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Fifth-generation organic light-emitting diodes exhibit delayed fluorescence even at low temperatures, enabled by exothermic reverse intersystem crossing from a negative singlet-triplet gap (STG), where the first excited singlet lies…
The study of light-matter interaction has led to many fundamental discoveries as well as numerous important technologies. Over the last decades, great strides have been made in increasing the strength of this interaction at the…
Optical cavities confine light on a small region in space which can result in a strong coupling of light with materials inside the cavity. This gives rise to new states where quantum fluctuations of light and matter can alter the properties…
One of the most intriguing topological features of open systems is exhibiting exceptional point (EP) singularities. Apart from the widely explored second-order EPs (EP2s), the explorations of higher-order EPs in any system requires more…
Photophysics of single-wall carbon nanotubes (SWCNTs) is intensively studied due to their potential application in light harvesting and optoelectronics. Excited states of SWCNTs form strongly bound electron-hole pairs, excitons, of which…
Fabry-Perot microcavities can strongly enhance interactions between light and molecules, leading to the formation of hybrid light-matter states known as polaritons. Polaritons possess much smaller effective masses and much larger group…
The study of light-matter interaction has seen a resurgence in recent years, stimulated by highly controllable, precise, and modular experiments in cavity quantum electrodynamics (QED). The achievement of strong coupling, where the coupling…
Organic semiconductors are particularly attractive for polaritonics due to their large exciton binding energies and oscillator strengths. Among them, the ladder-type conjugated polymer poly(paraphenylene) is distinguished by its rigid…
We investigate the many-body states of exciton-polaritons that can be observed by pump-probe spectroscopy. Here, a weak-probe `spin-down' polariton is introduced into a coherent state of `spin-up' polaritons created by a strong pump. We…
By employing single charge injections with an atomic force microscope, we investigated redox reactions of a molecule on a multilayer insulating film. First, we charged the molecule positively by attaching a single hole. Then we neutralized…
Strong-coupling between light and matter produces hybridized states (polaritons) whose delocalization and electromagnetic character allow for novel modifications in spectroscopy and chemical reactivity of molecular systems. Recent…
The ultrastrong light-matter interaction regime was investigated in metallic and superconducting complementary split ring resonators coupled to the cyclotron transition of two dimensional electron gases. The sub-wavelength light confinement…
We investigate the effect of far-off-resonant trapping light on ultracold bosonic RbCs molecules. We use kHz-precision microwave spectroscopy to measure the differential AC Stark shifts between the ground and first excited rotational levels…
In vibrational strong coupling (VSC), molecular vibrations strongly interact with the modes of an optical cavity to form hybrid light-matter states known as vibrational polaritons. Experiments show that the kinetics of thermally activated…
We demonstrate a new type of transition within the strong coupling regime, which alters the coupling mechanism in multimode cavities. We show that this transition drastically modifies the Hamiltonian describing the polaritons, such that…
The entanglement of an optically generated electron-hole pair in artificial quantum dot molecules is calculated considering the effects of decoherence by interaction with environment. Since the system evolves into a mixed states and due to…
Intermixed light-matter quasiparticles - polaritons - possess unique optical properties owned to their compositional nature. These intriguing hybrid states have been extensively studied over the past decades in a wide range of realizations…
We theoretically investigated the coupling between the exciton internal and center-of-mass motions in monolayer transition metal dichalcogenides subjected to a periodic electrostatic potential. The coupling leads to the emergence of…
We study the light-matter coupling of microcavity photons and an interband transition in a one-dimensional (1D) nanowire. Due to the Van Hove singularity in the density of states, resulting in a resonant character of the absorption line,…
Condensation of bosons causes spectacular phenomena such as superfluidity or superconductivity. Understanding the nature of the condensed particles is crucial for active control of such quantum phases. Fascinating possibilities emerge from…