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Interactions between electrons and lattice vibrations are responsible for a wide range of material properties and applications. Recently, there has been considerable interest in the development of resonant inelastic x-ray scattering (RIXS)…

A new experimental setup combining X-Ray Photon Correlation Spectroscopy (XPCS) in the hard x-ray regime and a high-pressure sample environment is developed to monitor the pressure dependence of the internal motion of complex systems down…

The surface sensitivity and probe depth in the x-ray regime of diamond for second harmonic generation (SHG) was investigated both analytically and computationally with velocity gauge real-time time-dependent density functional theory…

Materials Science · Physics 2026-04-22 Daniel Schacher , Tod A. Pascal , Keith V. Lawler , Craig P. Schwartz

Optical second-harmonic generation (SHG) is a nonlinear parametric process that doubles the frequency of incoming light. Only allowed in non-centrosymmetric materials, it has been widely used in frequency modulation of lasers, surface…

Materials Science · Physics 2021-01-05 Wontaek Kim , Je Yhoung Ahn , Juseung Oh , Ji Hoon Shim , Sunmin Ryu

High-harmonic generation (HHG) in solids has typically been explored in transparent dielectrics and semiconductors. Metals have long been dismissed due to their strong reflectivity at infrared wavelengths. Here, we demonstrate HHG from…

Under infrared ultrashort pulse laser stimulation, we investigated temperature-dependent second-harmonic generation (SHG) from nitrogen-vacancy (NV)-introduced bulk diamond. The SHG intensity decreases in the temperature range of 20-300…

Optics · Physics 2022-04-05 Aizitiaili Abulikemu , Yuta Kainuma , Toshu An , Muneaki Hase

Since the advent of x-ray free-electron lasers (XFELs), considerable efforts have been devoted to achieve x-ray pulses with better temporal coherence. Here, we put forward a scheme to generate fully coherent x-ray lasers (XRLs) based on…

Atomic Physics · Physics 2018-01-09 Chunhai Lyu , Stefano M. Cavaletto , Christoph H. Keitel , Zoltán Harman

The LUXE experiment aims at studying high-field QED in electron-laser and photon-laser interactions, with the 16.5 GeV electron beam of the European XFEL and a laser beam with power of up to 350 TW. The experiment will measure the spectra…

Instrumentation and Detectors · Physics 2021-12-20 O. Borysov

The European X-ray Free Electron Laser (XFEL) will deliver 30,000 fully coherent, high brilliance X-ray pulses per second each with a duration below 100 fs. This will allow the recording of diffraction patterns of single complex molecules…

Instrumentation and Detectors · Physics 2015-06-03 Jiaguo Zhang , Eckhart Fretwurst , Robert Klanner , Hanno Perrey , Ioana Pintilie , Thomas Poehlsen , Joern Schwandt

The advent of isolated and intense sub-femtosecond X-ray pulses enables tracking of quantummechanical motion of electrons in molecules and solids. The combination of X-ray spectroscopy and diffraction imaging is a powerful approach to…

The generation of harmonic radiation through a non-linear mechanism driven by bunching at fundamental frequency is an important option in the operation of high gain Free-Electron Lasers (FELs). The use of harmonic generation at a large…

Accelerator Physics · Physics 2016-09-08 Gianluca Geloni , Evgeni Saldin , Evgeni Schneidmiller , Mikhail Yurkov

We consider the elastic scattering of electrons by hydrogen atoms in the presence of a two-color circularly polarized laser field in the domain of moderate intensities below $10^{13}$ W/cm$^2$ and high projectile energies. A hybrid approach…

Atomic Physics · Physics 2023-06-16 Gabriela Buica

High-brightness femtosecond-to-attosecond pulses are indispensable for probing electron dynamics on their fundamental temporal scales. X-ray free-electron lasers (XFELs) at high repetition rates will facilitate high-statistics measurements…

Accelerator Physics · Physics 2026-05-01 Junhao Liu , Zhen Wang , Lanpeng Ni , Yujie Lu , Chao Feng , Zhentang Zhao

Sub-femtosecond x-ray burst is powerful tool for probing and imaging electronic and concomitant atomic motion in attosecond physics. For years, x-ray source (above 2 keV) had mainly been obtained from X-ray free electron laser (XFEL) or…

X-ray free electron laser (XFEL) can provide X-ray light with about four order of magnitude higher flux than synchrotron radiation. Pulse light from XFEL interacts with the target and the resulting photons are collected by detectors. The…

Instrumentation and Detectors · Physics 2021-10-13 Shuo Zhang , Jing-Kai Xia , Xu-Dong Ju

X-ray free electron lasers (XFELs) generate sequences of ultra-short, spatially coherent pulses of x-ray radiation. We propose the diffraction focusing spectrometer (DFS), which is able to measure the whole energy spectrum of the radiation…

Optics · Physics 2013-02-22 V. G. Kohn , O. Y. Gorobtsov , I. A. Vartanyants

X-ray free-electron lasers (XFELs) are cutting-edge scientific instruments for a wide range of disciplines. Conventionally, the narrow bandwidth is pursued in an XFEL. However, in recent years, the large-bandwidth XFEL operation schemes are…

Accelerator Physics · Physics 2019-02-27 Jiawei Yan , Haixiao Deng

In this work we provide theoretical background for the analysis of second-order correlation functions in experiments performed at the soft x-ray free-electron lasers (XFELs). Typically, soft x-ray beamlines at XFELs are equipped by the…

Optics · Physics 2021-08-18 Ivan A. Vartanyants , Ruslan Khubbutdinov

X-ray free-electron lasers (FELs) are promising tools for structural determination of macromolecules via coherent x-ray scattering. During ultrashort and ultraintense x-ray pulses with an atomic scale wavelength, samples are subject to…

Atomic Physics · Physics 2011-10-18 Sang-Kil Son , Linda Young , Robin Santra