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Magnetic van der Waals (vdW) materials offer a fantastic platform to investigate and exploit rich spin configurations stabilized in reduced dimensions. One tantalizing magnetic order is the interlayer antiferromagnetism in A-type vdW…

Recent research has revealed remarkable properties of the two-dimensional (2D) van der Waals layered crystal CrSBr, which is both a semiconductor and an A-type antiferromagnet. Here we show the role of strong magnetoelastic coupling in the…

Spin spirals form inside the magnetic layers of antiferromagnetic and noncollinearly-coupled magnetic multilayers in the presence of an external magnetic field. This spin structure can be modeled to extract the direct exchange stiffness of…

Mesoscale and Nanoscale Physics · Physics 2024-09-04 Elliot Wadge , Afan Terko , George Lertzman-Lepofsky , Paul Omelchenko , Bret Heinrich , Manuel Rojas , Erol Girt

CrCl3, a layered van der Waals (vdW) magnet, exhibits in-plane magnetic anisotropy and enhanced interlayer coupling upon stacking, making it an ideal platform to host exotic nanoscale magnetic phenomena such as magnon hydrodynamics and…

CrI3, which belongs to a rare category of two-dimensional (2D) ferromagnetic semiconductors, is of great interest for spintronic device applications. Unlike CrCl3 whose magnetism presents a 2D-Heisenberg behavior, CrI3 exhibits a larger van…

Materials Science · Physics 2018-03-14 G. T. Lin , X. Luo , F. C. Chen , J. Yan , J. J. Gao , Y. Sun , W. Tong , P. Tong , W. J. Lu , Z. G. Sheng , W. H. Song , X. B. Zhu , Y. P. Sun

The layered metamagnet CrSBr offers a rich interplay between magnetic, optical and electrical properties that can be extended down to the two-dimensional (2D) limit. Despite the extensive research regarding the long-range magnetic order in…

The degree of electronic coupling between individual layers in few-layer van der Waals heterostructures offers a route to engineer their magnetic, electronic, and optical functionalities. Using state-of-the-art first-principles…

Materials Science · Physics 2026-01-21 Sijia Ke , Yusuf Shaidu , Jeffrey B. Neaton

Bulk chromium triiodide (CrI$_3$) has long been known as a layered van der Waals ferromagnet. However, its monolayer form was only recently isolated and confirmed to be a truly two-dimensional (2D) ferromagnet, providing a new platform for…

Two-dimensional (2D) magnetic materials are promising candidates for spintronics and quantum technologies. One extensively studied example is the ferromagnetic (FM) CrI$_3$ monolayer with the honeycomb Cr$^{3+}$ ($t_{2g}^3$, $S$ = 3/2) spin…

Materials Science · Physics 2025-04-17 Ke Yang , Yueyue Ning , Yaozhenghang Ma , Yuxuan Zhou , Hua Wu

Layered chromium tellurides are model systems for studying low-dimensional magnetism in van der Waals materials. We report the synthesis and characterization of K$_{1-x}$CrTe$_2$ single crystals ($x \approx 0.3$), which crystallize in the…

Motivated by the recent experimental developments in van der Waals heterostructures, we investigate the emergent magnetism in Mott insulator - semimetal moir\'e superlattices by deriving effective spin models and exploring their phase…

Strongly Correlated Electrons · Physics 2024-11-05 M. A. Keskiner , Pouyan Ghaemi , M. Ö. Oktel , Onur Erten

Long-range magnetic orders in atomically thin ferromagnetic CrI3 give rise to new fascinating physics and application perspectives. The physical properties of two-dimensional (2D) ferromagnetism CrI3 are significantly influenced by…

Materials Science · Physics 2019-11-13 Kai Guo , Bowen Deng , Zhongtai Shi , Yue Li , Xin Wang , Lei Bi , Li Zhang , Haipeng Lu , Peiheng Zhou , Linbo Zhang , Yingchun Cheng , Bo Peng

External pressure suppresses the ferromagnetism of localized Cr 3d electron moments in the van der Waals insulator CrBr3, which cannot be explained without considering a dramatic pressure-induced crystal or electronic structure change. We…

CrI3 is a layered ferromagnetic insulator that has recently attracted enormous interest as it was the first example of a stand-alone monolayer ferromagnet, paving the way towards the study of two-dimensional magnetic materials and their use…

We identify a "twin-twist" angle in orthorhombic two-dimensional magnets that maximizes interlayer orbital overlap and enables strong interfacial coupling. Focusing on the van der Waals antiferromagnet CrSBr, we show that this twist angle,…

Despite serious effort, the nature of the magnetic interactions and the role of electron-correlation effects in magnetic two-dimensional (2D) van der Waals materials remain elusive. Using CrI$_3$ as a model system, we show that the…

Materials Science · Physics 2021-02-04 Liqin Ke , Mikhail I. Katsnelson

Atomically thin chromium triiodide (CrI3) has recently been identified as a layered antiferromagnetic insulator, in which adjacent ferromagnetic monolayers are antiferromagnetically coupled. This unusual magnetic structure naturally…

Moir\'e magnetism featured by stacking engineered atomic registry and lattice interactions has recently emerged as an appealing quantum state of matter at the forefront condensed matter physics research. Nanoscale imaging of moir\'e magnets…

Exchange-coupled interfaces are pivotal in exploiting two-dimensional (2D) ferromagnetism. Due to the extraordinary correlations among charge, spin, orbital and lattice degrees of freedom, layered magnetic transition metal chalcogenides…

The crystallographic, magnetic, and transport properties of the van der Waals bonded, layered compound CrTe3 have been investigated on single crystal and polycrystalline materials. The crystal structure contains layers made up of lozenge…

Strongly Correlated Electrons · Physics 2017-04-19 Michael A. McGuire , V. Ovidiu Garlea , Santosh KC , Valentino R. Cooper , Jiaqiang Yan , Huibo Cao , Brian C. Sales