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We report ultrafast surface pump and interface probe experiments on photoexcited carrier transport across single crystal bismuth films on sapphire. The film thickness is sufficient to separate carrier dynamics from lattice heating and…

Materials Science · Physics 2013-03-21 Y. M. Sheu , Y. J. Chien , C. Uher , S. Fahy , D. A. Reis

We study, by means of a Monte Carlo simulator, the hot phonon effect on the relaxation dynamics in photoexcited graphene and its quantitative impact as compared to considering an equilibrium phonon distribution. Our multi-particle approach…

Mesoscale and Nanoscale Physics · Physics 2016-02-02 José M. Iglesias , María J. Martín , Elena Pascual , Raúl Rengel

We perform a femtosecond-THz optical pump-probe spectroscopy to investigate the cooling dynamics of hot carriers in quasi-free standing bilayer epitaxial graphene. We observed longer decay time constants, in the range of 2.6 to 6.4 ps,…

Mesoscale and Nanoscale Physics · Physics 2023-02-03 Sachin Sharma , Rachael L. Myers-Ward , David Kurt Gaskill , Ioannis Chatzakis

We report ultrafast response of femtosecond photoexcited carriers in single layer reduced graphene oxide flakes suspended in water as well as few layer thick film deposited on indium tin oxide coated glass plate using pump-probe…

Materials Science · Physics 2011-06-30 Sunil Kumar , N. Kamaraju , K. S. Vasu , A. K. Sood

The coherent oscillations of mobile charge carriers near the surface of good conductors-surface plasmons-are been exploited in many applications in information technologies, clean energy, high-density data storage, photovoltaics, chemistry,…

Mesoscale and Nanoscale Physics · Physics 2023-12-20 Jacob Khurgin , Anton Yu. Bykov , Anatoly V. Zayats

Infrared pump-probe spectroscopy provides detailed information on the dynamics of hydrogen-bonded liquids. Due to dissipation of the absorbed pump pulse energy, also thermal equilibration dynamics contributes to the observed signal.…

Chemical Physics · Physics 2019-06-05 Riccardo Dettori , Michele Ceriotti , Johannes Hunger , Luciano Colombo , Davide Donadio

We report on time-resolved optical and terahertz ultrafast spectroscopy of charge-carrier dynamics in the room-temperature antiferromagnetic semiconductor $\alpha $-MnTe. By optically pumping the system with 1.55 eV photons at room…

We report on time-resolved mid-infrared-pump terahertz-transmission-probe studies of the topological-insulator materials $(Bi_{1-x}Sb_{x})_{2}Te_{3}$, in which by varying x charge carriers are chemically tuned to be of n-type or p-type.…

We report femtosecond time-resolved reflectivity measurements of coherent phonons in tellurium performed over a wide range of temperatures (3K to 296K) and pump laser intensities. A totally symmetric A$_{1}$ coherent phonon at 3.6 THz…

Materials Science · Physics 2015-05-20 N. Kamaraju , Sunil Kumar , M. Anija , A. K. Sood

Plasma accelerators utilize strong electric fields in plasma waves to accelerate charged particles, making them a compact alternative to radiofrequency technologies. Discharge capillaries are plasma sources used in plasma accelerator…

We report on the temporal lasing dynamics of high quality ZnO nanowires using time-resolved micro-photoluminescence technique. The temperature dependence of the lasing characteristics and of the corresponding decay constants demonstrate the…

We present detailed theoretical calculations of two color, time-resolved pump-probe differential reflectivity measurements. The experiments modeled were performed on InMnAs/GaSb heterostructures and showed pronounced oscillations in the…

Statistical Mechanics · Physics 2009-11-11 G. D. Sanders , C. J. Stanton , J. Wang , J. Kono , A. Oiwa , H. Munekata

We analyze ultrafast electron dynamics in the time domain upon optical excitation of propagating surface plasmon-polaritons (SPs) in metal-dielectric heterostructures. Developing a kinetic model where both local and non-local electron…

Mesoscale and Nanoscale Physics · Physics 2019-07-24 Ilya Razdolski , Alexander L. Chekhov , Alexander I. Stognij , Andrzej Stupakiewicz

The fast decay of carrier inversion in photoexcited graphene has been attributed to optical phonon emission and Auger recombination. Plasmon emission provides another pathway that, as we show here, drives the carrier relaxation dynamics on…

Mesoscale and Nanoscale Physics · Physics 2016-01-20 J. M. Hamm , A. F. Page , J. Bravo-Abad , F. J. Garcia-Vidal , O. Hess

Using ultrafast optical pump-probe spectroscopy, we study the relaxation dynamics of hot optical phonons in few-layer and multi-layer graphene films grown by epitaxy on silicon carbide substrates and by chemical vapor deposition on nickel…

We demonstrate that in confined plasmonic metal structures subject to ultra-fast laser excitation electron thermal diffusion can provide relaxation faster than the energy transfer to the lattice. This relaxation occurs due to excitation of…

Room temperature, wavelength non-degenerate ultrafast pump/probe measurements were performed on GaN and InGaN epilayers and an InGaN multiple quantum well structure. Carrier relaxation dynamics were investigated as a function of excitation…

Mesoscale and Nanoscale Physics · Physics 2015-06-24 Umit Ozgur , Henry O. Everitt

The dynamics of weakly magnetized collisionless plasmas in the presence of an imposed temperature gradient along an ambient magnetic field is explored with particle-in-cell simulations and modeling. Two thermal reservoirs at different…

High Energy Astrophysical Phenomena · Physics 2018-01-22 G. T. Roberg-Clark , J. F. Drake , C. S. Reynolds , M. Swisdak

Recent studies have established that the anti-Stokes Raman signal from plasmonic metal nanostructures can be used to determine the two separate temperatures that characterize carriers inside the metal -- the temperature of photoexcited "hot…

The first femtosecond carrier relaxation dynamics studies in heavy fermion compounds are presented. The carrier relaxation time shows a dramatic hundred-fold increase below the Kondo temperature revealing a dramatic sensitivity to the…

Strongly Correlated Electrons · Physics 2007-05-23 J. Demsar , L. A. Tracy , R. D. Averitt , S. A. Trugman , J. L. Sarrao , A. J. Taylor