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The anisotropic nature of the new two-dimensional (2D) material phosphorene, in contrast to other 2D materials such as graphene and transition metal dichalcogenide (TMD) semiconductors, allows excitons to be confined in a…

Understanding interfacial interactions in two-dimensional (2D) heterostructures is essential for advancing optoelectronic and quantum technologies. We investigate metal-organic chemical vapor deposition (MOCVD)-grown WSe$_2$ films (one to…

We present a many-body theory for exciton-trion-polaritons in doped two-dimensional materials. Exciton-trion-polaritons are robust coherent hybrid excitations involving excitons, trions, and photons. Signatures of these polaritons have been…

Mesoscale and Nanoscale Physics · Physics 2021-03-31 Farhan Rana , Okan Koksal , Minwoo Jung , Gennady Shvets , A. Nick Vamivakas , Christina Manolatou

Topological transition of the iso-frequency contour (IFC) from a closed ellipsoid to an open hyperboloid, will provide unique capabilities for controlling the propagation of light. However, the ability to actively tune these effects remains…

Optics · Physics 2018-03-20 Zhiwei Guo , Haitao Jiang , Yong Sun , Yunhui Li , Hong Chen

We use helicity-resolved ultrafast transient absorption spectroscopy to study spin-valley polarization dynamics in a vertically stacked MoSe$_{2}$/WSe$_{2}$ heterostructure. The experimental findings reveal details of interlayer charge…

Using first principles many-body theory methods (GW+BSE) we demonstrate that optical properties of graphane are dominated by localized charge-transfer excitations governed by enhanced electron correlations in a two-dimensional dielectric…

Materials Science · Physics 2015-05-18 Pierluigi Cudazzo , Claudio Attacalite , Ilya V. Tokatly , Angel Rubio

Vertical van der Waals (vdW) heterostructures consisting of graphene (Gr) and transition metal dichalcogenides (TMDs) have created a fascinating platform for exploring optical and electronic properties in the two-dimensional limit. Previous…

Transition metal dichalcogenide (TMDC) heterostructures have unique properties that depend on the twisting angle and stacking order of two or more monolayers. However, their practical applications are limited by the low photoluminescence…

Monolayer photonic materials offer a tremendous potential for on-chip optoelectronic devices. Their realization requires knowledge of optical coherence properties of excitons and trions that have so far been limited to nonlinear optical…

Mesoscale and Nanoscale Physics · Physics 2017-12-20 Gabriella D. Shepard , Jenny V. Ardelean , Daniel A. Rhodes , X. -Y. Zhu , James C. Hone , Stefan Strauf

Exact diagonalisations of the extended Hubbard model are performed. In the insulating regime it is shown that the nearest neighbour copper-oxygen repulsion, $V$, leads to Frenkel excitons in the charge transfer gap at values of $V$ of the…

Condensed Matter · Physics 2009-10-28 C. Vermeulen , W. Barford , E. R. Gagliano

Monolayer C$_3$N is an emerging two-dimensional indirect band gap semiconductor with interesting mechanical, thermal, and electronic properties. In this work we present a description of C$_3$N electronic and dielectric properties, focusing…

Mesoscale and Nanoscale Physics · Physics 2022-04-26 Miki Bonacci , Matteo Zanfrognini , Elisa Molinari , Alice Ruini , Marilia J. Caldas , Andrea Ferretti , Daniele Varsano

Two-dimensional transition metal dichalcogenides (TMDs) provide an attractive platform for studying strain dependent exciton transport at room temperature due to large exciton binding energy and strong bandgap sensitivity to mechanical…

Mesoscale and Nanoscale Physics · Physics 2022-03-23 Kanak Datta , Zhengyang Lyu , Zidong Li , Takashi Taniguchi , Kenji Watanabe , Parag B. Deotare

Excitons are composite bosons that can feature spin singlet and triplet states. In usual semiconductors, without an additional spin-flip mechanism, triplet excitons are extremely inefficient optical emitters. Transition metal…

Trilayer graphene is receiving an increasing level of attention due to its stacking--dependent magnetoelectric and optoelectric properties, and its more robust ferromagnetism relative to monolayer and bilayer variants. Additionally,…

Mesoscale and Nanoscale Physics · Physics 2022-06-10 M. F. C. Martins Quintela , N. M. R. Peres

Trions, three-body bound states composed of an exciton and an additional charge, are typically fragile and require external excitation to form. Here, we report the spontaneous emergence of a stable trion gas at the surface of the layered…

We have successfully confined trions into a one-dimensional restricted space of a MoSe2 device with CNT gate electrodes. The dry transfer process, including deterministic dry transfer of aligned CNTs, has led to an hBN-encapsulated MoSe2…

Mesoscale and Nanoscale Physics · Physics 2022-12-28 Takato Hotta , Haruna Nakajima , Shohei Chiashi , Taiki Inoue , Shigeo Maruyama , Kenji Watanabe , Takashi Taniguchi , Ryo Kitaura

Moir\'e superlattices formed by transition metal dichalcogenide (TMD) heterobilayers provide a versatile platform for studying strongly correlated electronic, excitonic, and topological phenomena in solids. In particular, angle-aligned…

We predict here the fine structure of an electrically tunable negatively charged exciton (trion) composed of two electrons and a hole confined in a gated bilayer graphene quantum dot (QD). We start with an atomistic approach, allowing us to…

Mesoscale and Nanoscale Physics · Physics 2025-06-02 Katarzyna Sadecka , Yasser Saleem , Daniel Miravet , Matthew Albert , Marek Korkusinski , Gabriel Bester , Pawel Hawrylak

The formation of well-defined three-dimensional (3D) redox-active molecular nanostructures at the electrode surfaces may open additional routes to achieve higher conductance in molecular junctions (MJs). We report here experimental and…

Materials Science · Physics 2023-11-30 Ritu Gupta , Shapath Bhandari , Savas Kaya , Konstantin P. Katin , Prakash Chandra Mondal

We study a mechanism to induce superconductivity in atomically thin semiconductors where excitons mediate an effective attraction between electrons. Our model includes interaction effects beyond the paradigm of phonon-mediated…

Mesoscale and Nanoscale Physics · Physics 2024-11-28 Jonas von Milczewski , Xin Chen , Atac Imamoglu , Richard Schmidt