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We report the first direct spectroscopic evidence for coherent electronic coupling between excitons and trions in atomically thin transition metal dichalcogenides, specifically monolayer MoSe2. Signatures of coupling appear as isolated…

Mesoscale and Nanoscale Physics · Physics 2014-09-30 Akshay Singh , Galan Moody , Sanfeng Wu , Yanwen Wu , Nirmal J. Ghimire , Jiaqiang Yan , David G. Mandrus , Xiaodong Xu , Xiaoqin Li

The ultrathin transition metal dichalcogenides (TMDs) have emerged as promising materials for various applications using two dimensional (2D) semiconductors. They have attracted increasing attention due to their unique optical properties…

Mesoscale and Nanoscale Physics · Physics 2016-09-20 Aïda Hichri , Imen Ben Amara , Sabrine Ayari , Sihem Jaziri

We report robust room temperature interlayer excitons in transition metal dichalcogenide heterostructures engineered via precise stacking orientation and twist-angle control. We integrate 2H-stacked…

Controlling the flow of charge neutral interlayer exciton (IX) quasiparticles can potentially lead to low loss excitonic circuits. Here, we report unidirectional transport of IXs along nanoscale electrostatically defined channels in an…

Raman scattering and photoluminescence (PL) emission are used to investigate a single layer of tungsten disulfide (WS$_{2}$) obtained by exfoliating n-type bulk crystals. Direct gap emission with both neutral and charged exciton…

Mesoscale and Nanoscale Physics · Physics 2013-12-05 A. A. Mitioglu , P. Plochocka , J. N. Jadczak , W. Escoffier , G. L. J. A. Rikken , L. Kulyuk , D. K. Maude

Despite the weak, van-der-Waals interlayer coupling, photoinduced charge transfer vertically across atomically thin interfaces can occur within surprisingly fast, sub-50fs timescales. Early theoretical understanding of the charge transfer…

Strong Coulomb interaction in atomically-thin transition metal dichalcogenides makes these systems particularly promising for studies of excitonic physics. Of special interest are the manifestations of the charged excitons, also known as…

Mesoscale and Nanoscale Physics · Physics 2020-08-26 M. M. Glazov

We discuss the conditions under which the predicted (but not yet observed) zero-field interlayer excitonic condensation in double layer graphene has a critical temperature high enough to allow detection. Crucially, disorder arising from…

Mesoscale and Nanoscale Physics · Physics 2013-12-16 D. S. L. Abergel , M. Rodriguez-Vega , Enrico Rossi , S. Das Sarma

The combination of repulsive and attractive Coulomb interactions in a quantum electron(e)-hole(h) fluid can give rise to novel correlated phases of multiparticle charge complexes such as excitons, trions and biexcitons. Here we report the…

Harnessing electronic excitations involving coherent coupling to bosonic modes is essential for the design and control of emergent phenomena in quantum materials [1]. In situations where charge carriers induce a lattice distortion due to…

Van der Waals (Vdw) heterostructures constructed from TMDCs provide an ideal platform for exploring various quasiparticle behaviors, with trion-composed of neutral exciton and charged carrier-being a notable example. There are typically…

Mesoscale and Nanoscale Physics · Physics 2024-09-27 Chen Wang , Yu Chen , Qiushi Ma , Peng Suo , Kaiwen Sun , Yifan Cheng , Xian Lin , Weimin Liu , Guohong Ma

A method is presented for optically preparing WS2 monolayers to luminesce from only the charged exciton (trion) state--completely suppressing the neutral exciton. When isolating the trion state, we observed changes in the Raman A1g…

Materials Science · Physics 2016-02-05 M. Currie , A. T. Hanbicki , G. Kioseoglou , B. T. Jonker

Monolayer phosphorene provides a unique two-dimensional (2D) platform to investigate the fundamental dynamics of excitons and trions (charged excitons) in reduced dimensions. However, owing to its high instability, unambiguous…

Materials Science · Physics 2015-04-30 Jiong Yang , Renjing Xu , Jiajie Pei , Ye Win Myint , Fan Wang , Zhu Wang , Shuang Zhang , Zongfu Yu , Yuerui Lu

We present a microscopic many-body calculation of the nonlinear two-dimensional coherent spectroscopy (2DCS) of trion-polaritons and exciton-polaritons in charge-tunable transition-metal-dichalcogenides monolayers placed in an optical…

Quantum Gases · Physics 2025-04-22 Hui Hu , Jia Wang , Riley Lalor , Xia-Ji Liu

Using a combination of ultraviolet-vacuum ultraviolet reflectivity and spectroscopic ellipsometry, we observe a resonant exciton at an unusually high energy of 6.3eV in epitaxial graphene. Surprisingly, the resonant exciton occurs at room…

Controlling excitons and their transport in two-dimensional (2D) transition metal dichalcogenides (TMDs) heterostructures is central to advancing photonics and electronics on-chip integration. We investigate the controlled generation and…

We investigate the transport of excitons and trions in monolayer semiconductor WS$_2$ subjected to controlled non-uniform mechanical strain. We actively control and tune the strain profiles with an AFM-based setup in which the monolayer is…

Mesoscale and Nanoscale Physics · Physics 2020-05-20 Moshe G. Harats , Jan N. Kirchhof , Mengxiong Qiao , Kyrylo Greben , Kirill I. Bolotin

Charged excitons, or trions, offering unique spin and charge degrees of freedom, have primarily been investigated in doped systems where charges are long considered indispensable. Here, we present an alternative route to ultra-efficient…

Mesoscale and Nanoscale Physics · Physics 2026-02-17 N. Fang , U. Erkilic , Y. R. Chang , S. Fujii , D. Yamashita , C. F. Fong , S. Morito , K. Kanahashi , T. Taniguchi , K. Watanabe , K. Ueno , K. Nagashio , Y. K. Kato

Charge doping in transition metal dichalcogenide is currently a subject of high importance for future electronic and optoelectronic applications. Here we demonstrate chemical doping in CVD grown monolayer (1L) of WS2 by a few commonly used…

Mesoscale and Nanoscale Physics · Physics 2020-01-08 Anand P. S. Gaur , Adriana M. Rivera , Saroj P. Dash , Sandwip Dey , Ram S. Katiyar , Satyaprakash Sahoo

The recent accessibility of high quality, charge neutral monolayer transition metal dichalcogenides with narrow exciton linewidths at the homogeneous limit provides an ideal platform to study excitonic many-body interactions. In particular,…