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The coherence of two, coupled two-level systems, representing vibrational modes in a semiclassical model, is calculated in weak and strong fields for various coupling schemes and for different relative phases between initial state…

Chemical Physics · Physics 2009-11-10 S. A. Malinovskaya , P. H. Bucksbaum , P. R. Berman

We study and experimentally implement a double-slit quantum eraser in the presence of a controlled decoherence mechanism. A two-photon state, produced in a spontaneous parametric down conversion process, is prepared in a maximally entangled…

Quantum Physics · Physics 2015-05-14 F. A. Torres-Ruiz , G. Lima , A. Delgado , S. Pádua , C. Saavedra

We optically probe the spectrum of ground and excited state transitions of an individual, electrically tunable self-assembled quantum dot molecule. Photocurrent absorption measurements show that the spatially direct neutral exciton…

Mesoscale and Nanoscale Physics · Physics 2011-11-15 K. Müller , G. Reithmaier , E. C. Clark , V. Jovanov , M. Bichler , H. J. Krenner , M. Betz , G. Abstreiter , J. J. Finley

The cause of decoherence in a quantum system can be traced back to the interaction with the environment. As it has been pointed out first by Dicke, in a system of N two-level atoms where each of the atoms is individually dipole coupled to…

Quantum Physics · Physics 2009-11-07 Peter Foldi , Mihaly G. Benedict , Attila Czirjak

Multidimensional coherent optical spectroscopy is one of the most powerful tools for investigating complex quantum mechanical systems. While it was conceived decades ago in magnetic resonance spectroscopy using micro- and radio-waves, it…

We find that two-color fields can induce field-free permanent dipoles in initially isotropic samples of chiral molecules via resonant electronic excitation in a one-$3\omega$-photon vs. three-$\omega$-photons scheme. These permanent dipoles…

Atomic Physics · Physics 2021-08-04 Andres F. Ordonez , Olga Smirnova

Ultrafast pump-probe technique is a powerful tool to understand and manipulate properties of materials for designing novel quantum devices. An intense, single cycle terahertz pulse can change the intrinsic properties of semiconductor…

Mesoscale and Nanoscale Physics · Physics 2020-07-13 Chen-Yen Lai , D. A. Yarotski , Jian-Xin Zhu

In wide-field nonlinear microscopy, wavefront modulation by means of phase-only spatial light modulators (SLMs) allows achieving simultaneous two-photon excitation and fluorescence emission from specific region-of-interests (ROIs) of…

Photonic quantum computing offers a promising platform for quantum information processing, benefiting from the long coherence times of photons and their ease of manipulation. This paper presents a scheme for implementing a deterministic…

Quantum Physics · Physics 2025-04-22 Evangelos Varvelis , Joachim Ankerhold

In this paper, single-molecule spectroscopy experiments based on continuous laser excitation are characterized through an open quantum system approach. The evolution of the fluorophore system follows from an effective Hamiltonian…

Quantum Physics · Physics 2009-04-09 Adrian A. Budini

Coherent manipulation of quantum states of light is key to photonic quantum information processing. In this Letter, we show that a passive two-level nonlinearity suffices to implement non-Gaussian quantum operations on propagating field…

Quantum Physics · Physics 2024-09-06 Mads M. Lund , Fan Yang , Victor Rueskov Christiansen , Danil Kornovan , Klaus Mølmer

Well controlled nonlinear interactions between light field pulses and single atoms could be used to implement optical quantum information technologies based on qubits encoded in superpositions of coherent states of light. Here, we…

Quantum Physics · Physics 2014-07-28 Akihiro Yamaguchi , Holger F. Hofmann

We present a pulsed and integrated, highly non-degenerate parametric downconversion (PDC) source of heralded single photons at telecom wavelengths, paired with heralding photons around 800 nm. The active PDC section is combined with a…

A two-level quantum system can absorb or emit not more than one photon at a time. Using this fundamental property, we demonstrate how a superconducting quantum system strongly coupled to a transmission line can be used as a sensor of the…

Quantum Physics · Physics 2020-03-04 T. Hönigl-Decrinis , R. Shaikhaidarov , S. E. de Graaf , V. N. Antonov , O. V. Astafiev

We introduce a simple model for electromagnetically induced transparency in which all fields are treated quantum mechanically. We study a system of three separated atoms at fixed positions in a one-dimensional multimode optical cavity. The…

Quantum Physics · Physics 2018-05-09 Thomas Purdy , Martin Ligare

Within optical quantum information processing, single-photon sources based on a two-level system in a semiconductor material allow for on-demand generation of single photons. To initiate the spontaneous emission process, it is necessary to…

Semiconductor quantum dots embedded in optical cavities are promising on-demand sources of single photons. Here, we theoretically study single photon emission from an optically driven two-photon Raman transition between the biexciton and…

The ability to tailor laser light on a chip using integrated photonics has allowed for extensive control over fundamental light-matter interactions in manifold quantum systems including atoms, trapped ions, quantum dots, and defect centers.…

We describe a high-resolution spectroscopy method, in which the detection of single excitation events is enhanced by a complete loss of coherence of a superposition of two ground states. Thereby, transitions of a single isolated atom nearly…

Atomic Physics · Physics 2014-03-25 Govinda Clos , Martin Enderlein , Ulrich Warring , Dietrich Leibfried , Tobias Schaetz

We describe the interaction of two two-level atoms in free space with propagating modes of the quantized electromagnetic field, using the time-dependent Heisenberg-Langevin method. For single- photon pulses, we consider the effect of the…

Quantum Physics · Physics 2014-11-14 Navneeth Ramakrishnan , Yimin Wang , Valerio Scarani