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The Mott insulator $\alpha$-RuCl$_3$ has generated great interest in the community due to its possible field-induced Kitaev quantum spin liquid state. Despite enormous effort spent trying to obtain the form of the low energy Hamiltonian,…

The isostructural series of $S=1$ quantum magnets Cs$_{1-x}$Rb$_{x}$FeCl$_{3}$ is investigated, using both thermodynamic measurements and inelastic neutron scattering experiments. It is found that increasing Rb content the system evolves…

Strongly Correlated Electrons · Physics 2019-12-11 S. Hayashida , L. Stoppel , Z. Yan , S. Gvasaliya , A. Podlesnyak , A. Zheludev

$\alpha$-RuCl$_3$ has been extensively studied recently because of potential bond-dependent Kitaev magnetic exchange interactions and the resulting quantum spin liquid phase that can be realized therein. It has been known that the covalency…

Strongly Correlated Electrons · Physics 2022-01-13 Heung-Sik Kim

$\alpha$-RuCl3 is a magnetic insulator exhibiting quantum spin liquid phases possibly found in the Kitaev honeycomb model. Much of the effort towards determining Hamiltonian parameters has focused on low magnetic field ordered phases. We…

Strongly Correlated Electrons · Physics 2023-01-05 Michael J. Lawler , Kimberly A. Modic , B. J. Ramshaw

We study excitations in weakly interacting pairs of quantum spin ladders coupled through geometrically frustrated bonds. The ground state is a disordered spin liquid, that at high fields is replaced by an ordered chiral helimagnetic phase.…

Strongly Correlated Electrons · Physics 2015-05-14 A. Zheludev , V. O. Garlea , A. Tsvelik , L. -P. Regnault , K. Habicht , K. Kiefer , B. Roessli

$\alpha$-RuCl$_3$ is a leading material for proximate Kitaev magnetism. We address the origin of the broad, $\Gamma$-point centered excitation continuum observed by inelastic neutron scattering at elevated temperatures in this compound.…

Materials Science · Physics 2026-02-12 Chaebin Kim , Martin Mourigal

Inspired by experiments on the magnetic field induced phases of the spin-orbit coupled $2d$ Mott insulator $\alpha$-RuCl$_3$, we study some general aspects of gapped $Z_2$ Quantum Spin Liquids (QSL) enriched by lattice translation symmetry.…

Strongly Correlated Electrons · Physics 2022-07-25 Xue-Yang Song , T. Senthil

Kitaev magnets have emerged as pivotal systems for investigating frustrated magnetism, providing a unique platform to explore quantum phases governed by the interplay between bond-dependent anisotropy and external magnetic fields. However,…

Strongly Correlated Electrons · Physics 2026-01-13 Shuai Liu , Hao Wu , Jinbin Li , Xiaoqun Wang , Qiang Luo

We examine the magnetic field dependent excitations of the dimerized spin-1/2 chain, copper nitrate, with antiferromagnetic intra-dimer exchange $J_1=0.44$ meV and exchange alternation $\alpha=J_2/J_1=0.24$. Magnetic excitations in three…

Strongly Correlated Electrons · Physics 2015-06-22 M. B. Stone , Y. Chen , D. H. Reich , C. Broholm , G. Xu , J. R. D. Copley , J. C. Cook

Muon spin rotation measurements have been performed on a powder sample of a-RuCl3, a layered material which previously has been proposed to be a quantum magnet on a honeycomb lattice close to a quantum spin liquid ground state. Our data…

Strongly Correlated Electrons · Physics 2016-07-20 F. Lang , P. J. Baker , A. A. Haghighirad , Y. Li , D. Prabhakaran , R. Valenti , S. J. Blundell

Motivated by the magnetic phase transition of a proximate Kitaev system $\alpha$-RuCl$_3$ in the presence of a magnetic field, we study the simplest but essential quantum spin model with the ferromagnetic nearest neighboring (NN) Kitaev…

Strongly Correlated Electrons · Physics 2020-10-14 Beom Hyun Kim , Shigetoshi Sota , Tomonori Shirakawa , Seiji Yunoki , Young-Woo Son

One of the most important issues in modern condensed matter physics is the realization of fractionalized excitations, such as the Majorana excitations in the Kitaev quantum spin liquid. To this aim, the 3d-based Kitaev material Na2Co2TeO6…

Motivated by experiments on spin-orbit coupled magnets with Kitaev exchange in magnetic fields, we present an analysis of the classical Kitaev honeycomb model in the presence of a magnetic field. We show that there is a spin liquid regime…

Strongly Correlated Electrons · Physics 2026-03-12 Paul A. McClarty , Roderich Moessner , Karlo Penc , Jeffrey G. Rau

The quest for quantum spin liquids has garnered significant attention due to their rich physics and disruptive prospects in quantum communication and computation. Spin-orbit coupling, electron correlation, and structural distortion play…

Strongly Correlated Electrons · Physics 2024-12-24 Deepak K Roy , Mukul Kabir

The quantum spin liquid (QSL) state is an exotic state of matter featuring a high degree of entanglement and lack of long-range magnetic order in the zero-temperature limit. The triangular antiferromagnet YbMgGaO4 is a candidate QSL host,…

What is the correct low-energy spin Hamiltonian description of $\alpha$-RuCl$_3$? The material is a promising Kitaev spin liquid candidate, but is also known to order magnetically, the description of which necessitates additional…

Strongly Correlated Electrons · Physics 2020-01-13 Pontus Laurell , Satoshi Okamoto

Geometrical frustration, quantum entanglement and disorder may prevent long-range order of localized spins with strong exchange interactions, resulting in a novel state of matter. $\kappa$-(BEDT-TTF)$_2$-Cu$_2$(CN)$_3$ is considered the…

Motivated by recent experimental observations in $\alpha$-RuCl$_3$, we study the $K$-$\Gamma$ model on the honeycomb lattice in an external magnetic field. By a slave-particle representation and Variational Monte Carlo calculations, we…

Strongly Correlated Electrons · Physics 2018-05-15 Zheng-Xin Liu , Bruce Normand

We report a comprehensive single-crystal neutron diffraction investigation of the Kitaev quantum magnet $\alpha$-RuCl$_{3}$ under hydrostatic pressure. Utilizing a He-gas pressure cell, we successfully applied an ideal hydrostatic pressure…

Strongly Correlated Electrons · Physics 2023-04-04 Xiao Wang , Fengfeng Zhu , Navid Qureshi , Ketty Beauvois , Junda Song , Thomas Mueller , Thomas Brückel , Yixi Su

Conventional crystalline magnets are characterized by symmetry breaking and normal modes of excitation called magnons with quantized angular momentum $\hbar$. Neutron scattering correspondingly features extra magnetic Bragg diffraction at…

Strongly Correlated Electrons · Physics 2018-10-31 K. W. Plumb , Hitesh J. Changlani , A. Scheie , Shu Zhang , J. W. Kriza , J. A. Rodriguez-Rivera , Yiming Qiu , B. Winn , R. J. Cava , C. L. Broholm
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