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Recently proposed non-adiabatic ring polymer molecular dynamics (NRPMD) approach has shown to provide accurate quantum dynamics by incorporating explicit electronic state descriptions and nuclear quantizations. Here, we present a rigorous…

Chemical Physics · Physics 2019-07-24 Sutirtha N. Chowdhury , Pengfei Huo

We study the real-time dynamics of quantum models with long-range interactions coupled to a heat-bath within the closed-time path-integral formalism. We show that quantum fluctuations depress the transition temperature. In the subcritical…

Condensed Matter · Physics 2009-10-30 Leticia F. Cugliandolo , Gustavo Lozano

Accurately modeling gas-surface collision dynamics presents a great challenge for theory, especially in the low energy (or temperature) regime where quantum effects are important. Here, a path integral based non-equilibrium ring polymer…

Chemical Physics · Physics 2019-12-06 Qinghua Liu , Liang Zhang , Yongle Li , Bin Jiang

The quantum harmonic oscillator is the fundamental building block to compute thermal properties of virtually any dielectric crystal at low temperatures in terms of phonons, extended further to cases with anharmonic couplings, or even…

Statistical Mechanics · Physics 2021-10-05 Vladislav Efremkin , Jean-Louis Barrat , Stefano Mossa , Markus Holzmann

Molecular dynamics with electronic friction (MDEF) approach can describe nonadiabatic effects accurately at metal surfaces in the weak nonadiabatic limit. That being said, MDEF treats nuclear motion classically, such that the nuclear…

Chemical Physics · Physics 2024-04-09 Rui-Hao Bi , Wenjie Dou

We initiate the study of utilizing Quantum Langevin Dynamics (QLD) to solve optimization problems, particularly those non-convex objective functions that present substantial obstacles for traditional gradient descent algorithms.…

Quantum Physics · Physics 2025-03-11 Zherui Chen , Yuchen Lu , Hao Wang , Yizhou Liu , Tongyang Li

We demonstrate a new method of simulation of nonstationary quantum processes, considering the tunneling of two {\it interacting identical particles}, represented by wave packets. The used method of quantum molecular dynamics (WMD) is based…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 Yu. E. Lozovik , A. V. Filinov , A. S. Arkhipov

The interaction of condensed phase systems with external electric fields is crucial in myriad processes in nature and technology ranging from the field-directed motion of cells (galvanotaxis), to energy storage and conversion systems…

Chemical Physics · Physics 2024-09-25 Kit Joll , Philipp Schienbein , Kevin M. Rosso , Jochen Blumberger

Quantum nuclear dynamics with wavepacket time-evolution is classically intractable and viewed as a promising avenue for quantum information processing. Here, we use an IonQ 11-qubit trapped-ion quantum computer, Harmony, to study the…

Quantum Physics · Physics 2024-12-05 Anurag Dwivedi , A. J. Rasmusson , Philip Richerme , Srinivasan S. Iyengar

Photonic Quantum Machine Learning (PQML) is an emerging method to implement scalable, energy-efficient quantum information processing by combining photonic quantum computing technologies with machine learning techniques. The features of…

Quantum Physics · Physics 2026-04-07 A. M. A. S. D. Alagiyawanna , Asoka Karunananda

A wide variety of dissipative and fluctuation problems involving a quantum system in a heat bath can be described by the independent-oscillator (IO) model Hamiltonian. Using Heisenberg equations of motion, this leads to a generalized…

Quantum Physics · Physics 2009-11-11 R. F. O'Connell

Both nonzero temperature and chemical potentials break the Lorentz symmetry present in vacuum quantum field theory by singling out the rest frame of the heat bath. This leads to complications in the application of thermal perturbation…

High Energy Physics - Phenomenology · Physics 2023-09-11 Juuso Österman , Philipp Schicho , Aleksi Vuorinen

We show that treating the blackbody radiation field as a heat bath enables one to utilize powerful techniques from the realm of stochastic physics (such as the fluctuation-dissipation theorem and the related radiation damping) in order to…

Quantum Physics · Physics 2010-09-23 R. F. O'Connell

Effects of nuclear dynamics on the energetics of polythiophene relevant for the performance of organic solar cells are studied for the first time. Nuclear motions change the expectation values of frontier orbital energies and the band gap…

Chemical Physics · Physics 2016-02-05 Sergei Manzhos

In this paper, a hybrid quasi-static atomistic simulation method at finite temperature is developed, which combines the advantages of MD for thermal equilibrium and atomic-scale finite element method (AFEM) for efficient equilibration. Some…

Atomic Physics · Physics 2015-06-17 Ran Xu , Bin Liu

Due to the wide range of technical applications of actinide elements, a thorough understanding of their electronic structure could complement technological improvements in many different areas. Quantum computing could greatly aid in this…

Recent developments in path integral methodology have significantly reduced the computational expense of including quantum mechanical effects in the nuclear motion in ab initio molecular dynamics simulations. However, the implementation of…

Computational Physics · Physics 2014-02-06 Michele Ceriotti , Joshua More , David E. Manolopoulos

Using a generalized Langevin equation of motion, quantum ballistic thermal transport is obtained from classical molecular dynamics. This is possible because the heat baths are represented by random noises obeying quantum Bose-Einstein…

Statistical Mechanics · Physics 2007-10-16 Jian-Sheng Wang

We review a molecular dynamics method for nucleon many-body systems called the quantum molecular dynamics (QMD) and our studies using this method. These studies address the structure and the dynamics of nuclear matter relevant to the…

Nuclear Theory · Physics 2014-01-31 Toshiki Maruyama , Gentaro Watanabe , Satoshi Chiba

In our recent work [H. Zhang, F.X. Trias, A. Oliva, D. Yang, Y. Tan, Y. Sheng. PIBM: Particulate immersed boundary method for fluid-particle interaction problems. Powder Technology. 272(2015), 1-13.], a particulate immersed boundary method…

Computational Physics · Physics 2015-02-05 Hao Zhang , Haizhuan Yuan , F. Xavier Trias , Aibing Yu , Yuanqiang Tan , Assensi Oliva
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