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Multi-electron dynamics in atoms and molecules very often occur on sub- to few-femtosecond timescales. The available intensities of extreme-ultraviolet (XUV) attosecond pulses have previously only allowed the time-resolved investigation of…

We investigate laser-driven electron dynamics in solids on the atomic scale and in real space within Floquet formalism, and develop a method based on subcycle-resolved x-ray-optical wave mixing to reconstruct those dynamics. We analyze how…

Optics · Physics 2020-12-21 Daria Popova-Gorelova , Robin Santra

In attosecond streaking, an electron is released by a short xuv pulse into a strong near infrared laser field. When the laser coupling between two states in the target is weak relative to the detuning, the streaking technique, which allows…

Atomic Physics · Physics 2015-05-19 Jan Conrad Baggesen , Lars Bojer Madsen

Using a combination of high-level ab initio electronic structure methods with efficient on-the-fly semiclassical evaluation of nuclear dynamics, we performed a massive scan of small polyatomic molecules searching for a long lasting…

Chemical Physics · Physics 2024-09-26 Alan Scheidegger , Jiří Vaníček , Nikolay V. Golubev

We propose a method to investigate the vibrational dynamics of single polyatomic molecular ions confined in a Paul trap. Quantum logic techniques are employed to detect the recoil of single photon absorption events in the molecule via a…

Quantum Physics · Physics 2019-08-27 Philipp Schindler

We propose a novel platform for the investigation of quantum wave packet dynamics, offering a complementary approach to existing theoretical models and experimental systems. It relies on laser-cooled neutral atoms which orbit around an…

Quantum Physics · Physics 2013-06-11 Fam Le Kien , Kohzo Hakuta , Philipp Schneeweiss , Arno Rauschenbeutel

Coherent electron displacement is a conventional strategy for processing quantum information, as it enables to interconnect distinct sites in a network of atoms. The efficiency of the processing relies on the precise control of the…

Quantum Physics · Physics 2020-12-02 Hicham Agueny

In the present paper, we develop a semiclassical quasi-static model accounting for molecular double ionization in an intense laser pulse. With this model, we achieve insight into the dynamics of two highly-correlated valence electrons under…

Atomic and Molecular Clusters · Physics 2009-11-13 Di-Fa Ye , Jing Chen , Jie Liu

Light-induced molecular dynamics often involve the excitation of several electronic, vibrational, and rotational states. Since the ensuing electronic and nuclear motion determines the pathways and outcomes of photoinduced reactions, our…

The ultrafast electronic and nuclear dynamics of H2 laser-induced double ionization is studied using a time-dependent wave packet approach that goes beyond the fixed nuclei approximation. The double ionization pathways are analyzed by…

Quantum Physics · Physics 2011-11-09 Sebastien Saugout , Christian Cornaggia , Annick Suzor-Weiner , Eric Charron

We investigate theoretically electron dynamics under a VUV attosecond pulse train which has a controlled phase delay with respect to an additional strong infrared laser field. Using the strong field approximation and the fact that the…

Atomic Physics · Physics 2015-05-13 P. Riviere , O. Uhden , U. Saalmann , J. M. Rost

We show that interference phenomena plays a big role for the electron yield in ionization of atoms by an ultra-short laser pulse. Our theoretical study of single ionization of atoms driven by few-cycles pulses extends the photoelectron…

Quantum Physics · Physics 2009-11-13 Diego Arbo , Emil Persson , Joachim Burgdoerfer

Controlling the interactions between atoms with external fields opened up new branches in physics ranging from strongly correlated atomic systems to ideal Bose and Fermi gases and Efimov physics. Such control usually prepares samples that…

We investigate the photoionization dynamics of atoms subjected to intense, ultrashort laser pulses through the use of quantum trajectories. This method provides a unique and consistent framework for examining electron dynamics within a…

Atomic Physics · Physics 2024-08-01 Taylor Moon , Klaus Bartschat , Nicolas Douguet

Propagation of ultrashort optical pulses in a dense resonant medium is considered in the semiclassical limit. In our analysis, we place emphasis on several main points. First, we study transformations of spectra in the process of pulse…

Optics · Physics 2011-07-20 Denis Novitsky

A phase controlled wave packet, recently used in experiment of wave packet interferometry of adiatomic molecule, is investigated to obtain mesoscopic superposition structures, useful in quantum metrology. This analysis provides a new way of…

Quantum Physics · Physics 2012-04-30 Suranjana Ghosh

We study dynamics of an artificial two-level atom in an open 1D space by measuring evolution of its coherent and incoherent emission. States of the atom -- a superconducting flux qubit coupled to a transmission line -- are fully controlled…

Quantum Physics · Physics 2015-05-27 A. A. Abdumalikov , O. V. Astafiev , Y. Nakamura , J. S. Tsai

We propose a novel method that uses the oscillation of an atomic excited wave packet observed through a pump-probe technique to accurately determine the zero time delay between a pair of ultrashort laser pulses. This physically-based…

Optics · Physics 2009-11-13 Qun Zhang , John W. Hepburn

Molecular rotational spectroscopy based on strong-field-ionization-induced nitrogen laser is employed to investigate the time evolution of the rotational wave packet composed by a coherent superposition of quantum rotational states created…

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