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We calculate the potential energy surfaces for graphene adsorbed on Cu(111), Ni(111), and Co(0001) using density functional theory and the Random Phase Approximation (RPA). For these adsorption systems covalent and dispersive interactions…

Materials Science · Physics 2012-08-24 T. Olsen , J. Yan , J. J. Mortensen , K. S. Thygesen

We introduce and demonstrate the coarse-graining of static and dynamical properties of host-guest systems constituted by methane in two different microporous materials. The reference systems are mapped to occupancy-based pore-scale lattice…

Computational Physics · Physics 2019-08-05 Giovanni Pireddu , Federico G. Pazzona , Pierfranco Demontis , Magdalena A. Załuska-Kotur

We perform a density functional theory study of the effects of oxygen adsorption on the structural and electronic properties of Gr/Co(0001) and Gr/Co/Ir(111) interfaces. In both interfaces, the graphene-Co distance increases with increasing…

Materials Science · Physics 2022-08-05 Dario A. Leon , Andrea Ferretti , Daniele Varsano , Elisa Molinari , Claudia Cardoso

We present a model study to estimate the sensitivity of the optical absorption of multilayered graphene structure to the subnanometer interlayer separation. Starting from a transfer-matrix formalism we derive semi-analytical expressions for…

Optics · Physics 2022-11-28 Devashish Pandey , Sanshui Xiao , Martijn Wubs

The moir\'e superstructure of graphene grown on metals can drive the assembly of molecular architectures, as iron-phthalocyanine (FePc) molecules, allowing for the production of artificial molecular configurations. A detailed analysis of…

The contact of water with graphene is of fundamental importance and of great interest for numerous promising applications, but how graphene interacts with water remains unclear. Here we used atomic force microscopy to investigate…

Mesoscale and Nanoscale Physics · Physics 2016-04-12 Hsien-Chen Ko , Wei-Hao Hsu , Chih-Wen Yang , Chung-Kai Fang , Yi-Hsien Lu , Ing-Shouh Hwang

Two approximations used by Sengupta [Phys. Rev. B {\bf 100}, 075429 (2019)] in numerically computing the adsorption rate of cold hydrogen atoms on suspended graphene are critically examined. The independent boson model approximation (IBMA)…

Mesoscale and Nanoscale Physics · Physics 2020-06-12 Dennis P. Clougherty

Graphane is a layered material consisting of a sheet of hydrogenated graphene, with a C:H ratio of 1:1. We study isotopic effects in the properties of chair graphane, where H atoms alternate in a chairlike arrangement on both sides of the…

Materials Science · Physics 2021-07-28 Carlos P. Herrero , Rafael Ramirez

The plane wave scattering and absorption by finite and infinite gratings of free-space standing infinitely long graphene strips are studied in the THz range. A novel numerical approach, based on graphene surface impedance, hyper-singular…

Mesoscale and Nanoscale Physics · Physics 2013-10-02 Olga V. Shapoval , Juan Sebastian Gomez-Diaz , Julien Perruisseau-Carrier , Juan R. Mosig , Alexander I. Nosich

We systematically derive an exact coarse-grained description for interacting particles with thermodynamically consistent stochastic dynamics, applicable across different observation scales, the mesoscopic and the macroscopic. We implement…

Statistical Mechanics · Physics 2026-03-05 Atul Tanaji Mohite , Heiko Rieger

The integral equation coarse-graining (IECG) approach is a promising high-level coarse-graining (CG) method for polymer melts, with variable resolution from soft spheres to multi CG sites, which preserves the structural and thermodynamical…

Soft Condensed Matter · Physics 2018-07-24 Mohammadhasan Dinpajooh , Marina G. Guenza

CO$_2$ capture using carbon-based materials, particularly graphene and graphene-like materials, is a promising strategy to deal with CO$_2$ emissions. However, significant gaps remain in our understanding of the molecular-level interaction…

We introduce an effective tight-binding model to discuss penta-graphene and present an analytical solution. This model only involves the $\pi$-orbitals of the sp$^2$-hybridized carbon atoms and reproduces the two highest valence bands. By…

Mesoscale and Nanoscale Physics · Physics 2016-03-07 T. Stauber , J. I. Beltrán , J. Schliemann

We present an accurate interatomic potential for graphene, constructed using the Gaussian Approximation Potential (GAP) machine learning methodology. This GAP model obtains a faithful representation of a density functional theory (DFT)…

Materials Science · Physics 2018-02-14 Patrick Rowe , Gábor Csányi , Dario Alfè , Angelos Michaelides

A great efficacy of molecular quantum chemistry applied to basic graphene problems has been recently demonstrated by the authors when studying the formation of peculiar composites between carbon nanotubes and graphene as well as considering…

Mesoscale and Nanoscale Physics · Physics 2011-02-07 Elena F Sheka , Nadezhda A Popova

The distribution of diffuse gas in the intergalactic medium (IGM) imprints a series of hydrogen absorption lines on the spectra of distant background quasars known as the Lyman-$\alpha$ forest. Cosmological hydrodynamical simulations…

Cosmology and Nongalactic Astrophysics · Physics 2017-05-31 Alberto Rorai , Joseph F. Hennawi , Jose Oñorbe , Martin White , J. Xavier Prochaska , Girish Kulkarni , Michael Walther , Zarija Lukić , Khee-Gan Lee

The random phase approximation (RPA) is attracting renewed interest as a universal and accurate method for first-principles total energy calculations. The RPA naturally accounts for long-range dispersive forces without compromising accuracy…

Materials Science · Physics 2013-03-04 Thomas Olsen , Kristian S. Thygesen

Pillared Graphene Frameworks are a novel class of microporous materials made by graphene sheets separated by organic spacers. One of their main features is that the pillar type and density can be chosen to tune the material properties. In…

Materials Science · Physics 2017-07-04 Andrea Pedrielli , Simone Taioli , Giovanni Garberoglio , Nicola Maria Pugno

The adsorption of fluorine, chlorine, bromine, and iodine diatomic molecules on graphene has been investigated using density functional theory with taking into account nonlocal correlation effects by means of vdW-DF approach. It is shown…

Mesoscale and Nanoscale Physics · Physics 2010-09-15 A. N. Rudenko , F. J. Keil , M. I. Katsnelson , A. I. Lichtenstein

We exploited graphene nanoribbons based meta-surface to realize coherent perfect absorption (CPA) in the mid-infrared regime. It was shown that quasi-CPA frequencies, at which CPA can be demonstrated with proper phase modulations, exist for…

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