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We demonstrate a simple and scalable approach to increase conversion efficiencies of nonlinear metasurfaces by incorporating them into multipass cells and by letting the pump beam to interact with the metasurfaces multiple times. We…

Attosecond light sources based on high-order harmonic generation (HHG) constitute to date the only table-top solution for producing coherent broadband radiation covering the spectral range from the extreme ultraviolet to the soft X-rays.…

We propose a novel picture of high-harmonic generation (HHG) in solids based on the concept of temporally changing band structures. To demonstrate the utility of this picture, we focus on the high-order sideband generation (HSG) caused by…

Materials Science · Physics 2019-08-14 Tomohiro Tamaya , Takeo Kato

Owing to the discrete frequency spectrum of whispering gallery resonators (WGRs), the resonance and phase-matching conditions for the interacting waves in the case of second-harmonic generation (SHG) cannot generally be fulfilled…

Optics · Physics 2021-04-23 Jan Szabados , Nicolás Amiune , Boris Sturman , Ingo Breunig

Time-varying metamaterials rely on large and fast changes of the linear permittivity. Beyond the linear terms, however, the effect of a non-perturbative modulation of the medium on harmonic generation and the associated nonlinear…

High harmonic generation (HHG) is an extreme nonlinear frequency up-conversion process during which extremely short duration optical pulses at very short wavelengths are emitted. A major concern of HHG is the small conversion efficiency at…

A laser pulse composed of a fundamental and an appropriately phased second harmonic can drive a time-dependent current of photoionized electrons that generates broadband THz radiation. Over the propagation distances relevant to many…

By employing a pump-probe technique for enhanced spectral mapping of the dynamics in nonlinear frequency conversion, we demonstrate that photo-induced second-harmonic generation (SHG) in silicon nitride (Si3N4) microresonators can persist…

Diffractive neural networks (DNNs) are an emerging approach for the realization of photonic artificial intelligence, especially due to their suitability for machine-vision applications and high-dimensional photonic information processing at…

Optics · Physics 2026-03-27 Marie Braasch , Anna Kartashova , Elena Goi , Thomas Pertsch , Sina Saravi

Solid-state high harmonic generation spectroscopy (sHHG) is a promising technique for studying electronic structure, symmetry, and dynamics in condensed matter systems. Here, we report on the implementation of an advanced sHHG spectrometer…

Since the first observation of second harmonic generation (SHG), there have been extensive studies on this nonlinear phenomenon not only to clarify its physical origin but also to realize unconventional functionalities. Nonetheless, a…

Integrated thin-film lithium niobate platform has recently emerged as a promising candidate for next-generation, high-efficiency wavelength conversion systems that allow dense packaging and mass-production. Here we demonstrate efficient,…

Optical second harmonic generation (SHG) is a nonlinear optical effect widely used for nonlinear optical microscopy and laser frequency conversion. Closed-form analytical solution of the nonlinear optical responses is essential for…

High-harmonic generation is one of the most extreme nonlinear-optical processes observed to date. By focusing an intense laser pulse into a gas, the light-atom interaction that occurs during the process of ionising the atoms results in the…

Nonlinear frequency conversion provides essential tools for light generation, photon entanglement, and manipulation. Transition metal dichalcogenides (TMDs) possess huge nonlinear susceptibilities and 3R-stacked TMD crystals further combine…

For the growing demand of frequency combs in mid-infrared (mid-IR), known as the "molecular fingerprint" region of the spectrum [1], down conversion of near-IR frequency combs through half- harmonic generation offers numerous benefits…

Optics · Physics 2015-10-14 Alireza Marandi , Kirk A. Ingold , Marc Jankowski , Robert L. Byer

We theoretically study the generation of optical frequency combs and corresponding pulse trains in doubly resonant intracavity second-harmonic generation (SHG). We find that, despite the large temporal walk-off characteristic of realistic…

Optics · Physics 2016-04-27 F. Leo , T. Hansson , I. Ricciardi , M. De Rosa , S. Coen , S. Wabnitz , M. Erkintalo

We theoretically demonstrate x-ray second harmonic generation (SHG) with strong-field-driven high harmonic generation (HHG) from core electrons in gas-phase atoms, highlighting its potential as a powerful spectroscopic tool for studying…

Atomic Physics · Physics 2025-03-31 Xinhua Xie

Recent advancements in ultrafast laser systems and high harmonic generation (HHG) techniques have enabled time-resolved photoemission spectroscopy on femtosecond timescales, opening up unprecedented opportunities to explore quantum…

Strongly Correlated Electrons · Physics 2025-11-03 Takeshi Suzuki , Kozo Okazaki

We theoretically investigate second harmonic generation that originates from the nonlinear, magnetic Lorentz force term from single and multiple apertures carved on thick, opaque metal substrates. The linear transmission properties of…