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Lithium transition metal phospho-olivines are useful electrode materials, owing to their stability, high safety, low cost and cyclability. We report phonon studies using neutron inelastic scattering experiments, ab-initio density functional…

Materials Science · Physics 2014-08-19 Prabhatasree Goel , M. K. Gupta , R. Mittal , S. Rols , S. J. Patwe , S. N. Achary , A. K. Tyagi , S. L. Chaplot

We present results from ab initio calculations of the mechanical properties of the rhombohedral phase (beta) of vanadium metal reported in recent experiments, and other predicted high-pressure phases (gamma and bcc), focusing on properties…

Materials Science · Physics 2009-11-13 B. Lee , R. E. Rudd , J. E. Klepeis , R. Becker

We have used ab-initio density functional theory technique to understand the phase transitions and structural changes in various high temperature/pressure phases of LiAlO2. The electronic band structure as well as phonon spectra are…

Materials Science · Physics 2018-06-05 Baltej Singh , M. K. Gupta , R. Mittal , S. L. Chaplot

Ab initio investigations of structural, electronic, and dynamical properties of the high-temperature $\beta$ phase of copper pyrophosphate were performed using density functional theory. The electronic band structure shows the Mott…

Elastic and structural properties of $\beta$-Ga$_2$O$_3$ and $\alpha$-Ga$_2$O$_3$ are investigated from first principles. The full elastic tensors and elastic moduli of both phases at $0$ K are computed in the framework of semi-local…

Materials Science · Physics 2022-01-04 Konstantin Lion , Pasquale Pavone , Claudia Draxl

We report studies on the vibrational and elastic behavior of lithium oxide, Li2O around its superionic transition temperature. Phonon frequencies calculated using the ab-initio and empirical potential model are in excellent agreement with…

Materials Science · Physics 2012-06-04 M. K. Gupta , Prabhatasree Goel , R. Mittal , N. Choudhury , S. L. Chaplot

We study the temperature and pressure dependence of the structural and electronic properties of the iron pnictide superconductor BaFe2As2. We use density functional theory based Born-Oppenheimer molecular dynamics simulations to investigate…

Strongly Correlated Electrons · Physics 2013-08-06 Steffen Backes , Harald O. Jeschke

Plutonium dioxide is of high technological importance in nuclear fuel cycle and is particularly crucial in long-term storage of Pu-based radioactive waste. Using first-principles density-functional theory, in this paper we systematically…

Materials Science · Physics 2011-09-29 Ping Zhang , Bao-Tian Wang , Xian-Geng Zhao

We present a study of the structural phase transition, mechanical and thermodynamic properties of UO$_{2}$ by means of the local density approximation (LDA)$+U$ approach. A phase transition pressure of 40 GPa, which agrees well with the…

Strongly Correlated Electrons · Physics 2013-09-25 Bao-Tian Wang , Ping Zhang , Raquel Lizárraga , Igor Di Marco , Olle Eriksson

BaPd2As2 belongs to 122 pnictide group, famous for exhibiting superconductivity at high temperatures and other electronic correlations. Unlike the 122 iron arsenides, BaPd2As2 exhibits superconductivity at low temperature when realized in…

Superconductivity · Physics 2018-10-31 F. Parvin , S. H. Naqib

The elastic, thermodynamic, and optical properties of Mo_{2}TiAlC_{2} are investigated by first-principles calculations. Our results indicate that the a axis is stiffer than c axis within 0~100 GPa. Elastic constants calculations predict…

Mesoscale and Nanoscale Physics · Physics 2017-09-26 Qinghe Gao , Zhijun Xu , Ling Tang , Xianjun Zuo , Guozhu Jia , An Du , Rongfeng Linghu , Yundong Guo , Zejin Yang

The elastic properties and lattice dynamics of Ti$_2$AlC, Ti$_2$AlN, Ti$_2$GaC, Ti$_2$GaN, Ti$_2$PbC, Ti$_2$CdC and Ti$_2$SnC have been investigated using the density functional theory within the generalized gradient approximations as…

Materials Science · Physics 2020-11-17 G. K. Arusei , M. Chepkoech , G. O. Amolo , N. Wambua

Using first-principal density functional theory (DFT) we explained the importance of pseudopotential for decribing the electronic and vibrational properties of rutile TiO2 (R-TiO2). Calculations were performed using the generalized gradient…

Chemical Physics · Physics 2018-11-12 Sugata Chowdhury , Nacole King , Winnie Wong-Ng

While the vibrational thermodynamics of materials with small anharmonicity at low temperatures has been understood well based on the harmonic phonons approximation; at high temperatures, this understanding must accommodate how phonons…

Materials Science · Physics 2015-10-20 Tian Lan

Density functional perturbation theory calculations of alpha-quartz using extended norm conserving pseudopotentials have been used to study the elastic properties and phonon dispersion relations along various high symmetry directions as a…

Materials Science · Physics 2007-05-23 N. Choudhury , S. L. Chaplot

We have investigated the finite temperature elastic properties of AlRE (RE=Y, Tb, Pr, Nd, Dy) with B2-type structures from first principles. The phonon free energy and thermal expansion is obtained from the quasiharmonic approach based on…

Materials Science · Physics 2011-11-08 Rui Wang , Shaofeng Wang , Xiaozhi Wu

The structural, electronic, mechanic, vibrational and thermodynamic properties of Ti2SiB which is a hypothetical MAX phase compound, have been investigated using density functional theory calculations. The structural optimization of Ti2SiB…

Materials Science · Physics 2018-05-15 Aysenur Gencer , Gokhan Surucu

We investigate the lattice dynamics and thermodynamics of nonmagnetic bcc vanadium as a function of temperature and pressure, using the first principles linear response linear-muffin-tin-orbital method. The calculated phonon density of…

Materials Science · Physics 2007-05-23 Xianwei Sha , R. E. Cohen

Structural and elastic properties of Ba$_{2}$P$_{7}$X (X=Cl, Br, I) (Barium Phosphide Halides) Zintl compounds have been investigated using the pseudo-potential plane-wave (PP-PW) method based on the density functional theory (DFT) within…

Materials Science · Physics 2019-10-03 M. Radjai , D. Maouche , N. Guechi , S. Cheddadi , Z. Kechidi

The wide band gap semiconductor \b{eta}-Ga2O3 shows promise for applications in high-power and high-temperature electronics. The phonons of \b{eta}-Ga2O3 play a crucial role in determining its important material characteristics for these…

Materials Science · Physics 2019-02-08 K. A. Mengle , E. Kioupakis