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We discuss the emergence and growth of the cooperativity accompanying vitrification based on the density fluctuation dynamics for fragile glass-forming liquids. (i) The relaxation of density fluctuations proceeds by the particle (density)…

Soft Condensed Matter · Physics 2019-11-11 Akira Furukawa

We investigate the relation between the cooperative length and the relaxation time, represented respectively by the culling time and the persistence time, in the Fredrickson-Andersen, Kob-Andersen and spiral kinetically-constrained models.…

Statistical Mechanics · Physics 2015-10-01 Eial Teomy , Yair Shokef

We use molecular dynamics computer simulations to study the relaxation dynamics of Na2O-2(SiO2) in its molten, highly viscous state. We find that at low temperatures the incoherent intermediate scattering function for Na relaxes about 100…

Statistical Mechanics · Physics 2009-11-07 Jurgen Horbach , Walter Kob

We present the results of a large scale molecular dynamics computer simulation of a binary, supercooled Lennard-Jones fluid. At low temperatures and intermediate times the time dependence of the intermediate scattering function is well…

Condensed Matter · Physics 2009-10-22 Walter Kob , Hans C. Andersen

The evolution of non-hydrodynamic slow processes near the QCD critical point is explored with the novel Hydro+ framework, which extends the conventional hydrodynamic description by coupling it to additional explicitly evolving slow modes…

Nuclear Theory · Physics 2020-12-01 Lipei Du , Ulrich Heinz , Krishna Rajagopal , Yi Yin

Using molecular dynamics simulations of a binary Lennard-Jones model of glass-forming liquids, we examine how the decay of the normalized neighbor-persistence function $C_{\rm B}(t)$, which decays from unity at short times to zero at long…

Soft Condensed Matter · Physics 2025-02-04 Katrianna S. Sarkar , Kevin A. Interiano-Alberto , Jack F. Douglas , Robert S. Hoy

A molecular dynamics simulation is performed for a supercooled liquid of rigid diatomic molecules. The time-dependent self and collective density correlators of the molecular centers of mass are determined and compared with the predictions…

Statistical Mechanics · Physics 2009-10-30 Stefan Kammerer , Walter Kob , Rolf Schilling

We present the results of a large scale computer simulation of supercooled silica. We find that at high temperatures the diffusion constants show a non-Arrhenius temperature dependence whereas at low temperature this dependence is also…

Disordered Systems and Neural Networks · Physics 2015-06-25 Jurgen Horbach , Walter Kob , Kurt Binder

In the present study, we performed molecular-dynamics simulations and investigated dynamical heterogeneity in a supercooled liquid under a steady shear flow. Dynamical heterogeneity can be characterized by three quantities: the correlation…

Soft Condensed Matter · Physics 2012-04-25 Hideyuki Mizuno Ryoichi Yamamoto

We discuss the density fluctuations of a fluid due to zero point motion. These can be regarded as density fluctuations in the phonon vacuum state. We assume a linear dispersion relation with a fixed speed of sound and calculate the density…

Quantum Physics · Physics 2010-04-22 L. H. Ford , N. F. Svaiter

The relaxation dynamics of a model fluid of platelike colloidal particles is investigated by means of a phenomenological dynamic density functional theory. The model fluid approximates the particles within the Zwanzig model of restricted…

Soft Condensed Matter · Physics 2011-09-14 Markus Bier , Rene van Roij

The emergence of the solid state in glass-forming materials upon cooling is accompanied by changes in both thermodynamic and viscoelastic properties and by a precipitous drop in fluidity. Here, we investigate changes in basic elastic…

Soft Condensed Matter · Physics 2023-06-14 Xiaolei Xu , Jack F. Douglas , Wen-Sheng Xu

In the realm of nanoscience, the dynamic behaviors of liquids at scales beyond the conventional structural relaxation time, $\tau$, unfold a fascinating blend of solid-like characteristics, including the propagation of collective shear…

Soft Condensed Matter · Physics 2024-09-11 Yuanxi Yu , Sha Jin , Xue Fan , Mona Sarter , Dehong Yu , Liang Hong , Matteo Baggioli

Inspired by one--dimensional light--particle systems, the dynamics of a non-Hamiltonian system with long--range forces is investigated. While the molecular dynamics does not reach an equilibrium state, it may be approximated in the…

Statistical Mechanics · Physics 2019-01-23 Romain Bachelard , Nicola Piovella , Shamik Gupta

The absence of a simple fluctuation-dissipation theorem is a major obstacle for studying systems that are not in thermodynamic equilibrium. We show that for a fluid in a non-equilibrium steady state characterized by a constant temperature…

Statistical Mechanics · Physics 2024-07-03 T. R. Kirkpatrick , D. Belitz

Large scale simulations of two-dimensional bidisperse granular fluids allow us to determine spatial correlations of slow particles via the four-point structure factor $S_4(q,t)$. Both cases, elastic ($\varepsilon=1$) as well as inelastic…

Statistical Mechanics · Physics 2014-07-16 Karina E. Avila , Horacio E. Castillo , Andrea Fiege , Katharina Vollmayr-Lee , Annette Zippelius

We propose a theoretical framework for the dynamics of bulk isotropic hard-sphere systems in the presence of randomly pinned particles and apply this theory to supercooled water to validate it. Structural relaxation is mainly governed by…

Soft Condensed Matter · Physics 2022-09-14 Anh D. Phan

We investigate dynamical heterogeneities in the collective relaxation of a concentrated microgel system, for which the packing fraction can be conveniently varied by changing the temperature. The packing fraction dependent mechanical…

Soft Condensed Matter · Physics 2011-05-31 David A. Sessoms , Irmgard Bischofberger , Luca Cipelletti , Véronique Trappe

We report a molecular dynamics (MD) study of the collective dynamics of a simple monatomic liquid -interacting through a two body potential that mimics that of lithium- across the liquid-glass transition. In the glassy phase we find…

Disordered Systems and Neural Networks · Physics 2009-11-07 T. Scopigno , G. Ruocco , F. Sette , G. Viliani

Collective response dynamics of a strongly coupled system departs from the continuum phase upon transition to the quasicrystalline phase, or formation of a Wigner lattice. The wave nonlinearity leading to the modulational instability in…

Plasma Physics · Physics 2023-01-25 Sandip Dalui , Prince Kumar , Devendra Sharma