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Quantum computational chemistry holds great promise for simulating molecular systems more efficiently than classical methods by leveraging quantum bits to represent molecular wavefunctions. However, current implementations face significant…

Quantum Physics · Physics 2025-09-10 Weitang Li , Shi-Xin Zhang , Zirui Sheng , Cunxi Gong , Jianpeng Chen , Zhigang Shuai

Quantum Machine Learning (QML) models of molecular HOMO-LUMO-gaps often struggle to achieve satisfying data-efficiency as measured by decreasing prediction errors for increasing training set sizes. Partitioning training sets of organic…

Chemical Physics · Physics 2021-10-07 Bernard Mazouin , Alexandre Alain Schöpfer , O. Anatole von Lilienfeld

We address the inverse problem of identifying nonlocal interaction potentials in nonlinear aggregation-diffusion equations from noisy discrete trajectory data. Our approach involves formulating and solving a regularized variational problem,…

Analysis of PDEs · Mathematics 2025-01-31 Jose A. Carrillo , Gissell Estrada-Rodriguez , Laszlo Mikolas , Sui Tang

Hohenberg and Kohn have proven that the electronic energy and the one-particle electron density can, in principle, be obtained by minimizing an energy functional with respect to the density. While decades of theoretical work have produced…

Machine learning (ML) has recently gained attention as a means to develop more accurate exchange-correlation (XC) functionals for density functional theory, but functionals developed thus far need to be improved on several metrics,…

Chemical Physics · Physics 2022-03-14 Kyle Bystrom , Boris Kozinsky

At the intersection of quantum computing and machine learning, quantum machine learning (QML) is poised to revolutionize artificial intelligence. However, the vulnerability of the current generation of quantum computers to noise and…

Quantum Physics · Physics 2026-01-13 Eromanga Adermann , Haiyue Kang , Martin Sevior , Muhammad Usman

We obtain the conductance of a system of electrons connected to leads, within time-dependent density-functional theory, using a direct relation between the conductance and the density response function. Corrections to the non-interacting…

Materials Science · Physics 2007-10-04 P. Bokes , J. Jung , R. W. Godby

The computation of dynamical response functions is central to many problems in condensed matter physics. Owing to the rapid growth of quantum correlations following a quench, classical methods face significant challenges even if an…

Quantum Physics · Physics 2025-05-09 Esther Cruz , Dominik S. Wild , Mari Carmen Bañuls , J. Ignacio Cirac

A common approach to modeling dispersion interactions and overcoming the inaccurate description of long-range correlation effects in electronic structure calculations is the use of pairwise-additive potentials, as in the…

Materials Science · Physics 2024-07-10 Heikki Muhli , Tapio Ala-Nissila , Miguel A. Caro

The task of preserving entanglement against noises is of crucial importance for both quantum communication and quantum information transfer. To this aim, quantum error correction (QEC) codes may be employed to compensate, at least…

Quantum Physics · Physics 2023-03-21 Alessio Morea , Michele N. Notarnicola , Stefano Olivares

We train a deep convolutional neural network to predict hydrodynamic results for flow coefficients, average transverse momenta and charged particle multiplicities in ultrarelativistic heavy-ion collisions from the initial energy density…

High Energy Physics - Phenomenology · Physics 2023-03-09 H. Hirvonen , K. J. Eskola , H. Niemi

Interacting defect systems are ubiquitous in materials under realistic scenarios, yet gaining an atomic-level understanding of these systems from a computational perspective is challenging - it often demands substantial resources due to the…

Materials Science · Physics 2024-03-21 Hao Yu

Errors in quantum computers are of two kinds: sudden perturbations to isolated qubits, and slow random drifts of all the qubits. The latter may be reduced, but not eliminated, by means of symmetrization, namely by using many replicas of the…

Quantum Physics · Physics 2007-05-23 Asher Peres

We demonstrate that continuous-variable quantum error correction based on Gaussian ancilla states and Gaussian operations (for encoding, syndrome extraction, and recovery) can be very useful to suppress the effect of non-Gaussian error…

Quantum Physics · Physics 2008-11-24 Peter van Loock

Using an end-to-end differentiable implementation of the Kohn-Sham self-consistent field equations, we obtain an accurate neural network-based exchange and correlation (XC) functional of the electronic density. The functional is optimized…

Chemical Physics · Physics 2021-06-09 Sebastian Dick , Marivi Fernandez-Serra

Quantum machine learning (QML) requires powerful, flexible and efficiently trainable models to be successful in solving challenging problems. We introduce density quantum neural networks, a model family that prepares mixtures of trainable…

This paper derives and demonstrates a new, purely density-based ab initio approach for calculation of the energies and properties of many-electron systems. It is based upon the discovery of relationships that govern the "mechanics" of the…

Chemical Physics · Physics 2024-09-04 James C. Ellenbogen

Motivated by the intriguing physics of quasi-2d fermionic systems, such as high-temperature superconducting oxides, layered transition metal chalcogenides or surface or interface systems, the development of many-body computational methods…

Strongly Correlated Electrons · Physics 2022-06-22 Steffen Backes , Jae-Hoon Sim , Silke Biermann

We introduce a local machine-learning method for predicting the electron densities of periodic systems. The framework is based on a numerical, atom-centred auxiliary basis, which enables an accurate expansion of the all-electron density in…

Chemical Physics · Physics 2021-11-10 Alan M. Lewis , Andrea Grisafi , Michele Ceriotti , Mariana Rossi

Continuous quantum error correction has been found to have certain advantages over discrete quantum error correction, such as a reduction in hardware resources and the elimination of error mechanisms introduced by having entangling gates…