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We report strong third-harmonic generation (THG) in monolayer graphene grown by chemical vapor deposition (CVD) and transferred to an amorphous silica (glass) substrate; the photon energy is in three-photon resonance with the…

Mesoscale and Nanoscale Physics · Physics 2013-06-12 Sung-Young Hong , Jerry I. Dadap , Nicholas Petrone , Po-Chun Yeh , James Hone , Richard M. Osgood

The microscopic quantum theory of nonlinear stimulated scattering of chiral particles in doped $AB$ stacked bilayer graphene on Coulomb field of charged impurities in the presence of strong coherent electromagnetic radiation is presented.…

Mesoscale and Nanoscale Physics · Physics 2019-07-26 A. G. Ghazaryan , Kh. V. Sedrakian

We use an exact solution of the relaxation-time Boltzmann equation in a uniform AC electric field to describe the nonlinear optical response of graphene in the terahertz (THz). The cases of monolayer, bilayer and ABA-stacked trilayer…

Mesoscale and Nanoscale Physics · Physics 2014-09-23 N. M. R. Peres , Yu. V. Bludov , Jaime E. Santos , Antti-Pekka Jauho , M. I. Vasilevskiy

We report on theoretical study of second harmonic generation in graphene. Phenomenological analysis based on symmetry arguments is carried out. It is demontrated, that in ideal graphene samples second harmonic generation is possible only if…

Mesoscale and Nanoscale Physics · Physics 2015-03-17 M. M. Glazov

Graphene is a unique platform for tunable opto-electronic applications thanks to its linear band dispersion, which allows electrical control of resonant light-matter interactions. Tuning the nonlinear optical response of graphene is…

The low-energy (intraband) range of the third harmonic generation of graphene in the terahertz regime is governed by the damping terms induced by the interactions. A controlled many-body description of the scattering processes is thus a…

Mesoscale and Nanoscale Physics · Physics 2021-03-24 Habib Rostami , Emmanuele Cappelluti

We present a formulation for the nonlinear optical response in gapped graphene, where the low-energy single-particle spectrum is modeled by massive Dirac theory. As a representative example of the formulation presented here, we obtain…

Strongly Correlated Electrons · Physics 2012-05-30 S. A. Jafari

Due to its linear dispersion, monolayer graphene is expected to generate a third harmonic response at terahertz frequencies. There have been a variety of different models of this effect and recently it has been experimentally observed.…

Mesoscale and Nanoscale Physics · Physics 2022-04-06 Parvin Navaeipour , Marc M. Dignam

We observe enhanced second-harmonic generation in monolayer graphene in the presence of an ultra-strong terahertz field pulse with a peak amplitude of 250 kV/cm. This is a strongly nonperturbative regime of light-matter interaction in which…

We investigate high-order harmonic generation (HHG) in graphene with a quantum master equation approach. The simulations reproduce the observed enhancement in HHG in graphene under elliptically polarized light [N. Yoshikawa et al, Science…

Materials Science · Physics 2021-02-03 Shunsuke A. Sato , Hideki Hirori , Yasuyuki Sanari , Yoshihiko Kanemitsu , Angel Rubio

We theoretically study the THz-induced high-order harmonic generation (HHG) and nonlinear electric transport in graphene based on the quantum master equation with the relaxation time approximation. To obtain microscopic insight into the…

Mesoscale and Nanoscale Physics · Physics 2022-08-02 Wenwen Mao , Angel Rubio , Shunsuke A. Sato

We consider the interaction of gapped graphene in the two-band approximation using an explicit time-dependent approach. In addition to the full high-order harmonic generation (HHG) spectrum, we also obtain the perturbative harmonic response…

Materials Science · Physics 2017-02-01 Darko Dimitrovski , Lars Bojer Madsen , Thomas Garm Pedersen

High-order frequency mixing in graphene using a two-color radiation field consisting of the fundamental and the second harmonic fields of an ultrashort linearly polarized laser pulse is studied. It is shown that the harmonics originated…

Mesoscale and Nanoscale Physics · Physics 2022-05-25 Hamlet K. Avetissian , Garnik F. Mkrtchian , Andreas Knorr

If we stack up two layers of graphene while changing their respective orientation by some twisting angle, we end up with a system that has striking differences when compared to single-layer graphene. For a very specific value of this twist…

Mesoscale and Nanoscale Physics · Physics 2024-09-18 Eduardo B. Molinero , Anushree Datta , María J. Calderón , Elena Bascones , Rui E. F. Silva

Graphene has unique properties paving the way for groundbreaking future applications. Its large optical nonlinearity and ease of integration in devices notably makes it an ideal candidate to become a key component for all-optical switching…

We study cascaded harmonic generation of hybrid surface plasmons in integrated planar waveguides composed of a graphene layer and a doped-semiconductor slab. We derive a comprehensive model of cascaded third harmonic generation through…

Optics · Physics 2015-10-14 Daria A. Smirnova , Alexander S. Solntsev

We report on time-resolved ultrafast terahertz third-harmonic generation spectroscopy of nonequilibrium dynamics of Weyl fermions in a nanometer thin film of the Weyl semimetal TaP. Terahertz third-harmonic generation is observed at room…

Strongly Correlated Electrons · Physics 2025-11-26 Patrick Pilch , Changqing Zhu , Sergey Kovalev , Renato M. A. Dantas , Amilcar Bedoya-Pinto , Stuart S. P. Parkin , Zhe Wang

Nonlinear optics is an increasingly important field for scientific and technological applications, owing to its relevance and potential for optical and optoelectronic technologies. Currently, there is an active search for suitable nonlinear…

Triple point fermions are elusive electronic excitations that generalize Dirac and Weyl modes beyond the conventional high energy paradigm. Yet, finding real materials naturally hosting these excitations at the Fermi energy has remained…

Mesoscale and Nanoscale Physics · Physics 2019-06-18 Aline Ramires , J. L. Lado

We develop a theory for quantum phases and quantum multicriticality in bilayer graphene in the presence of an explicit energy gap in the non-interacting spectrum by extending previous renormalization group (RG) analyses of electron-electron…

Strongly Correlated Electrons · Physics 2014-11-18 Robert E. Throckmorton , S. Das Sarma