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Methods for reconstructing the spectral density of a vibrational environment from experimental data can yield key insights into the impact of the environment on molecular function. Although such experimental methods exist, they generally…

Chemical Physics · Physics 2025-09-11 Roosmarijn de Wit , Jonathan Keeling , Brendon W. Lovett , Alex W. Chin

Experiments studying vibrational effects on electronic transport through single molecules have observed several seemingly inconsistent behaviors, ranging from up to 30 harmonics of a vibrational frequency in one experiment, to an absence of…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Vivek Aji , J. E. Moore , C. M. Varma

Recent progress in the field of molecular electronics has revealed the fundamental importance of the coupling between the electronic degrees of freedom and specific vibrational modes. Considering the examples of a molecular dimer and a…

Mesoscale and Nanoscale Physics · Physics 2017-02-22 Jakub K. Sowa , Jan A. Mol , G. Andrew D. Briggs , Erik M. Gauger

We consider a double dot system of equivalent, capacitively coupled semiconducting quantum dots, each coupled to its own lead, in a regime where there are two electrons on the double dot. Employing the numerical renormalization group, we…

Strongly Correlated Electrons · Physics 2007-05-23 Martin R. Galpin , David E. Logan , H. R. Krishnamurthy

The zero bias conductance of quantum dots coupled to ferromagnetic leads is investigated. In the strong coupling regime, it is found that the conductance is a non-monotonic function of the angle between the magnetisation directions in the…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 J. Fransson

We discuss the electronic transport through molecules in the Kondo regime. We concentrate here on the influence of molecular vibrations. Two types of vibrations are investigated: (i) the breathing internal molecular modes, where the…

Mesoscale and Nanoscale Physics · Physics 2009-12-21 J. Mravlje , A. Ramsak

Addressing the feasibilty of quantum communication with electrons we consider entangled spin states of electrons in a double-dot which is weakly coupled to in--and outgoing leads. We show that the entanglement of two electrons in the…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 Daniel Loss , Eugene V. Sukhorukov

We study the influence of the phonon environment on the electron dynamics in a doped quantum dot molecule. A non-perturbative quantum kinetic theory based on correlation expansion is used in order to describe both diagonal and off-diagonal…

Mesoscale and Nanoscale Physics · Physics 2015-05-20 A. Grodecka-Grad , J. Förstner

We discuss the topical and fundamental problem of strong-coupling between a quantum dot an the single mode of a microcavity. We report seminal quantitative descriptions of experimental data, both in the linear and in the nonlinear regimes,…

Mesoscale and Nanoscale Physics · Physics 2010-07-12 F. P. Laussy , E. del Valle , A. Gonzalez-Tudela , E. Cancellieri , D. Sanvitto , C. Tejedor

Recent advances in quantum electronics have allowed to engineer hybrid nano-devices comprising on chip a microwave electromagnetic resonator coupled to an artificial atom, a quantum dot. These systems realize novel platforms to explore…

Mesoscale and Nanoscale Physics · Physics 2014-07-25 Marco Schiró , Karyn Le Hur

Electronic transport in a model molecular device coupled to local phonon modes is theoretically analyzed. The method allows for obtaining an accurate approximation of the system's quantum state irrespective of the electron and phonon energy…

Mesoscale and Nanoscale Physics · Physics 2007-10-10 Antonino La Magna , Ioannis Deretzis

When a mesoscopic conductor is coupled to a high-quality electromagnetic cavity the flow of charges and the flux of photons leaking out of the cavity can both depend strongly on the coupled quantum dynamics of the system. Using a…

Mesoscale and Nanoscale Physics · Physics 2016-06-08 Björn Kubala , Joachim Ankerhold , A. D. Armour

Quantum dots are small conductive regions in a semiconductor, containing a variable number of electrons (N=1 to 1000) that occupy well defined discrete quantum states. They are often referred to as artificial atoms with the unique property…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 T. H. Oosterkamp , T. Fujisawa , W. G. van der Wiel , K. Ishibashi , R. V. Hijman , S. Tarucha , L. P. Kouwenhoven

Coherent dynamics of coupled molecules are effectively characterized by the two-dimensional (2D) electronic coherent spectroscopy. Depending on the coupling between electronic and vibrational states, oscillating signals of purely…

Chemical Physics · Physics 2013-10-17 Vytautas Butkus , Donatas Zigmantas , Darius Abramavicius , Leonas Valkunas

We study the interplay between strong electron-electron and electron-phonon interactions within a two-orbital molecule coupled to metallic leads, taking into account Holstein-like coupling of a local phonon mode to the molecular charge as…

Strongly Correlated Electrons · Physics 2013-04-26 G. I. Luiz , E. Vernek , L. Deng , K. Ingersent , E. V. Anda

We study a two-electron quantum dot molecule in a magnetic field by the direct diagonalization of the Hamiltonian matrix. The ground states of the molecule with the total spin S=0 and S=1 provide a possible realization for a qubit of a…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 A. Harju , S. Siljamäki , R. M. Nieminen

We study electron addition spectra of quantum dots in a broad range of electron occupancies starting from the first electron. Spectra for dots containing <200 electrons reveal a surprising feature. Electron additions are not evenly spaced…

Mesoscale and Nanoscale Physics · Physics 2009-10-30 N. B. Zhitenev , R. C. Ashoori , L. N. Pfeiffer , K. W. West

The effect of electron-phonon coupling on the current noise in a molecular junction is investigated within a simple model. The model comprises a 1-level bridge representing a molecular level that connects between two free electron…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Michael Galperin , Abraham Nitzan , Mark A. Ratner

In this paper, we investigate the quantum transport of a double quantum dot coupled with a nanomechanical resonator at arbitrary strong electron-phonon coupling regimes. We employ the generalized quantum master equation to study full…

Mesoscale and Nanoscale Physics · Physics 2012-04-22 Chen Wang , Jie Ren , Baowen Li , Qing-Hu Chen

We present a theory of full counting statistics for electron transport through interacting electron systems with non-Markovian dynamics. We illustrate our approach for transport through a single-level quantum dot and a metallic…

Strongly Correlated Electrons · Physics 2007-05-23 Alessandro Braggio , Jürgen König , Rosario Fazio