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Time-dependent density-functional theory (TDDFT) is widely used to describe electronic excitations in complex finite systems with large numbers of atoms, such as biomolecules and nanocrystals. The first part of this paper will give a simple…

Materials Science · Physics 2008-08-15 C. A. Ullrich , V. Turkowski

We consider the elastic scattering of electrons by hydrogen atoms in the presence of a two-color circularly polarized laser field in the domain of moderate intensities below $10^{13}$ W/cm$^2$ and high projectile energies. A hybrid approach…

Atomic Physics · Physics 2023-06-16 Gabriela Buica

High-resolution photoelectron momentum distributions of Xe atoms ionized by 800-nm linearly polarized laser fields have been traced at intensities from 1.1*1013 to 3.5*1013W/cm2 using velocity-map imaging techniques. At certain laser…

Atomic Physics · Physics 2015-12-09 Min Li , Peng Zhang , Siqiang Luo , Yueming Zhou , Qingbin Zhang , Pengfei Lan , Peixiang Lu

Using the recently developed Coulomb Quantum Orbit Strong-Field Approximation (CQSFA), we perform a systematic analysis of several features encountered in above-threshold ionization (ATI) photoelectron angle-resolved distributions (PADs),…

Atomic Physics · Physics 2017-10-11 A. S. Maxwell , A. Al-Jawahiry , T. Das , C. Figueira de Morisson Faria

We discuss the theory of coupled ionization--dissociation fronts produced when molecular clouds are exposed to $\lambda < 1110$\AA\ radiation from hot stars. A steady, composite structure is developed, which generally includes an ionized…

Astrophysics · Physics 2009-10-28 Frank Bertoldi , B. T. Draine

A robust and efficient frequency dependent and non-local exchange-correlation $f_{xc}(r,r';\omega)$ is derived by imposing time-dependent density-functional theory (TDDFT) to reproduce the many-body diagrammatic expansion of the…

Materials Science · Physics 2009-11-10 A. Marini , R. Del Sole , A. Rubio

The laser-induced fragmentation dynamics of this most fundamental polar molecule HeH$^+$ are measured using an ion beam of helium hydride and an isotopologue at various wavelengths and intensities. In contrast to the prevailing…

Chemical Physics · Physics 2018-08-21 P. Wustelt , F. Oppermann , Lun Yue , M. Möller , T. Stöhlker , S. Gräfe , M. Lein , G. G. Paulus , A. M. Sayler

High-order harmonic generation via single-slit diffraction of relativistic laser pulses is investigated. Using fully kinetic 2D and 3D particle-in-cell simulations, we show that interesting optical phenomena emerge, including the generation…

Plasma Physics · Physics 2025-05-07 Longqing Yi

We study ionization of atoms in strong elliptically-polarized laser fields numerically and analytically. We focus on effects of laser ellipticity on the offset angle in photoelectron momentum distribution. This angle is considered to encode…

Atomic Physics · Physics 2023-04-26 J. Y. Che , J. Y. Huang , F. B. Zhang , C. Chen , G. G. Xin , Y. J. Chen

We show that atomic alignment presents a reliable way to study topology of astrophysical magnetic fields. The effect of atomic alignment arises from modulation of the relative population of the sublevels of atomic ground state pumped by…

Astrophysics · Physics 2008-11-26 Huirong Yan , A. Lazarian

A theoretical study of ionization of the hydrogen atom due to an XUV pulse in the presence of an IR laser is presented. Well-established theories are usually used to describe the problem of laser assisted photoelectron effect. However, the…

Atomic Physics · Physics 2017-11-10 A A Gramajo , R Della Picca , S D López , D G Arbó

The depolarized light scattering spectra of the glass forming liquid ortho-terphenyl have been calculated in the low frequency region using molecular dynamics simulation. Realistic system's configurations are produced by using a recent…

Soft Condensed Matter · Physics 2009-11-07 S. Mossa , G. Ruocco , M. Sampoli

We propose a real-time time-dependent ab__initio approach within a configuration-interaction-singles ansatz to decompose the high-harmonic generation (HHG) signal of molecules in terms of individual molecular-orbital (MO) contributions.…

Chemical Physics · Physics 2025-12-11 Marco Marchetta , Chiara Morassut , Julien Toulouse , Emanuele Coccia , Eleonora Luppi

We explore from a theoretical perspective angular distributions of electrons emitted from a Na$_8$ cluster after excitation by a short laser pulse. The tool of the study is time-dependent density-functional theory (TDDFT) at the level of…

Other Condensed Matter · Physics 2010-01-06 M. Baer , P. M. Dinh , L. V. Moskaleva , P. -G. Reinhard , N. Roesch , E. Suraud

We explore the effects of disordered charged defects on the electronic excitations observed in the photoemission spectra of doped transition metal oxides in the Mott insulating regime by the example of the $R_{1-x}$Ca$_x$VO$_3$ perovskites,…

Strongly Correlated Electrons · Physics 2018-04-09 Adolfo Avella , Andrzej M. Oleś , Peter Horsch

Despite spin (SAM) and orbital (OAM) angular momentum dynamics are well-studied in demagnetization processes, their components receive less focus. Here, we utilize the non-collinear spin version of real-time time-dependent density…

Mesoscale and Nanoscale Physics · Physics 2024-02-28 Junjie He , Shuo Li , Thomas Fruenheim

The spectral distribution of positron created by photon and the spectral distribution of photons radiated from electron in an oriented single crystal of intermediate thickness is calculated at intermediate energies. The energy loss of…

High Energy Physics - Phenomenology · Physics 2011-07-14 V. N. Baier , V. M. Katkov

The process of radiation from high-energy electron and electron-positron pair production by a photon in oriented single crystal is considered using the method which permits inseparable consideration of both coherent and incoherent…

High Energy Physics - Phenomenology · Physics 2009-11-11 V. N. Baier , V. M. Katkov

We present a machine learning algorithm for the prediction of molecule properties inspired by ideas from density functional theory. Using Gaussian-type orbital functions, we create surrogate electronic densities of the molecule from which…

Chemical Physics · Physics 2019-11-27 Michael Eickenberg , Georgios Exarchakis , Matthew Hirn , Stéphane Mallat , Louis Thiry