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In this article, we consider quantum crystals with defects in the reduced Hartree-Fock framework. The nuclei are supposed to be classical particles arranged around a reference periodic configuration. The perturbation is assumed to be small…

Mathematical Physics · Physics 2018-03-28 Salma Lahbabi

Existence of minimizers for the Dirac--Fock model in crystals was recently proved by Paturel and S\'er\'e and the authors \cite{crystals} by a retraction technique due to S\'er\'e \cite{Ser09}. In this paper, inspired by Ghimenti and…

Analysis of PDEs · Mathematics 2023-07-19 Isabelle Catto , Long Meng

This article is concerned with the derivation and the mathematical study of a new mean-field model for the description of interacting electrons in crystals with local defects. We work with a reduced Hartree-Fock model, obtained from the…

Mathematical Physics · Physics 2009-02-06 Eric Cancès , Amélie Deleurence , Mathieu Lewin

We study the periodic Hartree-Fock model used for the description of electrons in a crystal. The existence of a minimizer was previously shown by Catto, Le Bris and Lions (Ann. Inst. H. Poincare Anal. Non Lineaire} 18 (2001), no.6,…

Mathematical Physics · Physics 2008-12-18 Marco Ghimenti , Mathieu Lewin

In this article, we set up a functional setting for mean-field electronic structure models of Hartree-Fock or Kohn-Sham types for disordered crystals. The electrons are quantum particles and the nuclei are classical point-like articles…

Mathematical Physics · Physics 2013-12-11 Eric Cancès , Salma Lahbabi , Mathieu Lewin

We study the Hartree-Fock model for pseudorelativistic atoms, that is, atoms where the kinetic energy of the electrons is given by the pseudorelativistic operator \sqrt{(pc)^2+(mc^2)^2}-mc^2. We prove the existence of a Hartree-Fock…

Mathematical Physics · Physics 2013-10-30 Anna Dall'Acqua , Thomas Østergaard Sørensen , Edgardo Stockmeyer

This paper is devoted to the Hartree-Fock model with temperature in the euclidean space. For large classes of free energy functionals, minimizers are obtained as long as the total charge of the system does not exceed a threshold which…

Analysis of PDEs · Mathematics 2009-04-01 Jean Dolbeault , Patricio Felmer , Mathieu Lewin

We study the Hartree-Fock equation and the Hartree-Fock energy functional universally used in many-electron problems. We prove that the set of all critical values of the Hartree-Fock energy functional less than a constant smaller than the…

Mathematical Physics · Physics 2021-10-07 Sohei Ashida

For neutral and positively charged atoms and molecules, we prove the existence of infinitely many Hartree-Fock critical points below the first energy threshold (that is, the lowest energy of the same system with one electron removed). This…

Mathematical Physics · Physics 2017-11-22 Mathieu Lewin

In this note we establish the existence of ground states for atoms within several restricted Hartree-Fock theories. It is shown, for example, that there exists a ground state for closed shell atoms with $N$ electrons and nuclear charge $Z…

Mathematical Physics · Physics 2012-06-22 Fabian Hantsch

We prove within the Hartree-Fock theory of pseudo-relativistic atoms that the maximal negative ionization charge and the ionization energy of an atom remain bounded independently of the nuclear charge Z and the fine structure constant…

Mathematical Physics · Physics 2010-11-12 Anna Dall'Acqua , Jan Philip Solovej

The familiar unrestricted Hartree-Fock variational principle is generalized to include quasi-free states. As we show, these are in one-to-one correspondence with the one-particle density matrices and these, in turn provide a convenient…

Condensed Matter · Physics 2009-10-22 Volker Bach , Elliott H. Lieb , Jan philip Solovej

Automatic differentiation has become an important tool for optimization problems in computational science, and it has been applied to the Hartree-Fock method. Although the reverse-mode automatic differentiation is more efficient than the…

Chemical Physics · Physics 2022-11-28 Naruki Yoshikawa , Masato Sumita

We prove the existence of solutions of the reduced Hartree-Fock equations at finite temperature for a periodic crystal with a small defect, and show total screening of the defect charge by the electrons. We also show the convergence of the…

Mathematical Physics · Physics 2020-07-28 Antoine Levitt

We investigate the ground states of neutron stars and white dwarfs in the Hartree-Fock (HF) and Hartree-Fock-Bogoliubov (HFB) theories. It is known that the system is stable below a critical mass, which depends on the gravitational…

Analysis of PDEs · Mathematics 2025-09-26 Bin Chen , Yujin Guo , Phan Thành Nam , Dong Hao Ou Yang

A uniform derivation is presented of the self-consistent field equations in a finite basis set. Both restricted and unrestricted Hartree-Fock (HF) theory as well as various density functional (DF) approximations are considered. The unitary…

Computational Physics · Physics 2020-03-10 Susi Lehtola , Frank Blockhuys , Christian Van Alsenoy

In a recent article (Canc\`es, Deleurence and Lewin, Commun. Math. Phys., 281 (2008), pp. 129-177), we have rigorously derived, by means of bulk limit arguments, a new variational model to describe the electronic ground state of insulating…

Mathematical Physics · Physics 2015-05-13 Eric Cancès , Mathieu Lewin

Whereas many different models exist in the mathematical and physics literature for ground states of non-relativistic crystals, the relativistic case has been much less studied and we are not aware of any mathematical result on a fully…

Analysis of PDEs · Mathematics 2024-06-27 Isabelle Catto , Long Meng , Eric Paturel , Eric Séré

The Hartree-Fock equation admits homogeneous states that model infinitely many particles at equilibrium. We prove their asymptotic stability in large dimensions, under assumptions on the linearised operator. Perturbations are moreover…

Analysis of PDEs · Mathematics 2025-02-26 Charles Collot , Elena Danesi , Anne-Sophie de Suzzoni , Cyril Malézé

As a contribution to the study of Hartree-Fock theory we prove rigorously that the Hartree-Fock approximation to the ground state of the d-dimensional Hubbard model leads to saturated ferromagnetism when the particle density (more…

Strongly Correlated Electrons · Physics 2007-05-23 Volker Bach , Elliott H. Lieb , Marcos V. Travaglia
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