Related papers: Orbital-angular-momentum-resolved electron magneti…
Inversion-symmetric crystals are optically isotropic and thus naively not expected to show dichroism effects in optical absorption and photoemission processes. Here, we find a strong linear dichroism effect (up to 42.4%) in the conduction…
Orbital angular momentum (OAM) of light is an attractive degree of freedom for funda- mentals studies in quantum mechanics. In addition, the discrete unbounded state-space of OAM has been used to enhance classical and quantum…
For a twisted (vortex) Dirac particle in nonuniform electric and magnetic fields, the relativistic Foldy-Wouthuysen Hamiltonian is derived including high order terms describing new effects. The result obtained shows for the first time that…
When aiming for atomic resolution electron magnetic circular dichroism (EMCD) in STEM mode, the high convergence angle of the electron probe can lead to unforeseen artefacts and strong reductions of the signal to noise ratio (SNR) in the…
Recently developed circularly polarized X-ray light sources can probe ultrafast chiral electronic and nuclear dynamics through spatially localized resonant core transitions. We present simulations of time-resolved circular dichroism (TRCD)…
Using the fully-relativistic screened Korringa-Kohn-Rostoker method I study the orbital magnetism in the half-metallic Heusler alloys. Orbital moments are almost completely quenched and they are negligible with respect to the spin moments.…
Rashba-split surface band is characterized by a one-to-one correspondence between the electron's momentum k and its spin orientation. Here we show that a similar correspondence between momentum and orbital angular momentum (OAM) must exist…
The Fraunhofer diffraction of quantum particles from materials with sharp electron-density edges or symmetric bond structures is ubiquitous. In contrast, diffraction from atoms with characteristic asymptotically-diffused electron…
We suggest that in an anisotropic crystal there should be a new mechanism of dichroism related to a scissors mode, a kind of excitation observed in several other many-body systems. Such an effect should be found in crystals, amorphous…
Optically active achiral metasurfaces offer a promising way to detect chiral molecules based on chiroptic methods. The combination of plasmonic enhanced circular dichroism and reversible optical activity would boost the sensitivity and…
Structured x-rays carrying an orbital angular momentum break spatial inversion symmetry and have been proposed as a means to probe chirality. We theoretically investigate twisted non-resonant x-ray diffraction from chiral molecules and…
We propose an innovative monolithic interferometer to distinguish the topological charge of radiation carrying orbital angular momentum. Remarkably, our method requires to access only a small portion of the entire wavefront. The proposed…
We report the development of an instrument combining an ultrafast, high-repetition-rate, polarization-tunable monochromatic extreme ultraviolet (XUV, 21.6 eV) beamline and a next-generation momentum microscope endstation. This setup enables…
Orbital angular momentum (OAM) carried by helical light beams is an unbounded degree of freedom of photons that offers a promising playground in modern photonics. So far, integrated sources of coherent light carrying OAM are based on…
We demonstrate the polarization of electron orbital angular momentum (OAM) in neutral atoms by integrating the Zeeman effect with attosecond transient absorption spectroscopy (ATAS). Using density matrix simulations, we show that in a…
We show that a nonchiral atom can act as an antenna to induce a photoelectron circular dichroism in a nearby chiral molecule in a three-step process: The donor atom (antenna) is initially resonantly excited by circularly polarized…
The relation between crystal symmetries, electron correlations, and electronic structure steers the formation of a large array of unconventional phases of matter, including magneto-electric loop currents and chiral magnetism. Detection of…
Free electrons can efficiently absorb or emit plasmons excited in a thin conductor, giving rise to multiple energy peaks in the transmitted electron spectra separated by multiples of the plasmon energy. When the plasmons are chiral, this…
While spin polarization from synchrotron radiation is well established, the polarization of orbital angular momentum (OAM) in such radiative processes remains elusive. We study radiation and polarization of relativistic electrons in a…
We present a method for computing angle-resolved electron-energy-loss and gain spectroscopies for phonon and magnon excitations in transmission electron microscopy. Fractional scattering intensities are derived from the…