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Nanostars (NSTs) are spiky nanocrystals with plasmonic hot spots. In this study, we show that strong electromagnetic fields localized in the nanostar tips are able to generate large numbers of energetic (hot) electrons, which can be used…

Mesoscale and Nanoscale Physics · Physics 2016-12-20 Xiang-Tian Kong , Zhiming Wang , Alexander O. Govorov

Quantum emitters in solid-state crystals have recently attracted a lot of attention due to their simple applicability in optical quantum technologies. The polarization of single photons generated by quantum emitters is one of the key…

Energetic and optical properties of plasmonic nanocrystals strongly depend on their sizes, shapes, and composition. Whereas using plasmonic nanoparticles in biotesting has become routine, applications of plasmonics in energy are still early…

We provide the quantum mechanical description of the excitation of surface plasmon polaritons on metal surfaces by single-photons. An attenuated-reflection setup is described for the quantum excitation process in which we find remarkably…

Quantum Physics · Physics 2009-11-13 M. S. Tame , C. Lee , J. Lee , D. Ballester , M. Paternostro , A. V. Zayats , M. S. Kim

We propose a novel scheme of photon upconversion based on harnessing the energy of plasmonic hot carriers. Low-energy photons excite hot electrons and hot holes in a plasmonic nanoparticle, which are then injected into an adjacent…

Optics · Physics 2015-11-17 Gururaj V. Naik , Jennifer A. Dionne

We present a quantum-mechanical model for surface-assisted carrier excitation by optical fields in plasmonic nanostructures of arbitrary shape. We derive an explicit expression, in terms of local fields inside the metal structure, for…

Mesoscale and Nanoscale Physics · Physics 2019-04-15 Tigran V. Shahbazyan

It has been known for many years that metallic nanoparticles can catalyse various chemical reactions, both in the dark and under illumination, through different mechanisms. In the last decade or so, many claims of plasmon-assisted "hot"…

Optics · Physics 2020-11-13 Yonatan Sivan , Yonatan Dubi

Molecular aggregates on plasmonic nanoparticles have emerged as attractive systems for the studies of cavity quantum electrodynamics. They are highly tunable, scalable, easy to synthesize and offer sub-wavelength confinement, all while…

Harvesting non-equilibrium hot carriers from photo-excited metal nanoparticles has enabled plasmon-driven photochemical transformations and tunable photodetection with resonant nanoantennas. Despite numerous studies on the ultrafast…

Herein we report on our studies of radiative and non-radiative interaction between an individual quantum emitter and an anisotropic plasmonic nanostructure: a gold nanotriangle. Our theoretical and three-dimensional electromagnetic…

Optics · Physics 2018-06-18 Adarsh B. Vasista , G. V. Pavan Kumar

Strong coupling between plasmons and excitons gives rise to new hybrid polariton states with various fields of potential applications. Despite a plethora of research on plasmon--exciton systems, their transient behaviour is not yet fully…

Optics · Physics 2023-06-13 Felix Stete , Matias Bargheer , Wouter Koopman

Highly integrated single photon sources are key components in future quantum-optical circuits. Whereas the probabilistic generation of single photons can routinely be done by now, their triggered generation is a much greater challenge.…

Quantum Physics · Physics 2016-05-25 Jako Straubel , Robert Filter , Carsten Rockstuhl , Karolina Słowik

We investigate theoretically the formation of collective excitations in atomic scale quasi-one dimensional metallic nanostructures. The response of the system is calculated within the linear response theory and random phase approximation.…

Mesoscale and Nanoscale Physics · Physics 2008-04-17 Amy Cassidy , Ilya Grigorenko , Stephan Haas

Recent experiments claimed that the enhancement of catalytic reaction rates occurs via the reduction of activation barriers driven by non-equilibrium (``hot'') electrons in plasmonic metal nanoparticles. These experiments place plasmonic…

Chemical Physics · Physics 2020-04-22 Yonatan Sivan , Ieng Wai Un , Yonatan Dubi

We describe a technique that enables strong, coherent coupling between individual optical emitters and guided plasmon excitations in conducting nano-structures at optical frequencies. We show that under realistic conditions, optical…

Quantum Physics · Physics 2009-11-11 D. E. Chang , A. S. Sorensen , P. R. Hemmer , M. D. Lukin

Luminescence constitutes a unique source of insight into hot carrier processes in metals, including those in plasmonic nanostructures used for sensing and energy applications. However, being weak in nature, metal luminescence remains poorly…

We develop a general quantum theory of the coupled plasmonic modes resulting from the near-field interaction between localized surface plasmons in a heterogeneous metallic nanoparticle dimer. In particular, we provide analytical expressions…

Mesoscale and Nanoscale Physics · Physics 2016-03-02 Adam Brandstetter-Kunc , Guillaume Weick , Dietmar Weinmann , Rodolfo A. Jalabert

Plasmonic excitations decay within femtoseconds, leaving non-thermal (often referred to as "hot") charge carriers behind that can be injected into molecular structures to trigger chemical reactions that are otherwise out of reach -- a…

Materials Science · Physics 2025-01-28 Jakub Fojt , Paul Erhart , Christian Schäfer

We theoretically investigate equilibrium behaviors and photothermal effects of a flexible plasmonic metamaterial composed of aramid nanofibers and gold nanoparticles. The fiber matrix is considered as an external field to reconfigure a…

Mesoscale and Nanoscale Physics · Physics 2020-11-12 Anh D. Phan , Vu D. Lam , Katsunori Wakabayashi

Surface plasmon polaritons (plasmons) have the potential to interface electronic and optical devices. They could prove extremely useful for integrated quantum information processing. Here we demonstrate on-chip electrical detection of…

Mesoscale and Nanoscale Physics · Physics 2010-01-18 Reinier W. Heeres , Sander N. Dorenbos , Benny Koene , Glenn S. Solomon , Leo P. Kouwenhoven , Valery Zwiller