Related papers: Spatiotemporal imaging of valence electron motion
We use ultrafast electron crystallography to study structural changes induced in graphite by a femtosecond laser pulse. At moderate fluences of ~< 21mJ/cm^2, lattice vibrations are observed to thermalize on a time scale of ~8ps. At higher…
We demonstrate that electrons can be efficiently accelerated to high energy in spatially non-uniform, intense laser fields. Laser non-uniformities occur when a perfect plane wave reflects off a randomly perturbed surface. By solving for…
Ultrahigh peak power femtosecond laser pulses create extreme states of matter that are currently being probed with great interest. Plasma optics have been proposed for shaping and amplifying high-power pulses, but they are subject to huge…
Quantum coherence between electronic states of a photoionized molecule and the resulting process of ultrafast electron-hole migration have been put forward as a possible quantum mechanism of charge-directed reactivity governing the…
The motion of chemical bonds within molecules can be observed in real time, in the form of vibrational wavepackets prepared and interrogated through ultrafast nonlinear spectroscopy. Such nonlinear optical measurements are commonly…
We propose a continuous variable quantum state tomography protocol of electrons which result from the ionization of atoms or molecules by the absorption of extreme ultraviolet light pulses. Our protocol is benchmarked against a direct…
We present a combined numerical and theoretical study of atomic photoionization in the time domain. We show how a photoelectron wave packet rapidly changes its shape after being emitted, from a complex multi-peak structure to eventually a…
Efficient energy transfer from electromagnetic waves to ions has been demanded to control laboratory plasmas for various applications and could be useful to understand the nature of space and astrophysical plasmas. However, there exists a…
High frequency modulations appearing in the kinetic energy distribution of laser accelerated ions are proposed for retrieving the acceleration field dynamics at femtosecond time scale. Such an approach becomes possible if the laser-cycling…
The complex interaction dynamics of intense femtosecond (fs) pulses and their picosecond (ps)-long leading edge with nanostructured solids occur at both the nanometer and the femtosecond scales, making them extremely difficult to measure…
The use of electric fields for signalling and control in liquids is widespread, spanning bioelectric activity in cells to electrical manipulation of microstructures in lab-on-a-chip devices. However, an appropriate tool to resolve the…
Solitons are self-sustained wavepackets that occur in many physical systems. Their recent demonstration in optical microresonators has provided a new platform for study of nonlinear optical physics with practical implications for…
The basic properties of atoms, molecules and solids are governed by electron dynamics which take place on extremely short time scales. To measure and control these dynamics therefore requires ultrafast sources of radiation combined with…
The dynamics of solvated electrons were visualized using absorption imaging with sub-picosecond time resolution based on a pump-probe measurement during the early stages of femtosecond laser-induced plasma generation in water. The solvated…
X-ray photoelectron diffraction is a powerful tool for determining the structure of clean and adsorbate-covered surfaces. Extending the technique into the ultrafast time domain will open the door to studies as diverse as the direct…
Visualizing ultrafast dynamics at the atomic scale requires time-resolved pump-probe characterization with femtosecond temporal resolution. For single-shot ultrafast electron diffraction (UED) with fully relativistic electron bunch probes,…
We simulate, using a particle-in-cell code, the chain of acceleration processes at work during the Compton-based interaction of a dilute electron-ion plasma with an extreme-intensity, incoherent gamma-ray flux with a photon density several…
The nonlinear interaction of x-rays with matter is at the heart of understanding and controlling ultrafast molecular dynamics from an atom-specific viewpoint, providing new scientific and analytical opportunities to explore the structure…
Ultrashort light pulses are ubiquitous in modern research, but the electromagnetic field of the optical cycles is usually not easy to obtain as a function of time. Field-resolved pulse characterization requires either a nonlinear-optical…
Approaching energy coupling in laser-irradiated metals, we point out the role of electron-electron collision as an efficient control factor for ultrafast optical absorption. The high degree of laser-induced electron-ion nonequilibrium…