Related papers: Resolving the temporal evolution of line broadenin…
We develop a general microscopic theory describing the phonon decoherence of quantum dots and indistinguishability of the emitted photons in photonic structures. The coherence is found to depend fundamentally on the dimensionality of the…
Using a quantum electrodynamic framework, we calculate the off-resonant scattering of a broad-band X-ray pulse from a sample initially prepared in an arbitrary superposition of electronic states. The signal consists of single-particle…
Photonic Time Crystals (PTCs) - dielectric media with their refractive index modulated periodically in time, offer new opportunities in photonics arising from time reflections and momentum bandgaps. Here, we study the emission of light from…
Solid-state emitters are excellent candidates for developing integrated sources of single photons. Yet, phonons degrade the photon indistinguishability both through pure dephasing of the zero-phonon line and through phonon-assisted…
Multi-photon quantum walks in integrated optics are an attractive controlled quantum system, that can mimic less readily accessible quantum systems and exhibit behavior that cannot in general be accurately replicated by classical light…
Emitter dephasing is one of the key issues in the performance of solid-state single photon sources. Among the various sources of dephasing, acoustic phonons play a central role in adding decoherence to the single photon emission. Here, we…
The evolution from 3rd to 4th generation synchrotron radiation (SR) sources significantly enhanced their coherence, making coherent scattering techniques such as coherent X-ray diffraction imaging (CXDI) and X-ray photon correlation…
We demonstrate purely resonant continuous-wave optical laser excitation to coherently prepare an excitonic state of a single semiconductor quantum dot (QDs) inside a high quality pillar microcavity. As a direct proof of QD resonance…
Color centers in hexagonal boron nitride (hBN) emerge as promising quantum light sources at room temperature, with potential applications in quantum communications, among others. The temporal coherence of emitted photons (i.e. their…
Resonance fluorescence of a two-level emitter displays persistently anti-bunching irrespective of the excitation intensity, but inherits the driving laser's linewidth under weak monochromatic excitation. These properties are commonly…
In classical coherence theory, coherence time is typically related to the bandwidth of the optical field. Narrowing the bandwidth will result in the lengthening of the coherence time. This will erase temporal distinguishability of photons…
The ability to measure polarisation, spectrum, temporal dynamics, and spatial amplitude and phase of optical beams is essential to study fundamental phenomena in laser dynamics, telecommunications and nonlinear optics. Current…
The homogeneous spectral linewidth associated with light-matter interactions is a fundamental descriptor of the optical properties of materials, governed by the quantum dynamics of the condensed-matter system. We discuss here that the…
We develop a theory of the linear optical spectrum of excitons in quantum dot molecules, including the effect of exciton-phonon coupling beyond the Markov limit. The model reproduces the general trend of the zero-phonon line broadening as a…
Ultrafast spectroscopy of molecular systems is fundamentally constrained by the Fourier uncertainty principle: high temporal resolution smears out electronic state signatures, while high spectral resolution obscures dynamic information.…
We study theoretically the radiative recombination of excitons in double quantum dots in the presence of carrier-phonon coupling. We show that the phonon-induced pure dephasing effects and transitions between the exciton states strongly…
Dephasing processes significantly impact the performance of deterministic single-photon sources. Dephasing broadens the spectral line and suppresses the indistinguishability of the emitted photons, which is undesirable for many…
We observe experimentally that ensembles of quantum dots in three-dimensional (3D) photonic crystals reveal strongly nonexponential time-resolved emission. These complex emission decay curves are analyzed with a continuous distribution of…
Spectral diffusion is a result of random spectral jumps of a narrow line as a result of a fluctuating environment. It is an important issue in spectroscopy, because the observed spectral broadening prevents access to the intrinsic line…
We obtain time-resolved spectra of spontaneous emission and resonance fluorescence of a single multilevel emitter where two antiparallel transitions interfere and cause quantum beats. After rising as a single broad peak, the spontaneous…