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We report a study of magnetic dynamics in multiferroic hexagonal manganite HoMnO3 by far-infrared spectroscopy. Low-temperature magnetic excitation spectrum of HoMnO3 consists of magnetic-dipole transitions of Ho ions within the…

Materials Science · Physics 2009-11-13 D. Talbayev , A. D. LaForge , S. A. Trugman , N. Hur , A. J. Taylor , R. D. Averitt , D. N. Basov

We used Raman scattering to study the lattice and magnetic excitations in the hexagonal HoMnO3 single crystals. The E2 phonon mode at 237 cm-1 is affected by the magnetic order. This mode is related to the displacement of Mn and O ions in…

Strongly Correlated Electrons · Physics 2018-10-17 J. Liu , Y. Gallais , M-A. Measson , A. Sacuto , S. W. Cheong , M. Cazayous

Lattice and spin excitations have been studied by Raman scattering in hexagonal YbMnO3 single crystals. The temperature dependences of the phonon modes show that the E2 mode at 256 cm-1 related to the displacement of Mn and O ions in a-b…

Strongly Correlated Electrons · Physics 2012-11-12 J. Liu , C. Toulouse , P. Rovillain , M. Cazayous , Y. Gallais , M. -A. Measson , S. W. Cheong , N. Lee , A. Sacuto

Polarized Raman scattering and infrared reflection spectra of hexagonal HoMnO$_3$ single crystals in the temperature range 10-300 K are reported. Group-theoretical analysis is performed and scattering selection rules for the second order…

Strongly Correlated Electrons · Physics 2009-11-10 A. P. Litvinchuk , M. N. Iliev , V. N. Popov , M. M. Gospodinov

InMnO$_3$ is a peculiar member of the hexagonal manganites h-RMnO$_3$ (where R is a rare earth metal element), showing crystalline, electronic and magnetic properties at variance with the other compounds of the family. We have studied high…

Materials Science · Physics 2015-03-19 X. Fabrèges , I. Mirebeau , S. Petit , P. Bonville , A. A. Belik

Local structural measurements have been performed on hexagonal HoMnO3 in order to ascertain the specific changes in bond distances which accompany magnetic ordering transitions. The transition from paramagnetic to the antiferromagetic…

Strongly Correlated Electrons · Physics 2015-05-14 T. A. Tyson , T. Wu , K. H. Ahn , S. Kim , S. -W. Cheong

The dielectric constant of multiferroic hexagonal HoMnO_3 exhibits an unprecedented diversity of anomalies at low temperatures (1.8 K< T <10 K) and under external magnetic fields related to magnetic phase transitions in the coupled system…

Strongly Correlated Electrons · Physics 2009-11-11 F. Yen , C. R. dela Cruz , B. Lorenz , Y. Y. Sun , Y. Q. Wang , M. M. Gospodinov , C. W. Chu

Hexagonal Dy(0.5)Y(0.5)MnO3, a multiferroic rare-earth manganite with geometrically frustrated antiferromagnetism, has been investigated with single-crystal neutron diffraction measurements. Below 3.4 K magnetic order is observed on both…

Strongly Correlated Electrons · Physics 2011-08-29 Joel S. Helton , Deepak K. Singh , Harikrishnan S. Nair , Suja Elizabeth

Multiferroic rare earth manganites attracted recent attention because of the coexistence of different types of magnetic and ferroelectric orders resulting in complex phase diagrams and a wealth of physical phenomena. The coupling and mutual…

Strongly Correlated Electrons · Physics 2007-05-23 B. Lorenz , C. R. dela Cruz , F. Yen , Y. Q. Wang , Y. Y. Sun , C. W. Chu

HoFe1-xMnxO3 (0 < x < 1) single crystals have been grown by the optical floating zone technique. A structural transition from the orthorhombic to hexagonal modification has been established in the crystals in the concentration range of…

Spin-phonon coupling, the interaction of spins with surrounding lattice is a key parameter to understand the underlying physics of multiferroics and engineer their magnetization dynamics. Elementary excitations in multiferroic materials are…

Materials Science · Physics 2020-11-05 Bommareddy Poojitha , Anjali Rathore , Ankit Kumar , Surajit Saha

The low energy dynamical properties of the multiferroic hexagonal perovskite ErMnO3 have been studied by inelastic neutron scattering as well as terahertz and far infrared spectroscopies on synchrotron source. From these complementary…

Neutron scattering results are presented for spin-wave excitations of three ferromagnetic metallic $A_{1-x}A^{\prime}_{x}$MnO$_3$ manganites (where $A$ and $A^\prime$ are rare- and alkaline-earth ions), which when combined with previous…

Strongly Correlated Electrons · Physics 2007-05-23 F. Ye , Pengcheng Dai , J. A. Fernandez-Baca , Hao Sha , J. W. Lynn , H. Kawano-Furukawa , Y. Tomioka , Y. Tokura , Jiandi Zhang

Hexagonal HoMnO$_{3}$ is a frustrated antiferromagnet (T$_{N}$=72 K) ferroelectric (T$_{C}$=875 K) in which these two order parameters are coupled. Our neutron measurements of the spin wave dispersion for the S=2 Mn$^{3+}$ on the layered…

Strongly Correlated Electrons · Physics 2009-11-11 O. P. Vajk , M. Kenzelmann , J. W. Lynn , S. B. Kim , S. -W. Cheong

Strong magnetic-ferroelectric coupling in hexagonal HoMnO3 has been observed previously at spin reorientation temperature between P6'3cm' and the P6'3cm' magnetic phases. In contrast, YMnO3 has only a single magnetic phase (P6'3cm') and no…

Strongly Correlated Electrons · Physics 2013-03-26 Jagath Gunasekera , Owen P. Vajk , Yuan Wang , Kevin Tarwater , Tom W. Heitmann

A series of manganites Tb1-xHoxMnO3 (0<=x<=0.6) with orthorhombic structure are synthesized and detailed investigations on their multiferroicity are performed. Successive magnetic transitions upon temperature variation are evidenced for all…

Strongly Correlated Electrons · Physics 2010-04-19 C. L. Lu , S. Dong , K. F. Wang , J. -M. Liu

X-ray resonant magnetic scattering studies of rare earth magnetic ordering were performed on perovskite manganites RMnO3 (R = Dy, Gd) in an applied magnetic field. The data reveal that the field-induced three-fold polarization enhancement…

We report on the spin waves and crystal field excitations in single crystal LiFePO$_4$ by inelastic neutron scattering over a wide range of temperatures, below and above the antiferromagnetic transition of this system. In particular, we…

Strongly Correlated Electrons · Physics 2017-03-15 Yuen Yiu , Manh Duc Le , Rasmus Toft-Peterson , Georg Ehlers , Robert McQueeney , David Vaknin

We present data on the magnetic and magneto-elastic coupling in the hexagonal multiferroic manganite LuMnO3 from inelastic neutron scattering, magnetization and thermal expansion measurements. We measured the magnon dispersion along the…

Strongly Correlated Electrons · Physics 2010-12-01 H. J. Lewtas , A. T. Boothroyd , M. Rotter , D. Prabhakaran , H. Mueller , M. D. Le , B. Roessli , J. Gavilano , P. Bourges

Symmetry arguments are used to develop a spin Hamiltonian for the description of the complex magnetic ordering in HoMnO$_3$. Using a novel application of the Landau Lifshitz Gilbert dynamic torque equations to this model of the frustrated…

Strongly Correlated Electrons · Physics 2012-02-13 S. G. Condran , M. L. Plumer
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