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We report on theoretical investigations of the spin-orbit coupling effects in fluorinated graphene. First-principles density functional calculations are performed for the dense and dilute adatom coverage limits. The dense limit is…

Mesoscale and Nanoscale Physics · Physics 2015-04-07 Susanne Irmer , Tobias Frank , Sebastian Putz , Martin Gmitra , Denis Kochan , Jaroslav Fabian

The issue of whether local magnetic moments can be formed by introducing adatoms into graphene is of intense research interest because it opens the window to fundamental studies of magnetism in graphene, as well as of its potential…

Mesoscale and Nanoscale Physics · Physics 2012-06-12 X. Hong , K. Zou , B. Wang , S. -H. Cheng , J. Zhu

Adatom-decorated graphene offers a promising new path towards spintronics in the ultrathin limit. We combine experiment and theory to investigate the electronic properties of dilutely fluorinated bilayer graphene, where the fluorine adatoms…

Mesoscale and Nanoscale Physics · Physics 2015-10-07 Adam A. Stabile , Aires Ferreira , Jing Li , N. M. R. Peres , J. Zhu

We propose that the observed spin-relaxation in bilayer graphene is due to resonant scattering by magnetic impurities. We analyze a resonant scattering model due to adatoms on both dimer and non-dimer sites, finding that only the former…

Mesoscale and Nanoscale Physics · Physics 2016-03-01 Denis Kochan , Susanne Irmer , Martin Gmitra , Jaroslav Fabian

Spin transitions driven by a periodically varying electric potential in dilute fluorinated graphene quantum dots are investigated. Flakes of monolayer graphene are considered as well as electrostatic electron traps induced in bilayer…

Mesoscale and Nanoscale Physics · Physics 2016-12-22 D. P. Żebrowski , F. M. Peeters , B. Szafran

It is proposed that the observed small (100 ps) spin relaxation time in graphene is due to resonant scattering by local magnetic moments. At resonances, magnetic moments behave as spin hot spots: the spin-flip scattering rates are as large…

Mesoscale and Nanoscale Physics · Physics 2014-03-26 Denis Kochan , Martin Gmitra , Jaroslav Fabian

The elimination of extrinsic sources of spin relaxation is key in realizing the exceptional intrinsic spin transport performance of graphene. Towards this, we study charge and spin transport in bilayer graphene-based spin valve devices…

Spin transport experiments in graphene, a single layer of carbon atoms, indicate spin relaxation times that are significantly shorter than the theoretical predictions. We investigate experimentally whether these short spin relaxation times…

Mesoscale and Nanoscale Physics · Physics 2015-05-13 M. Popinciuc , C. Józsa , P. J. Zomer , N. Tombros , A. Veligura , H. T. Jonkman , B. J. van Wees

We perform a comparative study of the spin relaxation by spin-orbit coupling induced from adatoms (hydrogen and fluorine) in graphene. Two methods are applied, giving consistent results: a full quantum transport simulation of a graphene…

Mesoscale and Nanoscale Physics · Physics 2015-08-19 Jan Bundesmann , Denis Kochan , Fedor Tkatschenko , Jaroslav Fabian , Klaus Richter

We propose an intrinsic spin scattering mechanism in graphene originated by the interplay of atomic spin-orbit interaction and the local curvature induced by flexural distortions of the atomic lattice. Starting from a multiorbital…

Mesoscale and Nanoscale Physics · Physics 2013-09-25 S. Fratini , D. Gosálbez-Martínez , P. Merodio Cámara , J. Fernández-Rossier

We present density functional theory calculations of the binding energies of one, two and three fluorine adatoms on the same side of monolayer graphene. We show that fluorine dimers on graphene in a spin-singlet state are stable against…

Materials Science · Physics 2017-09-18 F Marsusi , N D Drummond

The scattering of two-dimensional massless Dirac fermions from local spin-orbit interactions with an origin in dilute concentrations of physisorbed atomic species on graphene is theoretically investigated. The hybridization between graphene…

Mesoscale and Nanoscale Physics · Physics 2014-08-21 Alexandre Pachoud , Aires Ferreira , B. Özyilmaz , A. H. Castro Neto

The decoration of graphene samples with adatoms or nanoparticles leads to the enhancement of spin-orbit interactions as well as to the introduction of symmetry-breaking effects that could have drastic effects on spin and electronic…

Mesoscale and Nanoscale Physics · Physics 2015-04-13 Mahmoud M. Asmar , Sergio E. Ulloa

We study the spin relaxation in a single-electron bilayer graphene quantum dot due to the spin-orbit coupling. The spin relaxation is assisted by the emission of acoustic phonons via the bond-length change and deformation potential…

Mesoscale and Nanoscale Physics · Physics 2025-05-21 Lin Wang , Guido Burkard

We report on spin transport features which are unique to high quality bilayer graphene, in absence of magnetic contaminants and strong intervalley mixing. The time-dependent spin polarization of propagating wavepacket is computed using an…

Mesoscale and Nanoscale Physics · Physics 2016-07-20 Dinh Van Tuan , Shaffique Adam , Stephan Roche

Electrons in graphene are theoretically expected to retain spin states much longer than most materials, making graphene a promising platform for spintronics and quantum information technologies. Here, we use first-principles density-matrix…

Materials Science · Physics 2022-03-17 Adela Habib , Junqing Xu , Yuan Ping , Ravishankar Sundararaman

We discuss the role of spin-flip scattering of electrons from the magnetized edges in graphene nanoribbons. The spin-flip scattering is associated with strong fluctuations of the magnetic moments at the edge. Using the Boltzmann equation…

Mesoscale and Nanoscale Physics · Physics 2015-06-19 V. K. Dugaev , M. I. Katsnelson

In graphene, out-of-plane (flexural) vibrations and static ripples imposed by the substrate relax the electron spin, intrinsically protected by mirror symmetry. We calculate the relaxation times in different scenarios, accounting for all…

Mesoscale and Nanoscale Physics · Physics 2017-05-08 I. M. Vicent , H. Ochoa , F. Guinea

The naturally weak spin-orbit coupling in Graphene can be largely enhanced by adatom deposition (e.g. Weeks et al. Phys. Rev. X 1, 021001 (2011)). However, the dynamics of the adatoms also induces a coupling between phonons and the electron…

Mesoscale and Nanoscale Physics · Physics 2015-07-29 Jhih-Shih You , Daw-Wei Wang , Miguel A. Cazalilla

Electron spin relaxation due to the D'yakonov-Perel' mechanism is investigated in bilayer graphene with only the lowest conduction band being relevant. The spin-orbit coupling is constructed from the symmetry group analysis with the…

Mesoscale and Nanoscale Physics · Physics 2013-05-14 L. Wang , M. W. Wu
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