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Disordered magnetic states known as spin liquids are of paramount importance in both fundamental and applied science. A classical state of this kind was predicted for the Ising antiferromagnetic triangular model more than half a century…
Recent experiments on the dipolar-octupolar pyrochlore compound Ce$_2$Zr$_2$O$_7$ indicate that it may realize a three-dimensional quantum spin liquid (QSL). In particular, the analyses of available data suggest that the system is in a…
Quantum spin liquids have been at the forefront of correlated electron research ever since their original proposal in 1973, and the realization that they belong to the broader class of intrinsic topological orders, along with the fractional…
We study quantum disordered ground states of the two dimensional Heisenberg-Kitaev model on the triangular lattice using a Schwinger boson approach. Our aim is to identify and characterize potential gapped quantum spin liquid phases that…
Quantum spin liquids may be considered "quantum disordered" ground states of spin systems, in which zero point fluctuations are so strong that they prevent conventional magnetic long range order. More interestingly, quantum spin liquids are…
A quantum spin liquid (QSL) is a state of matter where unpaired electrons' spins in a solid are quantum entangled, but do not show magnetic order in the zero-temperature limit. Because such a state may be important to the microscopic origin…
In this study, we performed high-magnetic-field magnetization, dielectric, and ultrasound measurements on an organic salt showing a ferroelectric spin-Peierls (FSP) state, which is in close proximity to a quantum critical point. In contrast…
Based on experimental data and our theoretical analysis, we provide a strategy for unambiguous establishing of gapless quantum spin liquid state (QSL) in herbertsmithite and other materials. To clarify the nature of QSL, we recommend…
At sufficiently low temperatures, condensed-matter systems tend to develop order. An exception are quantum spin-liquids, where fluctuations prevent a transition to an ordered state down to the lowest temperatures. While such states are…
Quantum spin liquids (QSLs) form an extremely unusual magnetic state in which the spins are highly correlated and fluctuate coherently down to the lowest temperatures, but without symmetry breaking and without the formation of any static…
In the quest for materials with unconventional quantum phases, the organic triangular-lattice antiferromagnet $\kappa$-(ET)$_2$Cu$_2$(CN)$_3$ has been extensively discussed as a quantum spin liquid (QSL) candidate. Recently, an intriguing…
Organic solids host various electronic phases. Especially, a milestone compound of organic solid, $\beta'$-$X$[Pd(dmit)$_2$]$_2$ with $X$=EtMe$_3$Sb shows quantum spin-liquid (QSL) properties suggesting a novel state of matter. However,…
Experimental quest for the hypothetical "quantum spin liquid" state has recently met a few promising candidate materials including organic salts \kappa-(ET)2Cu2(CN)3 and EtMe3Sb[Pd(dmit)2]2, S=1/2 triangular-lattice Heisenberg…
A quantum spin liquid (QSL) is a novel phase of matter with long-range entanglement where localized spins are highly correlated with the vanishing of magnetic order. Such exotic quantum states provide the opportunities to develop new…
Hydrogen in metals has attracted much attention for a long time from both basic scientific and technological points of view. Its electronic state has been investigated in terms of a proton embedded in the electron gas mostly by the local…
Quantum spin ice is an appealing proposal of a quantum spin liquid - systems where the magnetic moments of the constituent electron spins evade classical long-range order to form an exotic state that is quantum entangled and coherent over…
The Ce$^{3+}$ pseudospin-$\frac{1}{2}$ degrees of freedom in the pyrochlore magnet Ce$_2$Zr$_2$O$_7$ are known to possess dipole-octupole (DO) character, making it a candidate for novel quantum spin liquid (QSL) ground states at low…
Quantum fluctuations enhanced by frustration and subtle interplay between competing degrees of freedom offer an ideal ground to realize novel states with fractional quantum numbers in quantum materials that defy standard theoretical…
A three-dimensional system of interacting spins typically develops static long-range order when it is cooled. If the spins are quantum (S = 1/2), however, novel quantum paramagnetic states may appear. The most highly sought state among them…
While many-body systems can host long-ranged entangled quantum spin liquids (QSLs), the ingredients for realizing these as ground states can be prohibitively difficult. In many circumstances, one requires (i) a constrained Hilbert space and…