English
Related papers

Related papers: Stochastic Time-Dependent DFT with Optimally Tuned…

200 papers

We assess a variant of linear-response range-separated time-dependent density-functional theory (TDDFT), combining a long-range Hartree-Fock (HF) exchange kernel with a short-range adiabatic exchange-correlation kernel in the local-density…

Chemical Physics · Physics 2013-05-22 Julien Toulouse , Elisa Rebolini , Tim Gould , John F. Dobson , Prasenjit Seal , János G. Angyán

We present a perturbative approach within the scope of Kohn-Sham density functional theory (DFT). The method is based on the exact exchange-only optimized effective potential method, and correlation is included via perturbation expansion…

Chemical Physics · Physics 2007-05-23 P. Sule

We present a method for simulating the time evolution of one-dimensional correlated electron-phonon systems which combines the time-evolving block decimation algorithm with a dynamical optimization of the local basis. This approach can…

Strongly Correlated Electrons · Physics 2015-12-16 Christoph Brockt , Florian Dorfner , Lev Vidmar , Fabian Heidrich-Meisner , Eric Jeckelmann

Lead-free Cs$_3$Cu$_2$X$_5$ (X = Cl, Br, I) halides exhibit high photoluminescence quantum yields and excellent ambient stability, yet light-emitting devices based on these materials remain limited by poor optical outcoupling. In this work,…

Significant excitonic effects were observed in graphene by measuring its optical conductivity in a broad spectral range including the two-dimensional {\pi}-band saddle-point singularities in the electronic structure. The strong…

Materials Science · Physics 2015-05-20 Kin Fai Mak , Jie Shan , Tony F. Heinz

We explore the merits of linear-response range-separated time-dependent density-functional theory (TDDFT) for the calculation of photoionization spectra. We consider two variants of range-separated TDDFT, namely the timedependent…

Chemical Physics · Physics 2022-06-22 Karno Schwinn , Felipe Zapata , Antoine Levitt , Eric Cancès , Eleonora Luppi , Julien Toulouse

We build an effective field theory (EFT) for quasicrystals -- aperiodic incommensurate lattice structures -- at finite temperature, entirely based on symmetry arguments and a well-define action principle. By means of Schwinger-Keldysh…

High Energy Physics - Theory · Physics 2020-11-04 Matteo Baggioli , Michael Landry

We present the first exact solution for the time dependent equations of the macroscopic fluctuation theory (MFT) for the symmetric simple exclusion process by combining a generalization of the canonical Cole-Hopf transformation with the…

Statistical Mechanics · Physics 2022-08-31 Kirone Mallick , Hiroki Moriya , Tomohiro Sasamoto

Within the Floquet theory of periodically driven quantum systems, we demonstrate that a high-frequency electromagnetic field can be used as an effective tool to control excitonic properties of semiconductor quantum dots (QDs). It is shown,…

Mesoscale and Nanoscale Physics · Physics 2022-04-14 I. V. Iorsh , D. A. Zezyulin , S. A. Kolodny , R. E. Sinitsky , O. V. Kibis

We demonstrate how to apply the tensor-train format to solve the time-independent Schr\"{o}dinger equation for quasi one-dimensional excitonic chain systems with and without periodic boundary conditions. The coupled excitons and phonons are…

Computational Physics · Physics 2023-02-09 Patrick Gelß , Rupert Klein , Sebastian Matera , Burkhard Schmidt

We discuss how excitons can affect the generation of coherent radial breathing modes in ultrafast spectroscopy of single wall carbon nanotubes. Photoexcited excitons can be localized spatially and give rise to a spatially distributed…

This chapter concerns with the recent development of a new DFT methodology for accurate, reliable prediction of many-electron systems. Background, need for such a scheme, major difficulties encountered, as well as their potential remedies…

Chemical Physics · Physics 2019-04-19 Amlan K. Roy

The multiconfiguration time-dependent Hartree-Fock (MCTDHF) method is formulated for treating the coupled electronic and nuclear dynamics of diatomic molecules without the Born- Oppenheimer approximation. The method treats the full…

Computational Physics · Physics 2015-05-27 Daniel J. Haxton , Keith V. Lawler , C. William McCurdy

Dielectric screening is greatly important to an accurate calculation of the exciton binding energies in two-dimensional materials. In this work, we calculate the dielectric function and 2D polarizability of multilayer (up to three)…

Mesoscale and Nanoscale Physics · Physics 2017-08-03 M. A. Lino , J. S. de Sousa , D. R. da Costa , A. Chaves , J. M. Pereira , G. A. Farias

The dynamics of an electron--hole pair induced by the time--dependent screened Coulomb interaction is discussed. In contrast to the case where the static electron--hole interaction is considered we demonstrate the occurrence of important…

Materials Science · Physics 2009-11-10 Andrea Marini , Rodolfo Del Sole

Kohn-Sham Density Functional Theory (KS-DFT) has been traditionally solved by the Self-Consistent Field (SCF) method. Behind the SCF loop is the physics intuition of solving a system of non-interactive single-electron wave functions under…

The increasing need to simulate the dynamics of photoexcited molecular and nanosystems in the sub-picosecond regime demands new efficient tools able to describe the quantum nature of matter at a low computational cost. By combining the…

We study the lattice dynamics of iron superconductor FeSe, and address the fundamental question of how important is proper description of fluctuating magnetic moments in metallic systems for phonon dispersion and phonon density of states.…

Strongly Correlated Electrons · Physics 2021-01-04 Ghanashyam Khanal , Kristjan Haule

Integrated photonics provides an important platform for simulating physical models with high-performance chip-scale devices, where the lattice size and the time-dependence of a model are key ingredients for further enriching the…

Classical Density Functional Theory (DFT) is a statistical-mechanical framework to analyze fluids, which accounts for nanoscale fluid inhomogeneities and non-local intermolecular interactions. DFT can be applied to a wide range of…

Computational Engineering, Finance, and Science · Computer Science 2017-02-07 Andreas Nold , Benjamin D. Goddard , Peter Yatsyshin , Nikos Savva , Serafim Kalliadasis