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We investigate the fluorescence properties of colloidal quantum dots attached to gold rod nanoantennas. These structures are fabricated by a two step electron beam lithography process in combination with a chemical linking method. By…

When two or more metallic nanoparticles are in close proximity, their plasmonic modes may interact through the near field, leading to additional resonances of the coupled system or to shifts of their resonant frequencies. This process is…

We describe the process of Foerster transfer between semiconductor nanoparticles in the presence of a metal subsystem (metal nanocrystals). In the presence of metal nanocrystals, the Foerster process can become faster and more long-range.…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Alexander O. Govorov , Jaebeom Lee , Nicholas A. Kotov

We consider a hybrid plasmon-exciton system comprised of a resonant molecular subsystem and three Au wires supporting a dipole mode which can be coupled to a dark mode in controllable fashion by variation of a symmetry parameter. The…

Optics · Physics 2015-03-25 Maxim Sukharev , Paul N. Day , Ruth Pachter

Surface plasmon enhanced processes and hot-carrier dynamics in plasmonic nanostructures are of great fundamental interest to reveal light-matter interactions at the nanoscale. Using plasmonic tunnel junctions as a platform supporting both…

The interaction between intense light-matter not only promotes emerging applications in quantum and nonlinear optics but also facilitates changes in material properties. Plasmons can significantly enhance not only molecular chirality but…

Optics · Physics 2025-02-03 Nan Gao , Haoran Liu , Yurui Fang

Understanding the ultrafast processes at their natural-time scale is crucial for controlling and manipulating nanoscale optoelectronic devices under light-matter interaction. Here, we demonstrate that ultrafast plasmon resonances,…

Optics · Physics 2023-06-07 Hira Asif , Mehmet Emre Tasgin , Ramazan Sahin

Highly lossy nature of metals has severely limited the scope of practical applications of plasmonics. The conventional approach to circumvent this limitation has been to search for new materials with more favorable dielectric properties…

Optics · Physics 2019-07-11 H. Serhat Tetikol , M. Irsadi Aksun

The common model to describe exciton-plasmon interaction phenomenologically is the coupled oscillator model. Originally developed for atomic systems rather than solid-state matter, this model treats both excitons and plasmons as single…

Mesoscale and Nanoscale Physics · Physics 2024-10-23 Lara Greten , Robert Salzwedel , Diana Schutsch , Andreas Knorr

We measured the second-order correlation function of the cathodoluminescence intensity and investigated the Purcell effect by comparing the lifetimes of quantum emitters with and without metal structure. The increase in the electromagnetic…

The lifetime of localized surface plasmon plays an important role in many aspects of plasmonics and its applications. In small metal nanostructures, the dominant mechanism restricting plasmon lifetime is size-dependent Landau damping. We…

Mesoscale and Nanoscale Physics · Physics 2016-10-18 A. S. Kirakosyan , M. I. Stockman , T. V. Shahbazyan

Crystals of plasmonic metal nanoparticles have intriguing optical properties. They reach the regimes of ultrastrong and deep strong light-matter coupling, where the photonic states need to be included in the simulation of material…

Investigating nanoplasmonics using time-dependent approaches permits shedding light on the dynamic optical properties of plasmonic structures, which are intrinsically connected with their potential applications in photochemistry and…

Mesoscale and Nanoscale Physics · Physics 2024-06-18 Piero Lafiosca , Luca Nicoli , Silvio Pipolo , Stefano Corni , Tommaso Giovannini , Chiara Cappelli

Plasmonically enhanced fluorescence is a widely studied and applied phenomenon, however only a comparative theoretical and experimental analyses of coupled fluorophores and plasmonic nanoresonators makes it possible to uncover, how this…

The spontaneous fluorescence rates of single-molecule emitters are typically on the order of nanoseconds. However coupling them with plasmonic nanostructures can substantially increase their fluorescence yields. The confinement between the…

Mesoscale and Nanoscale Physics · Physics 2024-02-01 Jiří Doležal , Amandeep Sagwal , Rodrigo Cezar de Campos Ferreira , Martin Švec

There is an increasing scientific and technological interest on the design and implementation of nanoscale sources of quantum light. Here, we investigate the quantum statistics of the light scattered from a plasmonic nanocavity coupled to a…

Mesoscale and Nanoscale Physics · Physics 2019-03-14 R. Sáez-Blázquez , J. Feist , A. I. Fernández-Domínguez , F. J. García-Vidal

Quantum aspects, such as electron tunneling between closely separated metallic nanoparticles, are crucial for understanding the plasmonic response of nanoscale systems. We explore quantum effects on the response of the conductively coupled…

Materials Science · Physics 2015-12-08 Tuomas P. Rossi , Asier Zugarramurdi , Martti J. Puska , Risto M. Nieminen

Controlling quantum light-matter interactions at scales smaller than the diffraction limit at the single quantum emitter level is a critical challenge to the goal of advancing quantum technologies. We introduce a novel material platform…

The synthesis of metallic nanoparticle assemblies is nowadays well-controlled, such that these systems offer the possibility of controlling light at a sub-wavelength scale, thanks, for instance, to surface plasmons. Determining the energy…

Mesoscale and Nanoscale Physics · Physics 2025-10-06 Olivier Masset , Roland Bastardis , Francois Vernay

Multilayer assemblies of metal nanoparticles can act as photonic structures, where collective plasmon resonances hybridize with cavity modes to create plasmon-polariton states. For sufficiently strong coupling, plasmon polaritons…