect the photoionization cross-section of outer 5p and subvalent 5s electrons near 4d…

Atomic Physics · Physics 2015-06-03 M. Ya. Amusia , L. V. Chernysheva

We present a combined theoretical and experimental work investigating the angle-resolved phases of the photoionization process driven by a two-color field consisting of an attosecond pulse train and an infrared pulse in an ensemble of…

Photoelectron spectroscopy is a powerful method that provides insight into the quantum mechanical properties of a wide range of systems. The ionized electron wavefunction carries information on the structure of the bound orbital, the ionic…

Present photoionization experiments cannot measure molecular frame photoelectron angular distributions (MFPAD) from the outermost valence electrons of molecules. We show that details of the MFPAD can be retrieved with high-order harmonics…

Atomic Physics · Physics 2009-05-24 Anh-Thu Le , R. R. Lucchese , M. T. Lee , C. D. Lin

We develop an approximate model for the process of direct (nonsequential) two-photon double ionization of atoms. Employing the model, we calculate (generalized) total cross sections as well as energy-resolved differential cross sections of…

Quantum Physics · Physics 2016-08-17 Morten Førre , Sølve Selstø , Raymond Nepstad

We describe a numerical method that simulates the interaction of the helium atom with sequences of femtosecond and attosecond light pulses. The method, which is based on the close-coupling expansion of the electronic configuration space in…

Atomic Physics · Physics 2021-05-25 Luca Argenti , Eva Lindroth