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We consider counterions in the presence of a single planar surface with a spatially inhomogeneous charge distribution using Monte-Carlo simulations and strong-coupling theory. For high surface charges, multivalent counterions, or pronounced…

Soft Condensed Matter · Physics 2009-11-07 Andre G Moreira , Roland R Netz

Similarly-charged polyelectrolytes are known to attract each other and aggregate into bundles when the charge density of the polymers exceeds a critical value that depends on the valency of the counterions. The dynamics of aggregation of…

Soft Condensed Matter · Physics 2016-09-22 Anvy Moly Tom , R. Rajesh , Satyavani Vemparala

This paper studies mechanism of preconcentration of charged particles in a straight micro-channel embedded with permselective membranes, by numerically solving coupled transport equations of ions, charged particles and solvent fluid without…

Fluid Dynamics · Physics 2018-02-14 Zirui Li , Wei Liu , Yudan Zhu , Xiaohua Lu , Yuantong Gu , Jongyoon Han

Aqueous cations permeate subnanoscale pores by crossing free energy barriers dominated by competing enthalpic contributions from transiently decreased ion-solvent and increased ion-pore electrostatic interactions. This commonly accepted…

Mesoscale and Nanoscale Physics · Physics 2025-09-18 Yechan Noh , Demian Riccardi , Alex Smolyanitsky

The complexation between charged-neutral block copolymers and oppositely charged surfactants was investigated by light scattering experiments and by isothermal titration calorimetry (ITC). The copolymer was poly(sodium…

Materials Science · Physics 2011-07-27 J. Courtois , J. -F. Berret

In this review, we address the issue of the electrostatic complexation between charged-neutral diblock copolymers and oppositely charged nanocolloids. We show that nanocolloids such as surfactant micelles and iron oxide magnetic…

Soft Condensed Matter · Physics 2011-02-01 J. -F. Berret

Using the complex Langevin sampling strategy, field theoretic simulations are performed to study the equilibrium phase behavior and structure of symmetric polycation-polyanion mixtures without salt in good solvents. Static structure factors…

Soft Condensed Matter · Physics 2008-06-14 Jonghoon Lee , Yuri O. Popov , Glenn H. Fredrickson

We study the response of a model micro-electrochemical cell to a large ac voltage of frequency comparable to the inverse cell relaxation time. To bring out the basic physics, we consider the simplest possible model of a symmetric binary…

Fluid Dynamics · Physics 2013-12-12 Laurits H. Olesen , Martin Z. Bazant , Henrik Bruus

We study mixtures of charged surfactants, which alone in solution form uni- and multilamellar vesicles, and oppositely charged polyelectrolytes (PEs). The phase behavior is investigated at fixed surfactant concentration as a function of the…

Soft Condensed Matter · Physics 2007-05-23 Laurence Ramos , Edith Vivares

We model cyclic voltammetry experiments on supported lipid films where a non-trivial dependence of the capacitance on the applied voltage is observed. Previously, based on a mean-field treatment of the Flory-Huggins type, under the…

Soft Condensed Matter · Physics 2010-07-28 Andrey V. Brukhno , Anna Akinshina , Zachary Coldrick , Andrew Nelson , Stefan Auer

We examine the phase transition of polymer adsorption as well as the underlying kinetics of polymer binding from dilute solutions on a structureless solid surface. The emphasis is put on the properties of regular multiblock copolymers,…

Soft Condensed Matter · Physics 2009-09-03 A. Milchev , V. Rostiashvili , S. Bhattacharya , T. Vilgis

The adsorption of flexible and highly charged polyelectrolytes onto oppositely charged planar surfaces is investigated by means of Monte Carlo simulations. The effect of image forces stemming from the dielectric discontinuity at the…

Soft Condensed Matter · Physics 2016-08-31 Rene Messina

We present an experimentally guided, multi-phase, multi-species polyelectrolyte gel model to make quantitative predictions on the electro-chemical properties of articular cartilage. The mixture theory consists of two different types of…

Tissues and Organs · Quantitative Biology 2013-08-22 Sarthok Sircar , Elizabeth Aisenbrey , Stephanie J. Bryant , David M. Bortz

Poisson-Boltzmann theory is the cornerstone for soft matter electrostatics. We provide novel exact analytical solutions to this non-linear mean-field approach, for the diffuse layer of ions in the vicinity of a planar or a cylindrical…

Soft Condensed Matter · Physics 2020-01-29 L. Samaj , E. Trizac

Aggregation of stiff polyelectrolytes in solution and angle- and distance-dependent potential of mean force between two like-charged rods are studied in the presence of 3-valent salt using molecular dynamics simulations. In the bulk…

Soft Condensed Matter · Physics 2009-03-25 Sarah Mohammadinejad , Hossein Fazli , Ramin Golestanian

We study a classical system of identically charged counter-ions near a planar wall carrying a uniform surface charge density. The equilibrium statistical mechanics of the system depends on a single dimensionless coupling parameter. A new…

Soft Condensed Matter · Physics 2019-01-21 I. Palaia , M. Trulsson , L. Samaj , E. Trizac

The effective charge of a rigid polyelectrolyte (PE) approaching an oppositely charged surface is studied. The cases of a weak (annealed) and strongly charged PE with condensed counterions (such as DNA) are discussed. In the most…

Soft Condensed Matter · Physics 2009-10-31 Pierre Sens , Jean-Francois Joanny

Structural and thermodynamic properties of the model solution containing charged oligomers and the equivalent number of counterions were studied by means of the canonical Monte Carlo simulation technique. The oligomers are represented as…

Soft Condensed Matter · Physics 2012-02-21 T. Sajevic , J. Rescic , V. Vlachy

Recently plasmon excitations in bilayer lattice systems were studied extensively in the weak-coupling regime. Unlike single-layer systems, these bilayers exhibit two distinct modes, $\omega_{\pm}$, which show characteristic dependences upon…

Strongly Correlated Electrons · Physics 2026-01-21 Hiroyuki Yamase , Luciano Zinni , Matías Bejas , Andrés Greco

The formation of inter-polyelectrolyte complexes from the association of oppositely charged polymers in an electrolyte is studied. The charged polymers are linear oppositely charged polyelectrolytes, with possibly a neutral block. This…

Soft Condensed Matter · Physics 2012-06-27 Vladimir A. Baulin , Emmanuel Trizac
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