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We use ultrafast x-ray and electron diffraction to disentangle spin-lattice coupling of granular FePt in the time domain. The reduced dimensionality of single-crystalline FePt nanoparticles leads to strong coupling of magnetic order and a…

We theoretically investigate the optically-induced demagnetization of ferromagnetic FePt using the time-dependent density functional theory (TDDFT). We compare the demagnetization mechanism in the perturbative and nonperturbative limits of…

Materials Science · Physics 2024-04-26 M. S. Mrudul , Peter M. Oppeneer

Light-matter interaction at the nanoscale in magnetic alloys and heterostructures is a topic of intense research in view of potential applications in high-density magnetic recording. While the element-specific dynamics of electron spins is…

Magnetic x-ray diffraction combined with x-ray focusing optics is used to image individual antiferromagnetic spin density wave domains in a chromium single crystal at the micron scale. The cross section for non-resonant magnetic x-ray…

Other Condensed Matter · Physics 2007-06-01 Paul G. Evans , Eric D. Isaacs , Gabriel Aeppli , Zhonghou Cai , Barry Lai

Magnetic nanoparticles such as FePt in the L10-phase are the bedrock of our current data storage technology. As the grains become smaller to keep up with technological demands, the superparamagnetic limit calls for materials with higher…

Nuclear resonant x-ray diffraction in grazing incidence geometry is used to determine the lateral magnetic configuration in a one-dimensional lattice of ferromagnetic nanostripes. During magnetic reversal, strong nuclear superstructure…

The microscopic origin of laser-induced ultrafast demagnetization remains an open question, to which the non-thermal electronic distribution plays a vital role at the initial stage. Herein, we investigate the connection between the…

Materials Science · Physics 2025-12-25 Yu-Hui Song , Huan-Cheng Yang , Kai Liu , Zhong-Yi Lu

Diffraction imaging of non-equilibrium dynamics at atomic resolution is becoming possible with X-ray free-electron lasers. However, there are unresolved problems with applying this method to objects that are confined in only one dimension.…

Strongly Correlated Electrons · Physics 2018-02-19 Kenneth R. Beyerlein

Time-dependent density functional theory is implemented in an all electron solid-state code for the case of fully non-collinear spins. We use this to study laser induced demagnetization in Fe, Co and Ni. It is shown that this…

Materials Science · Physics 2014-06-26 K. Krieger , J. K. Dewhurst , P. Elliott , S. Sharma , E. K. U. Gross

We performed time-resolved x-ray resonant magnetic reflectivity measurements on a laser-excited ferromagnetic Fe thin film to simultaneously probe the transient structural and magnetic depth profiles with nanometer spatial and femtosecond…

Two complementary effects modify the GHz magnetization dynamics of nanoscale heterostructures of ferromagnetic and normal materials relative to those of the isolated magnetic constituents: On the one hand, a time-dependent ferromagnetic…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 Yaroslav Tserkovnyak , Arne Brataas , Gerrit E. W. Bauer , Bertrand I. Halperin

We use resonant soft X-ray diffraction to track the photo-induced dynamics of the antiferromagnetic structure in a NdNiO$_{3}$ thin film. Femtosecond laser pulses with a photon energy of 0.61 eV, resonant with electron transfer between…

Element-specific spectroscopies using synchrotron-radiation can provide unique insights into materials properties. The recently developed technique of X-ray detected ferromagnetic resonance (XFMR) allows studying the magnetization dynamics…

Materials Science · Physics 2023-05-17 Gerrit van der Laan , Thorsten Hesjedal

We report on time- and angle-resolved transverse magneto-optical Kerr effect spectroscopy in the soft x-ray range that, by analysis via polarization-dependent magnetic scattering simulations, allows us to determine the spatio-temporal and…

The objective of this article is to study the behavior of electromagnetic field under X-ray diffraction by time-dependent deformed crystals. Derived system of differential equations looks like the Takagi equations in the case of…

Computational Physics · Physics 2007-05-23 Svetlana Sytova

Exact calculated time evolutions in the framework of a many-electron model of itinerant magnetism provide new insights into the laser-induced ultrafast demagnetization observed in ferromagnetic (FM) transition metal thin films. The…

Strongly Correlated Electrons · Physics 2015-11-25 W. Töws , G. M. Pastor

Demagnetization in ferromagnetic transition metals driven by a femtosecond laser pulse is a fundamental problem in solid state physics, and its understanding is essential to the development of spintronics devices. Ab initio calculation of…

Materials Science · Physics 2024-01-02 Mitsuko Murakami , G. P. Zhang

We demonstrate the use of the magnetic-field-dependence of highly spatially confined, GHz-frequency ferromagnetic resonances in a ferromagnetic nanostructure for the detection of adsorbed magnetic nanoparticles. This is achieved in a large…

X-ray scattering has been an indispensable tool in advancing our understanding of matter, from the first evidence of the crystal lattice to recent discoveries of nuclei's fastest dynamics. In addition to the lattice, ultrafast resonant…

Scanning X-ray nanodiffraction microscopy is a powerful technique for spatially resolving nanoscale structural morphologies by diffraction contrast. One of the critical challenges in experimental nanodiffraction data analysis is posed by…

Applied Physics · Physics 2024-06-26 Aileen Luo , Tao Zhou , Martin V. Holt , Andrej Singer , Mathew J. Cherukara
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