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The rapidly developing and converging fields of polaritonic chemistry and quantum optics necessitate a unified approach to predict strongly-correlated light-matter interactions with atomic-scale resolution. Combining concepts from both…

Quantum Physics · Physics 2018-09-19 Johannes Flick , Prineha Narang

Polaritonic chemistry offers the possibility of modifying molecular properties and even influencing chemical reactivity through strong coupling between vibrational transitions and confined light modes in optical cavities. Despite…

Chemical Physics · Physics 2025-05-16 Thomas Schnappinger , Markus Kowalewski

We present a rigorous photonic mode model to describe the strong coupling between a monolayer of $\rm MoSe_2$ and a single gold nanoparticle. The onset of strong coupling is quantified by computing the three-dimensional hybrid quasinormal…

Localized plasmonic modes of metallic nanoparticles may hybridize like those of atoms forming a molecule. However, the rapid decay of the plasmonic fields outside the metal severely limits the range of these interactions to tens of…

Optics · Physics 2013-03-05 Adi Salomon , Yehiam Prior , Radoslaw Kolkowski , Joseph Zyss

We introduce crystal polaritons, hybrid excitations formed when the collective excitations of a periodic quantum-emitter array strongly couple to the resonant Bloch modes of a metasurface. This realizes a cavity-QED platform in which…

Two dimensional (2D) atomic crystals of graphene, and transition metal dichalcogenides have emerged as a class of materials that show strong light-matter interaction. This interaction can be further controlled by embedding such materials…

Intermixed light-matter quasiparticles - polaritons - possess unique optical properties owned to their compositional nature. These intriguing hybrid states have been extensively studied over the past decades in a wide range of realizations…

When the interaction between a molecular system and confined light modes in an optical or plasmonic cavity is strong enough to overcome the dissipative process, hybrid light-matter states (polaritons) become the fundamental excitations in…

Mesoscale and Nanoscale Physics · Physics 2020-01-08 Yu Zhang , Tammie Nelson , Sergei Tretiak

Vibrational strong coupling is emerging as a promising tool to modify molecular properties, by making use of hybrid light-matter states known as polaritons. Fabry-Perot cavities filled with organic molecules are typically used, and the…

Magnons and plasmons are two very different types of collective modes, acting on the spin and charge degrees of freedom, respectively. At first sight, the formation of hybrid plasmon-magnon polaritons in heterostructures of plasmonic and…

Mesoscale and Nanoscale Physics · Physics 2023-06-05 A. T. Costa , M. I. Vasilevskiy , J. Fernández-Rossier , N. M. R. Peres

We present a quantum theory for the interaction of a two level emitter with surface plasmon polaritons confined in single-mode waveguide resonators. Based on the Green's function approach, we develop the conditions for the weak and strong…

Mesoscale and Nanoscale Physics · Physics 2015-03-20 T. Hümmer , F. J. García-Vidal , L. Martín-Moreno , D. Zueco

Polaritons are compositional light-matter quasiparticles that have recently enabled remarkable breakthroughs in quantum and nonlinear optics, as well as in material science. Despite the enormous progress, however, a direct nanometer-scale…

The coherent strong coupling of molecules with confined light fields to create polaritons - part matter, part light - is opening exciting opportunities ranging from extended exciton transport and inter-molecular energy transfer to modified…

Plasmonic nanocavities enable access to the quantum properties of matter, but are often simplified to single mode models despite their complex multimode structure. Here, we show that off-resonant plasmonic modes in fact play a crucial role…

Quantum Physics · Physics 2024-11-13 Angus Crookes , Ben Yuen , Angela Demetriadou

Plasmonic structures interacting with light provide electromagnetic resonances which result in a high degree of local field confinement enabling the enhancement of light-matter interaction. Plasmonic structures typically consist of metals…

Polaritons are quasiparticles arising from the strong coupling of electromagnetic waves in cavities and dipolar oscillations in a material medium. In this framework, localized surface plasmon in metallic nanoparticles defining optical…

The strong coupling between two subsystems consisting of quantum emitters and photonic modes, at which the level splitting of mixed quantum states occurs, has been a central subject of quantum physics and nanophotonics due to various…

Optics · Physics 2021-06-30 Renming Liu , Yi-Cong Yu , Xue-Hua Wang

Quantum plasmonics extends cavity quantum electrodynamics (cQED) concepts to the nanoscale, taking benefit from the strongly subwavelength confinement of the plasmon modes supported by metal nanostructures. In this work, we describe in…

Quantum Physics · Physics 2022-09-15 H. Varguet , A. Diaz-Valles , S. Guérin , H. R. Jauslin , G. Colas des Francs

Strong coupling in the conventional sense requires that the Rabi cycling process between two interacting states is faster than other dissipation rates. Some recent experimental findings show intriguing properties that were attributed to…

Materials Science · Physics 2026-03-09 Ben Johns , Nitin Yadav , Anand Vinod , Kuljeet Kaur , Jino George

Physical and chemical properties of materials can be modified by a resonant optical mode. Such recent demonstrations have mostly relied on a planar cavity geometry, others have relied on a plasmonic resonator. However, the combination of…