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Metal-organic molecular adsorbates on metallic surfaces offer the potential to both generate materials for future (spin-)electronics applications as well as a better fundamental understanding of molecule-substrate interaction, provided that…

Materials Science · Physics 2024-09-17 A. Eschenlohr , R. Shi , J. Chen , P. Zhou , U. Bovensiepen , W. Hübner , G. Lefkidis

We theoretically study high-order harmonic generation (HHG) from solid-phase systems in spatially inhomogeneous strong laser fields originated by resonant plasmons within a metallic nanostructure. The intensity of the second plateau in HHG…

Optics · Physics 2016-09-12 Tao-Yuan Du , Zhong Guan , Xiao-Xin Zhou , Xue-Bin Bian

We show that optical second-harmonic generation (SHG) can be observed from individual single-walled carbon nanotubes (SWCNTs) and, furthermore, allows imaging of individual tubes. Detailed analysis of our results suggests that the…

Plasmonic nanostructures that support surface plasmon (SP) resonance potentially provide a route for the development of nanoengineered nonlinear optical devices. In this work, second-order nonlinear light scattering, specifically…

Computational Physics · Physics 2016-12-20 Xiaoyan Y. Z. Xiong , Li Jun Jiang , Wei E. I. Sha , Yat Hei Lo , Weng Cho Chew

Rhombohedral multilayer graphene hosts a rich landscape of correlated symmetry-broken phases, driven by strong interactions from its flat band edges. Aligning to hexagonal boron nitride (hBN) creates a moir\'e pattern, leading to recent…

Two-particle spectroscopy with correlated electron pairs is used to establish the causal link between the secondary electron spectrum, the $(\pi+\sigma)-$plasmon peak and the unoccupied band structure of highly oriented pyrolitic graphite.…

Spectroscopy of magnetization-induced second-harmonic generation (MSHG) is studied in magnetic Co$_{x}$Ag$_{1-x}$ granular films containing Co nanoparticles. A strong resonance of the magnetic contrast of the second-harmonic generation…

Adaptation and Self-Organizing Systems · Physics 2007-05-23 E. M. Kim , T. V. Murzina , A. F. Kravets , M. Inoue , G. Marowsky , O. A. Aktsipetrov

The optical response and the ground state of graphene and graphene-like systems are determined self-consistently. Deriving equations of motion for the basic variables, graphene Bloch equations are introduced and combined with a variational…

Materials Science · Physics 2012-01-10 T. Stroucken , J. H. Grönqvist , S. W. Koch

We analyze the electrostatic interactions between a single graphene layer and a SiO$_2$ susbtrate, and other materials which may exist in its environment. We obtain that the leading effects arise from the polar modes at the SiO$_2$ surface,…

Materials Science · Physics 2009-11-13 J. Sabio , C. Seoanez , S. Fratini , F. Guinea , A. H. Castro Neto , F. Sols

The notion of spontaneous symmetry breaking has been used to describe phase transitions in a variety of physical systems. In crystalline solids, the breaking of certain symmetries, such as mirror symmetry, is difficult to detect…

Materials Science · Physics 2020-07-01 Bryan T. Fichera , Anshul Kogar , Linda Ye , Bilal Gökce , Alfred Zong , Joseph G. Checkelsky , Nuh Gedik

We report the observations of unexpected layer-dependent, strong, and anisotropic second harmonic generations (SHGs) in atomically thin ReS2. Appreciable (negligible) SHGs are obtained from even (odd) numbers of ReS2 layers, which is…

Optics · Physics 2018-08-20 Yu Song , Siqi Hu , Miao-Ling Lin , Xuetao Gan , Ping-Heng Tan , Jianlin Zhao

Two-dimensional (2D) materials with zero band gap exhibit remarkable electronic properties with wide tunability. High harmonic generation (HHG) in such materials offers unique platforms to develop novel optoelectronic devices at nanoscale,…

Optics · Physics 2019-02-22 Rui Qin , Zi-Yu Chen

Missing second-order nonlinearity in centrosymmetric graphene overshadows its intriguing optical attribute. Here, we report redox-governed charge doping could effectively break the centrosymmetry of bilayer graphene (BLG), enabling a strong…

Dielectric metasurfaces have shown prominent applications in nonlinear optics due to strong field enhancement and low dissipation losses at the nanoscale. Chalcogenide glasses are one of the promising materials for the observation of…

The interaction between a graphene layer and a hexagonal Boron Nitride (hBN) substrate induces lateral displacements and strains in the graphene layer. The displacements lead to the appearance of commensurate regions and the existence of an…

Mesoscale and Nanoscale Physics · Physics 2014-09-05 Pablo San-Jose , Ángel Gutiérrez , Mauricio Sturla , Francisco Guinea

We investigate theoretically and experimentally the optical second harmonic generation (SHG) with a twisted Gaussian Schell model (TGSM) beam as the fundamental field. We use Type-II phase matching and analyze the cross spectral density…

Naturally or artificially stacking extra layers on single layer graphene (SLG) forms few-layer graphene (FLG), which has attracted tremendous attention owing to its exceptional properties inherited from SLG and new features generated by…

Mesoscale and Nanoscale Physics · Physics 2015-07-03 Chunxiao Cong , Ting Yu

The study of high-harmonic generation in confined quantum systems is vital to establishing a complete physical picture of harmonic generation from atoms and molecules to bulk solids. Based on a multilevel approach, we demonstrate how…

Mesoscale and Nanoscale Physics · Physics 2023-03-28 Xiao Zhang , Tao Zhu , Hongchuan Du , Hong-Gang Luo , Jeroen van den Brink , Rajyavardhan Ray

High-order harmonic generation (HHG) in solids has entered a new phase of intensive research, with envisioned band-structure mapping on an ultrashort time scale. This partly benefits from a flurry of new HHG materials discovered, but so far…

Materials Science · Physics 2018-09-12 G. P. Zhang , M. S. Si , M. Murakami , Y. H. Bai , Thomas F. George

Circularly polarized extreme ultraviolet (XUV) radiation is highly interesting for investigation of chirality-sensitive light-matter interactions. Recent breakthroughs have enabled generation of such light sources via high harmonic…

Optics · Physics 2019-02-19 Zi-Yu Chen , Rui Qin
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