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The generation of harmonics by atoms or ions in a two-color, coplanar field configuration with commensurate frequencies is investigated through both, an analytical calculation based on the Lewenstein model and the numerical ab initio…

Atomic Physics · Physics 2009-11-07 F. Ceccherini , D. Bauer , F. Cornolti

We present a generic approach for treating the effect of nuclear motion in the high-order harmonic generation from polyatomic molecules. Our procedure relies on a separation of nuclear and electron dynamics where we account for the…

Atomic Physics · Physics 2010-04-21 C. B. Madsen , M. Abu-samha , L. B. Madsen

We present a semiclassical model for plasmon-enhanced high-harmonic generation (HHG) in the vicinity of metal nanostructures. We show that both the inhomogeneity of the enhanced local fields and electron absorption by the metal surface play…

Optics · Physics 2015-07-29 A. Husakou , S. -J. Im , J. Herrmann

High-harmonic generation (HHG) in condensed-matter systems is both a source of fundamental insight into quantum electron motion and a promising candidate to realize compact ultraviolet and ultrafast light sources. Here we argue that the…

Mesoscale and Nanoscale Physics · Physics 2017-03-08 Joel D. Cox , Andrea Marini , F. Javier García de Abajo

Collinear double-pulse seeding of the High-Gain Harmonic Generation (HGHG) process in a free-electron laser (FEL) is a promising approach to facilitate various coherent nonlinear spectroscopy schemes in the extreme ultraviolet (XUV)…

Recent breakthroughs in high repetition-rate extreme ultraviolet (XUV) light sources and photoelectron analyzers have led to dramatic advances in the performance of time-resolved photoemission experiments. In this perspective article, we…

Optics · Physics 2024-10-16 Thomas K. Allison , Alice Kunin , Gerd Schönhense

The order of high harmonics emitted by an atom in an intense laser field is limited by the so-called cutoff frequency. Solving the time-dependent Schr\"odinger equation, we show that this frequency can be increased considerably by a…

Atomic Physics · Physics 2016-09-08 Carla Figueira de Morisson Faria , Jan-Michael Rost

We analyze the spectral properties of high-order harmonic radiation with photon energies extending beyond the regular cutoff energy in standard high-order harmonic generation. The extension of the regular harmonic cutoff results from…

Atomic Physics · Physics 2026-01-30 R. Esteban Goetz , Anh-Thu Le

The interaction of relativistically strong tailored laser pulses with an atomic system is considered. Due to a special tailoring of the laser pulse, the suppression of the relativistic drift of the ionized electron and a dramatic…

Atomic Physics · Physics 2007-05-23 M. Klaiber , K. Z. Hatsagortsyan , C. H. Keitel

The selection rules of high harmonic generation (HHG) are investigated using three-dimensional time-dependent density functional theory (TDDFT). From the harmonic spectra obtained with various real molecules and different forms of laser…

Atomic Physics · Physics 2016-09-28 Xi Liu , Xiaosong Zhu , Liang Li , Yang Li , Qingbin Zhang , Pengfei Lan , Peixiang Lu

High-harmonic generation (HHG) in crystalline solids have been examined so far on the basis of one-body energy-band structures arising from electron itineracy in a periodic potential. Here, we show emergence of HHG signals which are…

Strongly Correlated Electrons · Physics 2020-04-22 Shohei Imai , Atsushi Ono , Sumio Ishihara

High-harmonic generation (HHG), which is generation of multiple optical harmonic light, is an unconventional nonlinear optical phenomenon beyond perturbation regime. HHG, which was initially observed in gaseous media, has recently been…

The generation of high-order harmonics in bulk solids subjected to intense ultrashort laser pulses has opened up new avenues for research in extreme nonlinear optics and light-matter interaction on sub-cycle timescales. Despite significant…

High-harmonic generation (HHG) in solids is an emerging method to probe ultrafast electron dynamics in solids at attosecond timescale. In this work, we study HHG from monolayer and bilayer graphene. Bilayer graphenes with AA and AB stacking…

Optics · Physics 2021-03-26 M. S. Mrudul , Gopal Dixit

We theoretically investigate high-harmonic generation (HHG) in honeycomb-lattice graphene models when subjected to a DC electric field. By integrating the quantum master equation with the Boltzmann equation, we develop a numerical method to…

Mesoscale and Nanoscale Physics · Physics 2024-07-16 Minoru Kanega , Masahiro Sato

High-harmonic generation (HHG) is a coherent optical process in which the incident photon energy is up-converted to the multiples of its initial energy. In solids, under the influence of a strong laser field, electron-hole (e-h) pairs are…

A manifestation of electron-hole pairing in nonlinear electromagnetic response of a double layer graphene system is studied. It is shown that the pairing causes the appearance of a number of peaks in the frequency dependence of the…

Strongly Correlated Electrons · Physics 2017-10-20 K. V. Germash , D. V. Fil

High-harmonic generation (HHG) normally requires a careful adjustment of the driving laser intensity (typically $10^{14} - 10^{15}$ W/cm$^2$) and gas medium parameters to enable good phase matching conditions. In contrast with conventional…

We observe a new regime of coherent XUV radiation generation in noble gases induced by femtosecond pulses at very high intensities. This XUV emission has both a reduced divergence and spectral width as compared to high-order harmonic…

High-order sideband generation (HSG), as an analogue of the interband processes in high-harmonic generation (HHG) in solids, is a nonperturbative nonlinear optical phenomenon in semiconductors that are simultaneously driven by a relatively…

Optics · Physics 2023-05-31 Qile Wu , Mark S. Sherwin