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In this paper we study the response in time of N$_2$, O$_2$ and F$_2$ to laser pulses having a wavelength of 390nm. We find single ionization suppression in O$_2$ and its absence in F$_2$, in accordance with experimental results at $\lambda…

Quantum Physics · Physics 2009-11-10 Daniel Dundas , Jan M. Rost

Recent direct experimental observation of multiple highly-dispersive C$_{60}$ valence bands has allowed for a detailed analysis of the unique photoemission traits of these features through photon energy- and polarization-dependent…

Mesoscale and Nanoscale Physics · Physics 2023-01-18 Drew W. Latzke , Claudia Ojeda-Aristizabal , Jonathan D. Denlinger , Ryan Reno , Alex Zettl , Alessandra Lanzara

We focus on studying the opacity of iron, chromium, and nickel plasmas at conditions relevant to experiments carried out at Sandia National Laboratories [J. E. Bailey et al., Nature 517, 56 (2015)]. We calculate the photo-absorption…

Plasma Physics · Physics 2021-04-28 N. M. Gill , C. J. Fontes , C. E. Starrett

Photoelectron circular dichroism refers to the forward/backward asymmetry in the photoelectron angular distribution with respect to the propagation axis of circularly polarized light. It has recently been demonstrated in femtosecond…

Quantum Physics · Physics 2017-01-16 R. E. Goetz , T. A. Isaev , B. Nikoobakht , R. Berger , C. P. Koch

Using the molecular strong-field approximation we consider the effects of molecular symmetry on the ionization of molecules by a strong, linearly polarized laser pulse. Electron angular distributions and total ionization yields are…

The alignment dependence of the ionization behavior of H$_2$ exposed to intense ultrashort laser pulses is investigated on the basis of solutions of the full time-dependent Schr\"odinger equation within the fixed-nuclei and dipole…

Quantum Physics · Physics 2013-05-29 Yulian V. Vanne , Alejandro Saenz

The creation and detection of atomic polarization is examined theoretically, through the study of basic optical-pumping mechanisms and absorption and fluorescence measurements, and the dependence of these processes on the size of ground-…

Atomic Physics · Physics 2013-05-29 M. Auzinsh , D. Budker , S. M. Rochester

The orientational distribution function of the nematic phase of the semi-flexible rod-like virus fd is measured by x-ray diffraction as a function of concentration and ionic strength. The angular distribution of the scattered intensity from…

Soft Condensed Matter · Physics 2013-05-29 K. R. Purdy , Z. Dogic , S. Fraden , A. Ruehm , L. Lurio , S. G. J. Mochrie

Supplementing our STM and electron emission studies investigations, concluding in electron pairing in strong laser fields [1], further time-of-flight electron emission studies were carried out, changing the angle of polarization of the…

Optics · Physics 2015-06-02 N. Kroó , P. Rácz , S. Varró

We demonstrate that the angular distribution of photoelectrons from a strongly polarizable target exposed to a laser field can deviate noticeably from the prediction of conventional theory. Even within the dipole-photon approximation the…

Atomic and Molecular Clusters · Physics 2009-11-13 A. V. Korol , A. V. Solov'yov

We present combined experimental and theoretical results on strong-field ionization of oriented carbonyl-sulphide molecules by circularly-polarized laser pulses. The obtained molecular frame photoelectron angular distributions show…

Combining classical electrodynamics and density functional theory (DFT) calculations, we develop a general and rigorous theoretical framework that describes the energetics of metal surfaces under high electric fields. We show that the…

Materials Science · Physics 2019-05-22 Andreas Kyritsakis , Ekaterina Baibuz , Ville Jansson , Flyura Djurabekova

Tunneling ionization of an atom in ultrashort laser pulses is considered. When the driving laser pulse is switched-on and -off with a steep slope, the photoelectron momentum distribution (PMD) shows an edge-effect because of the…

Atomic Physics · Physics 2022-07-07 M. Klaiber , Q. Z. Lv , K. Z. Hatsagortsyan , C. H. Keitel

The application of a matrix-based reconstruction protocol for obtaining Molecular Frame (MF) photoelectron angular distributions (MFPADs) from laboratory frame (LF) measurements (LFPADs) is explored. Similarly to other recent works on the…

Chemical Physics · Physics 2021-09-01 Margaret Gregory , Paul Hockett , Albert Stolow , Varun Makhija

The photodissociation of the HD+ molecular ion in intense short- pulsed linearly polarized laser fields is studied using a time- dependent wave-packet approach where molecular rotation is fully included. We show that applying a coherent…

chem-ph · Physics 2019-04-04 Eric Charron , Annick Giusti-Suzor , Frederick Mies

We consider deflection of polarizable molecules by inhomogeneous optical fields, and analyze the role of molecular orientation and rotation in the scattering process. It is shown that molecular rotation induces spectacular rainbow-like…

Quantum Physics · Physics 2015-05-19 E. Gershnabel , I. Sh. Averbukh

Resonant angle scanned x-ray photoelectron diffraction (RXPD) allows the determination of the atomic and magnetic structure of surfaces and interfaces. For the case of magnetized nickel the resonant L2 excitation with circularly polarized…

Other Condensed Matter · Physics 2015-05-27 M. Morscher , F. Nolting , T. Brugger , T. Greber

We analyze the imprint of nodal planes in high-order harmonic spectra from aligned diatomic molecules in intense laser fields whose components exhibit orthogonal polarizations. We show that the typical suppression in the spectra associated…

Atomic Physics · Physics 2016-08-17 T. Das , C. Figueira de Morisson Faria

In the Kapitza-Dirac effect, atoms, molecules, or swift electrons are diffracted off a standing wave grating of the light intensity created by two counter-propagating laser fields. In ultrafast electron optics, such a coherent beam splitter…

Quantum Physics · Physics 2019-05-03 Nahid Talebi , Christoph Lienau

Novel low-band-gap copolymer oligomers are proposed on the basis of density functional theory (DFT) quantum chemical calculations of photophysical properties. These molecules have an electron donor-accepter (D-A) architecture involving…

Chemical Physics · Physics 2017-08-18 Tarek Mestiri , Ala Aldin M. H. M. Darghouth , Mark E. Casida , Kamel Alimi
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