Related papers: Anisotropy Control in Photoelectron Spectra: A Coh…
We measure the photoionization cross-section of vibrationally excited levels in the S2 state of azulene by femtosecond pump-probe spectroscopy. At the wavelengths studied (349-265 nm in the pump) the transient signals exhibit two distinct…
Characterizing time delays in molecular photoionization as a function of the ejected electron emission direction relative to the orientation of the molecule and the light polarization axis pro-vides unprecedented insights into the…
The time-dependent Schr\"{o}dinger equation for the hydrogen atom and its interaction with coherent intense high-frequency short laser pulses is solved numerically exactly by propagating the single-electron wave packets. Thereby, the…
Double-slit diffraction studies with photons or massive particles rank among the most beautiful experiments in physics. In particular, measurements at very low intensities demonstrate the particle-wave duality and the coherent superposition…
Entanglement is one of the most intriguing aspects of quantum mechanics and lies at the heart of the ongoing Second Quantum Revolution, where it is a resource that is used in quantum key distribution, quantum computing and quantum…
A theoretical study of the interference pattern imprinted on the doubly differential momentum distribution of the photoelectron due to atomic ionization induced by a short laser pulse is developed from a semiclassical standpoint. We use the…
We present and implement a new scheme for independent control of both the final and the transient population utilizing the symmetry properties of the system. By proper pulse shaping, utilizing the invariance of the two-photon absorption to…
Time-resolved X-ray scattering patterns from photoexcited molecules in solution are in many cases anisotropic at the ultrafast time scales accessible at X-ray Free Electron Lasers (XFELs). This anisotropy arises from the interaction of a…
We report fully differential photoelectron spectra from an {\it ab-inito} coupled channels treatment of CO$_2$. Photoionization by laser pulses centered at 400 nm and 800 nm wavelength are considered, with arbitrary molecular alignment and…
Quantum coherence between electronic states of a photoionized molecule and the resulting process of ultrafast electron-hole migration have been put forward as a possible quantum mechanism of charge-directed reactivity governing the…
Shaped pulses obtained by optimal control theory often possess unphysically broad spectra. In principle, the spectral width of a pulse can be restricted by an additional constraint in the optimization functional. However, it has so far been…
The ionization of atoms with sequences of attosecond pulses gives rise to excited ionic states that are entangled with the emitted photoelectron. Still, the ionic ensemble preserves some coherence that can be controlled through the laser…
Few-cycle pulses of intense 800 nm light are used to probe ionization and dissociation of carbon disulfide in the intensity and temporal regime where rescattering is expected to dominate the laser-molecule interaction. The wavepacket of the…
A Ramsey-type interferometer is suggested, employing a cold trapped ion and two time-delayed off-resonant femtosecond laser pulses. The laser light couples to the molecular polarization anisotropy, inducing rotational wavepacket dynamics.…
Coherent manipulation of single-photon wave packets is essentially important for optical quantum communication and quantum information processing. In this paper, we realize controllable splitting and modulation of single-photon-level pulses…
The ability of an environment to assist in one-photon phase control relies upon entanglement between the system and bath and on the breaking of the time reversal symmetry. Here, one photon phase control is examined analytically and…
While the spontaneous emission from independent emitters provides spatially uncorrelated photons - a typical manifestation of quantum randomness, the interference of the coherent scattering leads to a well-defined intensity pattern - a…
Ionization of atoms and molecules by absorption of a light pulse results in electron wavepackets carrying information on the atomic or molecular structure as well as on the dynamics of the ionization process. These wavepackets can be…
We address nonsequential double ionization induced by strong, linearly polarized laser fields of only a few cycles, considering a physical mechanism in which the second electron is dislodged by the inelastic collision of the first electron…
Owing to its numerical simplicity, a two-dimensional two-electron model atom, with each electron moving in one direction, is an ideal system to study non-perturbatively a fully correlated atom exposed to a laser field. Frequently made…