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The orthorhombic phase of Si-doped Fe carbide is synthesized at high pressures and temperatures using laser-heated diamond anvil cell (LHDAC), followed by its characterization using X-ray diffraction (XRD) measurements, Transmission…

Materials Science · Physics 2020-11-17 Pinku Saha , Konstantin Glazyrin , Goutam Dev Mukherjee

Fe-bearing MgO [(Mg$_{1-x}$Fe$_x$)O] is considered a major constituent of terrestrial exoplanets. Crystallizing in the B1 structure in the Earth's lower mantle, (Mg$_{1-x}$Fe$_x$)O undergoes a high-spin ($S=2$) to low-spin ($S=0$)…

Materials Science · Physics 2022-05-20 Han Hsu , Koichiro Umemoto

We report the magnetic and electrical characteristics of a polycrystalline specimen of FeTiO3 synthesized at high pressure that is isostructural with acentric LiNbO3 (LBO). Piezoresponse force microscopy, optical second harmonic generation,…

We report the first high pressure measurement of the Fe K-edge in hematite (Fe$_2$O$_3$) by X-ray absorption spectroscopy in partial fluorescence yield geometry. The pressure-induced evolution of the electronic structure as Fe$_2$O$_3$…

Being a lithophile element at ambient pressure, magnesium is long believed to be immiscible with iron. A recent study by Gao et al. [1] showed that pressure turns magnesium into a siderophile element and can produce unconventional Fe-Mg…

Using M\"ossbauer and EPR spectroscopy we have studied the insulating ferromagnetic La$_{1-x}$Ca$_x$Mn$_{0.99}$$^{57}$Fe$_{0.01}$O$_3$ ($x=0.175$) compound prepared in air and reduced atmosphere. The average hyperfine field follows a mean…

Strongly Correlated Electrons · Physics 2007-05-23 M. Pissas , G. Papavassiliou , E. Devlin , A. Simopoulos , V. Likodimos

Elements of group I in the Periodic table have valence electrons of s-type and are usually considered as simple metals. Crystal structures of these elements at ambient pressure are close-packed and high-symmetry of bcc and fcc types,…

Materials Science · Physics 2017-03-14 V F Degtyareva

Oxygen vacancies (VOs) effects on magnetic ordering in Eu0.5Ba0.5TiO3-{\delta} (EBTO3-{\delta}) thin films have been investigated using a combination of experimental measurements and first-principles density-functional calculations. Two…

Since the discovery of charge disproportionation in the FeO$_2$ square-lattice compound Sr$_3$Fe$_2$O$_7$ by M\"ossbauer spectroscopy more than fifty years ago, the spatial ordering pattern of the disproportionated charges has remained…

The effects of Fe-ion irradiation on the crystal structure and superconducting properties of MgB$_2$ thin films were investigated. Pristine samples were prepared using hybrid physical-chemical vapor deposition (HPCVD), and ion irradiation…

We present a combined experimental and computational first-principles study of the superionic and structural properties of CaF2 at high P-T conditions. We observe an anomalous superionic behavior in the low-P fluorite phase that consists in…

Materials Science · Physics 2015-06-19 Claudio Cazorla , Daniel Errandonea

We perform density functional calculations of the equilibrium 57Fe/54Fe ratios for ferrous iron dissolved in periclase and MgSiO3 perovskite at the pressures and temperatures of the Earth's mantle. Pressure increases the partitioning of…

Materials Science · Physics 2008-07-31 James R. Rustad , Piotr Zarzycki , Maryali P. Sauceda , Qing-zhu Yin

The emission spectra and the ionization structure of the low ionization stages of iron, Fe I--IV, in gaseous nebulae are studied. This work includes: (i) new atomic data: photoionization cross sections, total e-ion recombination rates,…

Astrophysics · Physics 2009-10-30 Manuel A. Bautista , Anil K. Pradhan

An oxygen hyperstoichiometric ferrite CaBaFe4O7+\delta (\delta \approx 0.14) has been synthesized using "soft" reduction of CaBaFe4O8. Like the oxygen stoichiometric ferrimagnet CaBaFe4O7, this oxide also keeps the hexagonal symmetry (space…

Strongly Correlated Electrons · Physics 2011-03-16 Tapati Sarkar , V. Duffort , V. Pralong , V. Caignaert , B. Raveau

An unusual Fe-H bonding rather than conventional OH bonding is identified at Fe3O4 (001) surface. This abnormal behavior is associated with the oxygen vacancies which exist on the surface region but also penetrate deep into the bulk Fe3O4.…

Strongly Correlated Electrons · Physics 2016-11-23 Fangyang Liu , Chen Chen , Hangwen Guo , Mohammad Saghayezhian , Gaomin Wang , Lina Chen , Wei Chen , Jiandi Zhang , E. W. Plummer

On account of the rapid development of noble gas chemistry in the past half-century both xenon and krypton compounds can now be isolated in macroscopic quantities. The same though does not hold true for the next lighter group 18 element,…

Materials Science · Physics 2021-11-01 Dominik Kurzydłowski , Patryk Zaleski-Ejgierd

We have successfully synthesized a new layered iron oxychalcogenide BaFe2OSe2 single crystal. This compound is built up of Ba and Fe-Se(O) layers alternatively stacked along the c-axis. The Fe-Se(O) layers contain double chains of…

Superconductivity · Physics 2015-06-05 Hechang Lei , Hyejin Ryu , John Warren , A. I. Frenkel , V. Ivanovski , B. Cekic , C. Petrovic

MSr2Y1.5Ce0.5Cu2Oz (M-1222) compounds, with M = Fe and Co, have been synthesized through a solid-state reaction route. Both compounds crystallize in a tetragonal structure (space group I4/mmm). A Rietveld structural refinement of…

Strongly Correlated Electrons · Physics 2016-08-31 V. P. S. Awana , Anurag Gupta , H. Kishan , S. K. Malik , W. B. Yelon , J. Linden , M. Karppinen , H. Yamauchi

Effect of He ion irradiation on three model Fe(100-x)Cr(x) alloys (x =5.8, 10.75 and 15.15) was investigated with the conversion electron M\"ossbauer spectroscopy. The study of the alloys irradiated with 25 keV ions revealed that the…

Materials Science · Physics 2014-11-21 S. M. Dubiel , J. Cieslak , H. Reuther

Density functional based simulations are employed to explore magnetoelectric effects in iron-based oxides, showing a unique layered structure. We theoretically predict CaFeO2 to be a promising magnetoelectric, showing…

Strongly Correlated Electrons · Physics 2015-06-15 Kunihiko Yamauchi , Tamio Oguchi , Silvia Picozzi