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We use the "generalized hierarchical equation of motion" proposed in Paper I to study decoherence in a system coupled to a spin bath. The present methodology allows a systematic incorporation of higher order anharmonic effects of the bath…

Chemical Physics · Physics 2018-01-17 Chang-Yu Hsieh , Jianshu Cao

Frequency standards based on atomic states, such as Rb or Cs vapors, or single trapped ions, are the most precise measures of time. Here we introduce a complementary device based on spins in a solid-state system - the nitrogen-vacancy…

Atomic Physics · Physics 2011-09-16 Jonathan S. Hodges , Dirk Englund

One approach to maintaining phase coherence of qubits through dynamical decoupling consists of applying a sequence of Hahn spin-echo pulses. Recent studies have shown that, in certain noise environments, judicious choice of the delay times…

Quantum Physics · Physics 2009-06-24 Hermann Uys , Michael J. Biercuk , John J. Bollinger

Long coherence times are key to the performance of quantum bits (qubits). Here, we experimentally and theoretically show that the Hahn-echo coherence time (T2) of electron spins associated with divacancy defects in 4H-SiC reaches 1.3 ms,…

Mesoscale and Nanoscale Physics · Physics 2016-10-03 Hosung Seo , Abram L. Falk , Paul V. Klimov , Kevin C. Miao , Giulia Galli , David D. Awschalom

Electron spin qubit coherence in quantum dots is ultimately limited by random nuclear spin bath fluctuations. Here we aim to eliminate this randomness by making spin bath evolution deterministic. We introduce spin bath control sequences,…

Mesoscale and Nanoscale Physics · Physics 2019-07-18 A. M. Waeber , M. Hopkinson , M. S. Skolnick , E. A. Chekhovich

We report the detection and polarization of nuclear spins in diamond at room temperature by using a single nitrogen-vacancy (NV) center. We use Hartmann-Hahn double resonance to coherently enhance the signal from a single nuclear spin while…

Spin qubit coherence is a fundamental resource for the realization of quantum technologies. For solid-state platforms, spin decoherence is dominated by the magneto-active environment in the lattice, limiting their applicability. While…

The nitrogen vacancy (NV) center in diamond, a well-studied, optically active spin defect, is the prototypical system in many state of the art quantum sensing and communication applications. In addition to the enticing properties intrinsic…

Characterizing and understanding the environment affecting quantum systems is critical to elucidate its physical properties and engineer better quantum devices. We develop an approach to reduce the quantum environment causing single-qubit…

Quantum Physics · Physics 2022-10-19 Won Kyu Calvin Sun , Paola Cappellaro

In the framework of nuclear magnetic resonance, we consider the general problem of the coherent control of a spin coupled to a bath by means of composite or continuous pulses of duration $\tau_\mathrm{p}$. We show explicity that it is…

Quantum Physics · Physics 2010-03-16 S. Pasini , P. Karbach , C. Raas , G. S. Uhrig

We consider a SQUID tunneling between 2 nearly degenerate flux states. Decoherence caused by paramagnetic and nuclear spins in the low-$T$ limit is shown to be much stronger than that from electronic excitations. The decoherence time…

Condensed Matter · Physics 2007-05-23 Nikolay Prokof'ev , Philip Stamp

The unpolarized spin environment surrounding a central spin qubit is typically considered as an incoherent source of dephasing, however, precise characterization and control of the spin bath can yield a resource for storing and sensing with…

Quantum Physics · Physics 2023-12-01 R. M. Goldblatt , A. M. Martin , A. A. Wood

We study the decoherence of a spin in a quantum dot due to its hyperfine coupling to a randomly fluctuating bath of nuclear spins. The system is modelled by the central spin model with the spin bath initially being at infinite temperature.…

Mesoscale and Nanoscale Physics · Physics 2013-09-02 Alexandre Faribault , Dirk Schuricht

We present a cluster expansion method for approximating quantum spin-bath dynamics in terms of a classical Gaussian stochastic process. The cluster expansion produces the two-point correlation function of the approximate classical bath,…

Mesoscale and Nanoscale Physics · Physics 2014-09-30 Wayne M. Witzel , Kevin Young , Sankar Das Sarma

Diamond nanocrystals can harbor spin qubit sensors capable of probing the physical properties of biological systems with nanoscale spatial resolution. These diamond nanosensors can readily be delivered into intact cells and even living…

We present a study of the prospects for coherence preservation in solid-state spin qubits using dynamical decoupling protocols. Recent experiments have provided the first demonstrations of multipulse dynamical decoupling sequences in this…

Mesoscale and Nanoscale Physics · Physics 2013-05-29 M. J. Biercuk , H. Bluhm

Spin decoherence poses a significant challenge in molecular magnets, with the nuclear spin bath serving as a prominent source. Intriguingly, spin qubits at the clock transition exhibit remarkable insensitivity to the surrounding nuclear…

Quantum Physics · Physics 2025-10-14 Xiao Chen , Haechan Park , Silas Hoffman , Shuanglong Liu , Hai-Ping Cheng

Electron spins in gate-defined quantum dots provide a promising platform for quantum computation. In particular, spin-based quantum computing in gallium arsenide takes advantage of the high quality of semiconducting materials, reliability…

Solid-state spin defects, especially nuclear spins with potentially achievable long coherence times, are compelling candidates for quantum memories and sensors. However, their current performances are still limited by the decoherence due to…

Quantum Physics · Physics 2023-08-09 Guoqing Wang , Ariel Rebekah Barr , Hao Tang , Mo Chen , Changhao Li , Haowei Xu , Ju Li , Paola Cappellaro

We experimentally resolve several weakly coupled nuclear spins in diamond using a series of novelly designed dynamical decoupling controls. Some nuclear spin signals, hidden by decoherence under ordinary dynamical decoupling controls, are…