Related papers: Pressure-tuning the quantum spin Hamiltonian of th…
We present a combined experimental and theoretical study of the triangular-lattice quantum antiferromagnet CsFeCl$_3$ under high magnetic fields and high pressure. Pulsed-field magnetization for the magnetic field along the symmetric $c$…
Triangular lattice antiferromagnets first attracted attention as a frustrated magnetic lattice which can serve as a platform to realize the resonating valence bond state. While the triangular lattice itself was shown to support classical…
Cs2CuCl4 is known to possess a quantum spin liquid phase with antiferromagnetic interaction below 2.8 K. We report the observation of a new metastable magnetic phase of the triangular frustrated quantum spin system Cs2CuCl4 induced by the…
We report a thorough theoretical study of the low temperature phase diagram of Cs_2CuCl_4, a spatially anisotropic spin S=1/2 triangular lattice antiferromagnet, in a magnetic field. Our results, obtained in a quasi-one-dimensional limit in…
The effects of pressure on a quantum spin liquid are investigated in an organic Mott insulator $\kappa$-(ET)$_2$Ag$_2$(CN)$_3$ with a spin-1/2 triangular lattice. The application of negative chemical pressure to…
The magnetic phase diagram and the thermodynamic properties of a square lattice containing antiferromagnetically coupled spin-1/2 triangles are studied. A Heisenberg Hamiltonian with three strong intra-triangle exchange coupling constants…
We present a study of the magnetic susceptibility $\chi_{mol}$ under variable hydrostatic pressure on single crystals of Cs$_2$CuCl$_{4-x}$Br$_x$. This includes the border compounds \textit{x} = 0 and 4, known as good realizations of the…
Mechanical modulation of the lattice parameter can modify the electronic structure and manipulate the magnetic coupling of a material without introducing impurities. Inspired by success in pressure-controlled magnetism, we investigate the…
The insulating ferrimagnet Cu2OSeO3 shows a rich variety of phases such as skyrmion lattice and helical magnetism controlled by interplay of different exchange interactions which can be tuned by external pressure. In this work we have…
In solid materials, the parameters relevant to quantum effects, such as the spin quantum number, are basically determined and fixed at the chemical synthesis, which makes it challenging to control the amount of quantum correlations. We…
Investigation of materials that exhibit quantum phase transition provides valuable insights into fundamental problems in physics. We present neutron scattering under pressure in a triangular-lattice antiferromagnet which has a quantum…
Magnetic and lattice excitations in the quantum antiferromagnet (C$_4$H$_{12}$N$_2$)Cu$_2$Cl$_6$ (PHCC) are studied across two pressure-induced phase transition at $P_c=4.3~\mathrm{kbar}$ and $P_1=13.4~\mathrm{kbar}$ using Raman…
KCuCl$_3$ is a three dimensionally coupled spin dimer system, which undergoes a pressure-induced quantum phase transition from a gapped ground state to an antiferromagnetic state at a critical pressure of $P_{\rm c} \simeq 8.2$ kbar.…
We present microscopic magnetic properties of a two dimensional triangular lattice Sc2Ga2CuO7, consisting of single and double triangular Cu planes. A Curie-Weiss temperature theta_CW = --44 K and an antiferromagnetic (AFM) exchange…
In the quest for materials with unconventional quantum phases, the organic triangular-lattice antiferromagnet $\kappa$-(ET)$_2$Cu$_2$(CN)$_3$ has been extensively discussed as a quantum spin liquid (QSL) candidate. Recently, an intriguing…
Quantum spin liquids (QSL) are theoretical states of matter with long-range entanglement and exotic quasiparticles. However, they generally elude quantitative theory, rendering their underlying phases mysterious and hampering efforts to…
An experiment demonstrating the quantum simulation of a spin-lattice Hamiltonian is proposed. Dipolar interactions between nuclear spins in a solid state lattice can be modulated by rapid radio-frequency pulses. In this way, the effective…
The effect of pressure ($P$) on magnetic susceptibility of CsCuCl$_3$ was examined in magnetic fields ($\rm \mu_0$$H$) of up to 51 T using a proximity detector oscillator (PDO), and the $H$-$P$ phase diagram of CsCuCl$_3$ was constructed…
Magnetization and neutron elastic scattering measurements under a hydrostatic pressure were performed on KCuCl3, which is a three-dimensionally coupled spin dimer system with a gapped ground state. It was found that an intradimer…
We propose a method for measuring spin Hamiltonians and apply it to the spin-1/2 Heisenberg antiferromagnet Cs2CuCl4, which shows a 2D fractionalized RVB state at low fields. By applying strong fields we fully align the spin moment of…