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We study dipole interseries transitions between the yellow and green exciton series in cuprous oxide including the complex valence band structure. To this end, we extend previous studies of the spectrum of complex green exciton resonances…

Mesoscale and Nanoscale Physics · Physics 2021-08-25 Patric Rommel , Jörg Main , Sjard Ole Krüger , Stefan Scheel

We report on the observation of the yellow exciton Lyman series up to the fourth term in Cu2O by time-resolved mid-infrared spectroscopy. The dependence of the oscillator strength on the principal quantum number n can be well reproduced…

Materials Science · Physics 2009-11-11 Takeshi Tayagaki , Andre Mysyrowicz , Makoto Kuwata-Gonokami

Rydberg excitons in Cu2O can be an emergent platform for solid-state quantum information processing by utilizing the exaggerated properties of high-lying excited states within the material. To develop practical quantum systems,…

Mesoscale and Nanoscale Physics · Physics 2021-05-19 Dungeon Daniel Kang , Aaron Gross , HeeBong Yang , Yusuke Morita , Kyung Soo Choi , Kosuke Yoshioka , Na Young Kim

We have used high resolution transmission spectroscopy to study the exciton level spectrum in Cu$_2$O subject to a longitudinal external electric field, i.e., in the geometry where the transmitted light is propagating along the field…

Materials Science · Physics 2017-02-01 J. Heckötter , M. Freitag , D. Fröhlich , M. Aßmann , M. Bayer , M. A. Semina , M. M. Glazov

We experimentally and numerically investigate the exchange interaction of the yellow excitons in cuprous oxide. By varying the material parameters in the numerical calculations, we can interpret experimental findings and understand their…

Materials Science · Physics 2021-02-19 Patric Rommel , Jörg Main , Andreas Farenbruch , Dmitri R. Yakovlev , Manfred Bayer

We report experimental and theoretical investigations of interacting excitons of the yellow series in cuprous oxide (Cu$_2$O) with principal quantum numbers up to $n=7$ by means of second harmonic generation (SHG). Using picosecond pulsed…

We study the absorption spectra of the yellow excitons in Cu$_2$O in high magnetic fields using polarization-resolved optical absorption measurements with a high frequency resolution. We show that the symmetry of the yellow exciton results…

Cuprous oxide (Cu${}_2$O) has recently been proposed as a promising solid-state host for excitonic Rydberg states with large principal quantum numbers ($n$), whose exaggerated wavefunction sizes ($\propto n^2)$ facilitate gigantic…

Quantum Physics · Physics 2022-11-01 Jacob DeLange , Kinjol Barua , Val Zwiller , Stephan Steinhauer , Hadiseh Alaeian

In this study we analyze the transmission spectrum of a thin plate of Cuprous Oxide in the range of the absorption of the yellow exciton states with the coherent transfer matrix method. We demonstrate that, in contrast to the usual analysis…

Mesoscale and Nanoscale Physics · Physics 2021-07-28 Heinrich Stolz , Rico Schwartz , Julian Heckötter , Marc Aßmann , Dirk Semkat , Sjard O. Krüger , Manfred Bayer

When an electron in a semiconductor gets excited to the conduction band the missing electron can be viewed as a positively charged particle, the hole. Due to the Coulomb interaction electrons and holes can form a hydrogen-like bound state…

Mesoscale and Nanoscale Physics · Physics 2024-10-03 Jan Ertl , Sebastian Rentschler , Jörg Main

Rydberg excitons are, with their ultrastrong mutual interactions, giant optical nonlinearities, and very high sensitivity to external fields, promising for applications in quantum sensing and nonlinear optics at the single-photon level. To…

We investigate the nonlinear refraction induced by Rydberg excitons in $\mathrm{Cu_2O}$. Using a high-precision interferometry imaging technique that spatially resolves the nonlinear phase shift, we observe significant shifts at extremely…

Rydberg excitons in the semiconductor Cu$_2$O have been observed in absorption experiments up to a principal quantum number of n = 28 at millikelvin temperatures [1]. Here, we extend the experimental parameter space by variing both…

Mesoscale and Nanoscale Physics · Physics 2025-11-03 Julian Heckötter , David Janas , Marc Aßmann , Manfred Bayer

A mechanism for amplification of weak quadrupole transitions of Rydberg excitons in Cu$_2$O by a plasmonic nanostructure is investigated. The theoretical description of exciton-plasmon interaction is presented and a field averaging…

Optics · Physics 2025-07-17 David Ziemkiewicz , Sylwia Zielińska-Raczyńska

We report exciton-mediated coupling between microwave and optical fields in cuprous oxide (Cu$_2$O) at low temperatures. Rydberg excitonic states with principal quantum number up to $n=12$ were observed at 4~K using both one-photon…

A resonant inelastic x-ray scattering study of the electronic structure of the semiconductor cuprous oxide, $\rm Cu_2O$, is reported. When the incident x-ray energy is tuned to the Cu K-absorption edge, large enhancements of the spectral…

Materials Science · Physics 2012-06-18 Young-June Kim , J. P. Hill , H. Yamaguchi , T. Gog , D. Casa

The observation of giant Rydberg excitons in cuprous oxide $\left(\mathrm{Cu_{2}O}\right)$ up to a principal quantum number of $n=25$ by T.~Kazimierczuk \emph{et al.} [Nature \textbf{514}, 343, (2014)] inevitably raises the question whether…

Materials Science · Physics 2017-12-07 Frank Schweiner , Jan Ertl , Jörg Main , Günter Wunner , Christoph Uihlein

We numerically investigate the odd parity states of the green exciton series in cuprous oxide. Taking into account the coupling to the yellow series and especially to the yellow continuum, the green excitons are quasi-bound resonances with…

Materials Science · Physics 2020-03-02 Patric Rommel , Patrik Zielinski , Jörg Main

We theoretically investigate the nonlinear optical transmission through a cuprous oxide crystal for wavelengths that cover the series of highly excited excitons, observed in recent experiments. Since such Rydberg excitons have strong van…

Mesoscale and Nanoscale Physics · Physics 2020-09-02 Valentin Walther , Thomas Pohl

Highly excited atoms with an electron moved into a level with large principal quantum number are fascinating hydrogen-like objects. The giant extension of these Rydberg atoms leads to huge interaction effects. Monitoring these interactions…

Mesoscale and Nanoscale Physics · Physics 2014-11-13 Tomasz Kazimierczuk , Dietmar Fröhlich , Stefan Scheel , Heinrich Stolz , Manfred Bayer
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